Polarization-controlled nonlinear computer-generated holography.

Dynamic phase-only beam shaping with a liquid crystal spatial light modulator is a powerful technique for tailoring the intensity profile or wave front of a beam. While shaping and controlling the light field is a highly researched topic, dynamic nonlinear beam shaping has hardly been explored so far. One potential reason is that generating the second harmonic is a degenerate process as it mixes two fields at the same frequency. To overcome this problem, we propose the use of type II phase matching as a control mechanism to distinguish between the two fields. Our experiments demonstrate that distributions of arbitrary intensity can be shaped in the frequency-converted field at the same quality as for linear beam shaping and with conversion efficiencies similar to without beam shaping. We envision this method as a milestone toward beam shaping beyond the physical limits of liquid crystal displays by facilitating dynamic phase-only beam shaping in the ultraviolet spectral range.

Coupling Raman, Brillouin and Nd3+ Photo Luminescence Spectroscopy to Distinguish the Effect of Uniaxial Stress from Cooling Rate on Soda-Lime Silicate Glass.

Evolution of spectroscopic properties of a soda-lime silicate glass with different thermal history and under applied uniaxial stress was investigated using Raman and Brillouin spectroscopies as well as Nd3+ photoluminescence techniques. Samples of soda-lime silicate with a cooling rate from 6 × 10-4 to 650 K/min were prepared either by controlled cooling from the melt using a differential scanning calorimeter or by a conventional annealing procedure. Uniaxial stress effects in a range from 0 to -1.3 GPa were investigated in situ by compression of the glass cylinders. The spectroscopic observations of rearrangements in the network structure were related to the set cooling rates or the applied uniaxial stress to calculate an interrelated set of calibrations. Comparing the results from Raman and Brillouin spectroscopy with Nd3+ photoluminescence analysis, we find a linear dependence that can be used to identify uniaxial stress and cooling rate in any given combination concurrently. The interrelated calibrations and linear dependence models are established and evaluated, and equations relating the change of glass network due to effects of cooling rate or uniaxial stress are given.

Label-Free Multiphoton Endomicroscopy for Minimally Invasive In Vivo Imaging.

Multiphoton microscopy of cellular autofluorescence and second harmonic generation from collagen facilitates imaging of living cells and tissues without the need for additional fluorescent labels. Here, a compact multiphoton endomicroscope for label-free in vivo imaging in small animals via side-viewing needle objectives is presented. Minimal invasive imaging at cellular resolution is performed in colonoscopy of mice without surgical measures and without fluorescent dyes as a contrast agent. The colon mucosa is imaged repeatedly in the same animal in a mouse model of acute intestinal inflammation to study the process of inflammation at the tissue level within a time period of ten days, demonstrating the capabilities of label-free endomicroscopy for longitudinal studies for the first time.

Mechanism of dynamic plasma motion in internal modification of glass by fs-laser pulses at high pulse repetition rate.

Evolution of free-electron density in internal modification of glass by fs-laser pulses at high pulse repetition rates is simulated based on rate equation model, which is coupled with thermal conduction model in order to incorporate the effect of thermal ionization. Model shows that highly absorbing small plasma generated near the geometrical focus moves toward the laser source periodically to cover the region, which is much larger than focus volume. The simulated results agree qualitatively with dynamic motion of plasma produced in internal modification of borosilicate glass by fs-laser pulses at 1 MHz through the observation using high-speed video camera. The paper also reveals the physical mechanism of the internal modification of glass when heat accumulation is significant.

Gap bridging in joining of glass using ultra short laser pulses.

Glass welding by ultra-short laser pulses provides hermetic welding seams with high mechanical stability. The required distance between the samples must be extremely small (<100nm), otherwise cracks will form inside the seam reducing its stability. However, to achieve such small gaps the roughness of the samples must be small enough necessitating additional polishing. Additionally, Van-der-Waals forces grow substantial at such distances thereby effectively preventing sample movement and an easy and precise sample alignment. Here we present a method utilizing ultra-short laser pulses which exploits a volume expansion of irradiated glass enabling the joining of glass plates across gaps of up to 1µm.

Gas bubble formation in fused silica generated by ultra-short laser pulses.

During processing of glass using ultra-fast lasers the formation of bubble-like structures can be observed in several glass types such as fused silica. Their formation can be exploited to generate periodic gratings in glasses but for other glass processing techniques such as waveguide-writing or glass welding by ultra-fast lasers the bubble formation proves often detrimental. In this work we present experiments and their results in order to gain understanding of the origins and on the underlying formation and transportation mechanisms of the gas bubbles.

Crack-free conditions in welding of glass by ultrashort laser pulse.

The spatial distribution of the laser energy absorbed by nonlinear absorption process in bulk glass w(z) is determined and thermal cycles due to the successive ultrashort laser pulse (USLP) is simulated using w(z) based on the transient thermal conduction model. The thermal stress produced in internal melting of bulk glass by USLP is qualitatively analyzed based on a simple thermal stress model, and crack-free conditions are studied in glass having large coefficient of thermal expansion. In heating process, cracks are prevented when the laser pulse impinges into glass with temperatures higher than the softening temperature of glass. In cooling process, shrinkage stress is suppressed to prevent cracks, because the embedded molten pool produced by nonlinear absorption process behaves like an elastic body under the compressive stress field unlike the case of CW-laser welding where the molten pool having a free surface produced by linear absorption process is plastically deformed under the compressive stress field.

Laser focus positioning method with submicrometer accuracy.

Accurate positioning of a sample is one of the primary challenges in laser micromanufacturing. There are a number of methods that allow detection of the surface position; however, only a few of them use the beam of the processing laser as a basis for the measurement. Those methods have an advantage that any changes in the processing laser beam can be inherently accommodated. This work describes a direct, contact-free method to accurately determine workpiece position with respect to the structuring laser beam focal plane based on nonlinear harmonic generation. The method makes workpiece alignment precise and time efficient due to ease of automation and provides the repeatability and accuracy of the surface detection of less than 1 µm.

Characteristics of laser absorption and welding in FOTURAN glass by ultrashort laser pulses.

The nonlinear absorptivity of FOTURAN glass to ultrashort laser pulses is evaluated by experimental measurement and thermal conduction model at different parameters including energy and repetition rate of the laser pulse, translation speed and thermal properties of the sample. The mechanical strength of an embedded laser-melted sample and an overlapped weld sample is determined by a three-point-bending test and a shear test, respectively. The results are related to the average absorbed laser power Wab. We found the mechanical strength of an overlapped weld joint to be as high as that of the base material for low Wab, if the sample pair is pre-bonded to provide optical contact.

Evaluation of nonlinear absorptivity in internal modification of bulk glass by ultrashort laser pulses.

Thermal conduction model is presented, by which nonlinear absorptivity of ultrashort laser pulses in internal modification of bulk glass is simulated. The simulated nonlinear absorptivity agrees with experimental values with maximum uncertainty of ± 3% in a wide range of laser parameters at 10 ps pulse duration in borosilicate glass. The nonlinear absorptivity increases with increasing energy and repetition rate of the laser pulse, reaching as high as 90%. The increase in the average absorbed laser power is accompanied by the extension of the laser-absorption region toward the laser source. Transient thermal conduction model for three-dimensional heat source shows that laser energy is absorbed by avalanche ionization seeded by thermally excited free-electrons at locations apart from the focus at pulse repetition rates higher than 100 kHz.