A diagnostic to measure neutral-atom density in fusion-research plasmas.

A femtosecond two-photon-absorption laser-induced-fluorescence (TALIF) diagnostic was designed, installed, and operated on the Princeton-Field-Reversed Configuration-2 device to provide non-invasive measurements of the time and spatially resolved neutral-atom densities in its plasmas. Calibration of the Ho density was accomplished by comparison with Kr TALIF. Measurements on plasmas formed of either H2 or Kr fill gases allowed examination of nominally long and short ionization mean-free-path regimes. With multi-kW plasma heating and H2 fill gas, a spatially uniform Ho density of order 1017 m-3 was measured with better than ±2 mm and 10 µs resolution. Under similar plasma conditions but with Kr fill gas, a 3-fold decrease in the in-plasma Kr density was observed.

Thermal hysteresis in microtubule assembly/disassembly dynamics: The aging-induced degradation of tubulin dimers.

The assembly/disassembly of biological macromolecules plays an important role in their biological functionalities. Although the dynamics of tubulin polymers and their super-assembly into microtubule structures is critical for many cellular processes, details of their cyclical polymerization/depolymerization are not fully understood. Here, we use a specially designed light scattering technique to continuously examine the effects of temperature cycling on the process of microtubule assembly/disassembly. We observe a thermal hysteresis loop during tubulin assembly/disassembly, consistently with earlier reports on the coexistence of tubulin and microtubules as a phase transition. In a cyclical process, the structural hysteresis has a kinetic component that depends on the rate of temperature change but also an intrinsic thermodynamic component that depends on the protein topology, possibly related to irreversible processes. Analyzing the evolution of such thermal hysteresis loops over successive cycles, we found that the assembly/disassembly ceases after some time, which is indicative of protein aging leading to its inability to self-assemble after a finite number of temperature cycles. The emergence of assembly-incompetent tubulin could have major consequences for human pathologies related to microtubules, including aging, neurodegenerative diseases and cancer.

Probing complex dynamics with spatiotemporal coherence-gated DLS.

We discuss the specific features of fiber-based implementations of optical sensing techniques based on spatiotemporal coherence-gated dynamic light scattering (DLS). This sensing approach has a number of unique capabilities such as an effective isolation of single scattering, a large sensitivity, and high collection efficiency, and it can also operate over a wide range of optical regimes while providing means for proper ensemble averaging. We review a number of applications in which these specific characteristics permit recovering information beyond the capabilities of traditional light-scattering-based techniques.

Passive sensing around the corner using spatial coherence.

When direct vision is obstructed, detecting an object usually involves either using mirrors or actively controlling some of the properties of light used for illumination. In our paradigm, we show that a highly scattering wall can transfer certain statistical properties of light, which, in turn, can assist in detecting objects even in non-line-of-sight conditions. We experimentally demonstrate that the transformation of spatial coherence during the reflection of light from a diffusing wall can be used to retrieve geometric information about objects hidden around a corner and assess their location. This sensing approach is completely passive, assumes no control over the source of light, and relies solely on natural broadband illumination.

Multimode interference dynamic light scattering.

When dealing with dynamic scattering systems, being able to collect strong signals while maintaining a high signal-to-noise ratio (SNR) is critical. It is well known that a spatially coherent measurement provides the largest SNR, while a partially coherent one provides better means for proper spatial averaging. In this Letter, we present a robust implementation of a fiber-based, single-mode, common-path interferometer assisted by multimode interference. We show that light can be efficiently collected from larger coherent regions while keeping a high SNR that is comparable to that of a pure single-mode arrangement. Additionally, our implementation allows having both a stable local oscillator encoding information on the fiber-medium interface and a linear dependence on scattering density. These two attributes, in turn, permit accessing the effective optical properties of the dynamic complex system.

Characterizing Viscoelastic Modulations in Biopolymer Hydrogels by Coherence-Gated Light Scattering.

pH-responsive hydrogels are of great interest for the controlled release of drugs. However, the changes in the structural and mechanical properties of hydrogels during the pH-responsive swelling/contraction process remains largely unknown. In this article, we demonstrate that coherence-gated dynamic light scattering can be used to in situ characterize the structural dynamics of chitosan (CS) hydrogels at different pH values and show that the CS hydrogels undergo viscoelastic modulations during the swelling/contraction/recovery process induced by pH changes. The conditions for the CS hydrogels to undergo these modulations are found by continuously monitoring the nonequilibrium, long-term dynamical process. Our findings are in a close correspondence to the macroscopic observations made at time points where the CS hydrogels are at equilibrium.

In situ characterization of structural dynamics in swelling hydrogels.

Characterizing the structural morphology and the local viscoelastic properties of soft complex systems raises significant challenges. Here we introduce a dynamic light scattering method capable of in situ, continuous monitoring of structural changes in evolving systems such as swelling gels. We show that the inherently non-stationary dynamics of embedded probes can be followed using partially coherent radiation, which effectively isolates only single scattering contributions even during the dramatic changes in the scattering regime. Using a simple and robust experimental setup, we demonstrate the ability to continuously monitor the structural dynamics of chitosan hydrogels formed by the Ag(+) ion-triggered gelation during their long-term swelling process. We demonstrate that both the local viscoelastic properties of the suspending medium and an effective cage size experienced by diffusing probe particles loaded into the hydrogel can be recovered and used to describe the structural dynamics of hydrogels with different levels of cross-linking. This characterization capability is critical for defining and controlling the hydrogel performance in different biomedical applications.

Near-Field Effects in Mesoscopic Light Transport.

In dense multiple scattering media, optical fields evolve through both homogeneous and evanescent waves. New regimes of light transport emerge because of the near-field coupling between individual scattering centers at mesoscopic scales. We present a novel propagation model that is developed in terms of measurable far- and near-field scattering cross sections. Our quantitative description explains the increase of total transmission in dense scattering media and its accuracy is established through both full-scale numerical calculations and enhanced backscattering experiments.

Polarization correlations in backscattering from media with different optical densities.

Random electromagnetic fields have a number of distinctive statistical properties that may depend on their origin. We show that, when two mutually coherent fields overlap, their individual characteristics are not completely lost. If assumptions can be made regarding the coherence properties of one of the fields, then the correlation length of the second one can be retrieved using the higher-order polarization properties of the combined field. We demonstrate experimentally that colloidal particles of different sizes can be identified based on polarization correlations measured even in situations of strong multiple scattering.

Exploring underwater target detection by imaging polarimetry and correlation techniques.

Underwater target detection is investigated by combining active polarization imaging and optical correlation-based approaches. Experiments were conducted in a glass tank filled with tap water with diluted milk or seawater and containing targets of arbitrary polarimetric responses. We found that target estimation obtained by imaging with two orthogonal polarization states always improves detection performances when correlation is used as detection criterion. This experimental study illustrates the potential of polarization imaging for underwater target detection and opens interesting perspectives for the development of underwater imaging systems.

Discrimination of field components in optical probe microscopy.

We demonstrate that the conventional optical signal in near-field scanning optical microscopy and the optical force induced topography contain complementary information about the complex three-dimensional field distribution. Crucially, the additional information about the field distribution can be retrieved without increasing the measurement complexity.

Negative nonconservative forces: optical "tractor beams" for arbitrary objects.

Based on the conservation of linear momentum on scattering from arbitrary objects, we demonstrate the generation of nonconservative optical forces that act in a direction opposite to the propagation of the incident beam. The concept can be applied to tailor the force fields produced on nonabsorbing bodies regardless of their sizes and shapes.

Correlations of polarization in random electro-magnetic fields.

Random electromagnetic fields have a number of distinctive statistical properties that may depend on their origin. We show here that when two mutually coherent fields are overlapped, the individual characteristics are not completely lost. In particular, we demonstrate that if assumptions can be made regarding the coherence properties of one of the fields, both the relative average strength and the field correlation length of the second one can be retrieved using higher-order polarization properties of the combined field.

On the concept of "tractor beams".

We demonstrate the existence of a class of optical beams where the nonconservative forces can be locally oriented in a direction opposite to the propagation wave vector. Objects placed in the vicinity of these locations will move toward the source of light. The behavior of these negative forces is discussed for the particular case of nondiffracting rotating scale-invariant vector electromagnetic waves.

Complex degree of mutual polarization in randomly scattered fields.

Random electromagnetic fields resulting from light-matter interaction have strong intensity fluctuations and are characterized by various statistical parameters. The local polarization of these fields can also vary randomly leading to different degrees of global depolarization. Here we demonstrate that the spatial variability of the vectorial properties contains information about the origins of randomly scattered fields. In particular, we show that the complex degree of mutual polarization provides the high-order polarization correlations necessary to identify the sources of different random fields. Scattered fields with similar global properties but different origins can be efficiently discriminated from one single realization of the light-matter interaction.

Conservative and nonconservative torques in optical binding.

We show that in the canonical case of two lossless spheres that are electromagnetically coupled there is interplay between conservative and nonconservative forces, which is controlled by the polarization of the bounding field. We demonstrate that this phenomenon leads to new mechanisms to induce torques on spherically symmetric, optically isotropic, and lossless objects. The electromagnetic interaction can be exploited to apply orbital torque about the mutual center of mass of the bounded spheres as well as spin around the individual axes. When the incident field is linearly polarized, the torques are mostly conservative and affect only transient behaviors while for circularly polarized fields, the torques are entirely nonconservative, resulting in steady rotations. Means to control the magnitudes of orbital and spin torques are presented and applications to nanorotator machines are discussed.

Fluctuations of scattered waves: going beyond the ensemble average.

The interaction between coherent waves and random media is a complicated, deterministic process that is usually examined upon ensemble averaging. The result of one realization of the interaction process depends on the specific disorder present in an experimentally controllable interaction volume. We show that this randomness can be quantified and structural information not apparent in the ensemble average can be obtained. We use the information entropy as a viable measure of randomness and we demonstrate that its rate of change provides means for discriminating between media with identical mean characteristics.

Spin hall effect of light in spherical geometry.

Electromagnetic waves carry angular momenta, and, due to spin-orbit interaction, an encounter with a gradient of refractive index leads to transport of spin similar to the electronic spin Hall effect. We show here that transversal spin transport is possible even when the symmetry of optical interaction is of higher dimensionality. We demonstrate that for a wave in a pure state of polarization, the spin-orbit interaction results in a spiraling power flow that is determined by the extent of the interaction. As a result, the spin transport can be resonantly enhanced in a spherical geometry. Our results open the possibility for developing new functionalities for photonic devices.

Coupled dipole method for modeling optical properties of large-scale random media.

We present an extension of the coupled dipole approximation technique to model optical properties of large-scale slabs of homogeneous and inhomogeneous materials. This method is based on a modification of the Green's function to take into account the interaction between dipoles located at arbitrary distances within the slab. This method allows modeling of various aspects of the structural morphology of composite materials, including component size and spatial distribution as well as surface roughness effects. Our procedure provides an adequate description of far-field optical properties such as the specular and diffuse reflection of light.

Stochastic scattering polarimetry.

We introduce the general concept of stochastic scattering polarimetry and demonstrate that the anisotropic polarizability of a scattering object can be obtained by analyzing the statistical moments of polarimetrically measured intensity distributions. This general procedure is valid even in situations where the state of polarization of the incident field is not known. The efficiency of recovering different scattering polarizabilities is demonstrated numerically for several particular cases pertaining to both far- and near-field optics.