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1.
Soft Matter ; 20(9): 2132-2140, 2024 Feb 28.
Artigo em Inglês | MEDLINE | ID: mdl-38351724

RESUMO

We combine theory and experiments to explore the kinematics and actuation of intrinsically curved folds (ICFs) in otherwise developable shells. Unlike origami folds, ICFs are not bending isometries of flat sheets, but arise via non-isometric processes (growth/moulding) or by joining sheets along curved boundaries. Experimentally, we implement both, first making joined ICFs from paper, then fabricating flat liquid crystal elastomer (LCE) sheets that morph into ICFs upon heating/swelling via programmed metric changes. Theoretically, an ICF's intrinsic geometry is defined by the geodesic curvatures on either side, κgi. Given these, and a target 3D fold-line, one can construct the entire surface isometrically, and compute the bending energy. This construction shows ICFs are bending mechanisms, with a continuous family of isometries trading fold angle against fold-line curvature. In ICFs with symmetric κgi, straightening the fold-line culminates in a fully-folded flat state that is deployable but weak, while asymmetric ICFs ultimately lock with a mechanically strong finite-angle. When unloaded, freely-hinged ICFs simply adopt the (thickness t independent) isometry that minimizes the bend energy. In contrast, in LCE ICFs a competition between flank and ridge selects a ridge curvature that, unusually, scales as t-1/7. Finally, we demonstrate how multiple ICFs can be combined in one LCE sheet, to create a versatile intrinsically curved gripper that lifts a heavy weight.

2.
Nat Commun ; 14(1): 1877, 2023 Apr 04.
Artigo em Inglês | MEDLINE | ID: mdl-37015926

RESUMO

Despite spectacular progress in microfluidics, small-scale liquid manipulation, with few exceptions, is still driven by external pumps and controlled by large-scale valves, increasing cost and size and limiting complexity. By contrast, optofluidics uses light to power, control and monitor liquid manipulation, potentially allowing for small, self-contained microfluidic devices. Here we demonstrate a soft light-propelled actuator made of liquid crystal gel that pumps microlitre volumes of water. The strip of actuating material serves as both a pump and a channel leading to an extremely simple microfluidic architecture that is both powered and controlled by light. The performance of the pump is well explained by a simple theoretical model in which the light-induced bending of the actuator competes with the liquid's surface tension. The theory highlights that effective pumping requires a threshold light intensity and strip width. The proposed system explores the benefits of shifting the complexity of microfluidic systems from the fabricated device to spatio-temporal control over stimulating light patterns.

3.
Materials (Basel) ; 15(22)2022 Nov 18.
Artigo em Inglês | MEDLINE | ID: mdl-36431699

RESUMO

"How would you build a robot, the size of a bacteria, powered by light, that would swim towards the light source, escape from it, or could be controlled by means of different light colors, intensities or polarizations?" This was the question that Professor Diederik Wiersma asked PW on a sunny spring day in 2012, when they first met at LENS-the European Laboratory of Nonlinear Spectroscopy-in Sesto Fiorentino, just outside Florence in northern Italy. It was not just a vague question, as Prof. Wiersma, then the LENS director and leader of one of its research groups, already had an idea (and an ERC grant) about how to actually make such micro-robots, using a class of light-responsive oriented polymers, liquid crystal elastomers (LCEs), combined with the most advanced fabrication technique-two-photon 3D laser photolithography. Indeed, over the next few years, the LCE technology, successfully married with the so-called direct laser writing at LENS, resulted in a 60 micrometer long walker developed in Prof. Wiersma's group (as, surprisingly, walking at that stage proved to be easier than swimming). After completing his post-doc at LENS, PW returned to his home Faculty of Physics at the University of Warsaw, and started experimenting with LCE, both in micrometer and millimeter scales, in his newly established Photonic Nanostructure Facility. This paper is a review of how the ideas of using light-powered soft actuators in micromechanics and micro-robotics have been evolving in Warsaw over the last decade and what the outcomes have been so far.

4.
Adv Mater ; 32(33): e2002779, 2020 Aug.
Artigo em Inglês | MEDLINE | ID: mdl-32627876

RESUMO

The ability to grip and handle small objects, from sub-millimeter electronic components to single-micrometer living cells, is vital for numerous ever-shrinking technologies. Mechanical grippers, powered by electric, pneumatic, hydraulic or piezoelectric servos, are well suited for the job at larger scales, but their complexity and need for force transmission prevent their miniaturization and remote control in tight spaces. Using liquid crystal elastomer microstructures that can change shape quickly and reversibly in response to light, a light-powered gripping tool-optical pliers-is built by growing two bending jaws on the tips of optical fibers. By delivering UV light to trigger polymerization via a micrometer-size fiber core, structures of similar size can be made without resorting to any microfabrication technology, such as laser photolithography. The tool is operated using visible light energy supplied through the fibers, with no force transmission. The elastomer growth technique readily offers micrometer-scale, remotely controlled functional structures with different modes of actuation as building blocks for the microtoolbox.

5.
ACS Appl Mater Interfaces ; 12(7): 8681-8686, 2020 Feb 19.
Artigo em Inglês | MEDLINE | ID: mdl-31994378

RESUMO

The photomechanical response of liquid crystal polymer networks (LCNs) can be used to directly convert light energy into different forms of mechanical energy. In this study, we demonstrate how a traveling deformation, induced in a liquid crystal polymer ring by a spatially modulated laser beam, can be used to drive the ring (the rotor) to rotate around a stationary element (the stator), thus forming a light-powered micromotor. The photomechanical response of the polymer film is modeled numerically, different LCN molecular configurations are studied, and the performance of a 5.5 mm diameter motor is characterized.

6.
Macromol Rapid Commun ; 40(16): e1900279, 2019 Aug.
Artigo em Inglês | MEDLINE | ID: mdl-31348563

RESUMO

Crawling by means of the traveling deformation of a soft body is a widespread mode of locomotion in nature-animals across scales, from microscopic nematodes to earthworms to gastropods, use it to move around challenging terrestrial environments. Snails, in particular, use mucus-a slippery, aqueous secretion-to enhance the interaction between their ventral foot and the contact surface. In this study, a millimeter-scale soft crawling robot is demonstrated that uses a similar mechanism to move efficiently in a variety of configurations: on horizontal, vertical, as well as upside-down surfaces; on smooth and rough surfaces; and through obstacles comparable in size to its dimensions. The traveling deformation of the robot soft body is generated via a local light-induced phase transition in a liquid crystal elastomer and resembles the pedal waves of terrestrial gastropods. This work offers a new approach to micro-engineering with smart materials as well as a tool to better understand this mode of locomotion in nature.


Assuntos
Elastômeros/química , Luz , Cristais Líquidos/química , Animais , Desenho de Equipamento , Tamanho da Partícula , Caramujos
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