Frequency Upshift of the Transverse Optical Phonon Resonance in GaAs by Femtosecond Electron-Hole Excitation.

The impact of transient electric currents on the transverse optical (TO) phonon resonance is studied after excitation by two femtosecond near-infrared pulses via the fourth-order nonlinear terahertz emission. Nonlinear signals due to interband shift currents and heavy-hole-light-hole polarizations are separated from Raman-induced TO phonon coherences. The latter display a frequency upshift by some 100 GHz upon interband excitation of an electron-hole plasma. The frequency shift is caused by transverse electronic shift currents, which modify the dielectric function. A local-field model based on microscopic current densities reproduces the observed frequency upshift.

Resonant Second-Order Nonlinear Terahertz Response of Gallium Arsenide.

The second-order nonlinear response of bulk GaAs in the terahertz (THz) range is mapped via the THz field emitted after near-infrared interband excitation. Phase-resolved THz detection reveals three nonlinear processes occurring in parallel, the Raman excitation of transverse optical phonons, the creation of coherent polarizations on heavy-hole-light-hole transitions, and the generation of displacive shift currents with a THz spectrum controlled by the near-infrared optical phase. Theoretical calculations reproduce the data and demonstrate the interband character of shift currents.

Strong Amplification of Coherent Acoustic Phonons by Intraminiband Currents in a Semiconductor Superlattice.

Sound amplification in an electrically biased superlattice (SL) is studied in optical experiments with 100 fs time resolution. Coherent SL phonons with frequencies of 40, 375, and 410 GHz give rise to oscillatory reflectivity changes. With currents from 0.5 to 1.3 A, the Fourier amplitude of the 410 GHz phonon increases by more than a factor of 2 over a 200 ps period. This amplification is due to stimulated Cerenkov phonon emission by electrons undergoing intraminiband transport. The gain coefficient of 8×10^{3} cm^{-1} is reproduced by theoretical calculations and holds potential for novel sub-THz phonon emitters.

Photospin-orbit coupling in photonic structures.

We show that the inclusion of nonlocality in the constitutive relations in photonic structures has important repercussions in their eigenmode configuration and distribution. In the case of optical activity, the primary manifestation of nonlocality, these features are traced to a photospin-orbit interaction analogous to the electron spin-orbit interaction in asymmetric semiconducting compounds; its impact can be assimilated to that of a magnetic field whose magnitude and direction follow that of the photon quasimomentum, with implications in photospin transport and photospintronics.

Nonlinear magneto-optical Bragg gratings.

In magneto-optical gratings the magnetic dipolar coupling superimposed on the electric dipolar one introduces nonreciprocity and spectral discrimination between circular polarization states, measured by a Zeeman-like splitting of the photonic Bragg resonances. In a nonlinear regime the degree of nonreciprocity is modified by the photoinduced interplay of these splittings and their Stark-like shifts. We predict novel magneto-optical modulation schemes for switching between orthogonal circular polarization states of transmission or reflection operated by means of an intense linearly polarized optical pulse train.