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1.
Sci Adv ; 7(19)2021 May.
Artigo em Inglês | MEDLINE | ID: mdl-33962941

RESUMO

Efficient control of photons is enabled by hybridizing light with matter. The resulting light-matter quasi-particles can be readily programmed by manipulating either their photonic or matter constituents. Here, we hybridized infrared photons with graphene Dirac electrons to form surface plasmon polaritons (SPPs) and uncovered a previously unexplored means to control SPPs in structures with periodically modulated carrier density. In these periodic structures, common SPPs with continuous dispersion are transformed into Bloch polaritons with attendant discrete bands separated by bandgaps. We explored directional Bloch polaritons and steered their propagation by dialing the proper gate voltage. Fourier analysis of the near-field images corroborates that this on-demand nano-optics functionality is rooted in the polaritonic band structure. Our programmable polaritonic platform paves the way for the much-sought benefits of on-the-chip photonic circuits.

2.
Nat Nanotechnol ; 16(5): 525-530, 2021 May.
Artigo em Inglês | MEDLINE | ID: mdl-33589812

RESUMO

Patterning graphene with a spatially periodic potential provides a powerful means to modify its electronic properties1-3. In particular, in twisted bilayers, coupling to the resulting moiré superlattice yields an isolated flat band that hosts correlated many-body phases4,5. However, both the symmetry and strength of the effective moiré potential are constrained by the constituent crystals, limiting its tunability. Here, we have exploited the technique of dielectric patterning6 to subject graphene to a one-dimensional electrostatic superlattice (SL)1. We observed the emergence of multiple Dirac cones and found evidence that with increasing SL potential the main and satellite Dirac cones are sequentially flattened in the direction parallel to the SL basis vector, behaviour resulting from the interaction between the one-dimensional SL electric potential and the massless Dirac fermions hosted by graphene. Our results demonstrate the ability to induce tunable anisotropy in high-mobility two-dimensional materials, a long-desired property for novel electronic and optical applications7,8. Moreover, these findings offer a new approach to engineering flat energy bands where electron interactions can lead to emergent properties9.

3.
Nat Nanotechnol ; 13(7): 566-571, 2018 07.
Artigo em Inglês | MEDLINE | ID: mdl-29736033

RESUMO

The ability to manipulate electrons in two-dimensional materials with external electric fields provides a route to synthetic band engineering. By imposing artificially designed and spatially periodic superlattice potentials, electronic properties can be further altered beyond the constraints of naturally occurring atomic crystals1-5. Here, we report a new approach to fabricate high-mobility superlattice devices by integrating surface dielectric patterning with atomically thin van der Waals materials. By separating the device assembly and superlattice fabrication processes, we address the intractable trade-off between device processing and mobility degradation that constrains superlattice engineering in conventional systems. The improved electrostatics of atomically thin materials allows smaller wavelength superlattice patterns relative to previous demonstrations. Moreover, we observe the formation of replica Dirac cones in ballistic graphene devices with sub-40 nm wavelength superlattices and report fractal Hofstadter spectra6-8 under large magnetic fields from superlattices with designed lattice symmetries that differ from that of the host crystal. Our results establish a robust and versatile technique for band structure engineering of graphene and related van der Waals materials with dynamic tunability.

4.
Nat Mater ; 17(5): 411-415, 2018 05.
Artigo em Inglês | MEDLINE | ID: mdl-29581552

RESUMO

Monolayers (MLs) of transition-metal dichalcogenides (TMDs) exhibit unusual electrical behaviour under magnetic fields due to their intrinsic spin-orbit coupling and lack of inversion symmetry1-15. Although recent experiments have also identified the critical role of carrier interactions within these materials11,15, a complete mapping of the ambipolar Landau level (LL) sequence has remained elusive. Here we use single-electron transistors (SETs)16,17 to perform LL spectroscopy in ML WSe2, and provide a comprehensive picture of the electronic structure of a ML TMD for both electrons and holes. We find that the LLs differ notably between the two bands, and follow a unique sequence in the valence band (VB) that is dominated by strong Zeeman effects. The Zeeman splitting in the VB is several times higher than the cyclotron energy, far exceeding the predictions of a single-particle model and, moreover, tunes significantly with doping 15 . This implies exceptionally strong many-body interactions, and suggests that ML WSe2 can serve as a host for new correlated-electron phenomena.

5.
Science ; 345(6192): 61-4, 2014 Jul 04.
Artigo em Inglês | MEDLINE | ID: mdl-24994646

RESUMO

Symmetry-breaking in a quantum system often leads to complex emergent behavior. In bilayer graphene (BLG), an electric field applied perpendicular to the basal plane breaks the inversion symmetry of the lattice, opening a band gap at the charge neutrality point. In a quantizing magnetic field, electron interactions can cause spontaneous symmetry-breaking within the spin and valley degrees of freedom, resulting in quantum Hall effect (QHE) states with complex order. Here, we report fractional QHE states in BLG that show phase transitions that can be tuned by a transverse electric field. This result provides a model platform with which to study the role of symmetry-breaking in emergent states with topological order.

6.
Nat Nanotechnol ; 9(8): 594-9, 2014 Aug.
Artigo em Inglês | MEDLINE | ID: mdl-24952474

RESUMO

Individual electrons in graphene behave as massless quasiparticles. Unexpectedly, it is inferred from plasmonic investigations that electrons in graphene must exhibit a non-zero mass when collectively excited. The inertial acceleration of the electron collective mass is essential to explain the behaviour of plasmons in this material, and may be directly measured by accelerating it with a time-varying voltage and quantifying the phase delay of the resulting current. This voltage-current phase relation would manifest as a kinetic inductance, representing the reluctance of the collective mass to accelerate. However, at optical (infrared) frequencies, phase measurements of current are generally difficult, and, at microwave frequencies, the inertial phase delay has been buried under electron scattering. Therefore, to date, the collective mass in graphene has defied unequivocal measurement. Here, we directly and precisely measure the kinetic inductance, and therefore the collective mass, by combining device engineering that reduces electron scattering and sensitive microwave phase measurements. Specifically, the encapsulation of graphene between hexagonal boron nitride layers, one-dimensional edge contacts and a proximate top gate configured as microwave ground together enable the inertial phase delay to be resolved from the electron scattering. Beside its fundamental importance, the kinetic inductance is found to be orders of magnitude larger than the magnetic inductance, which may be utilized to miniaturize radiofrequency integrated circuits. Moreover, its bias dependency heralds a solid-state voltage-controlled inductor to complement the prevalent voltage-controlled capacitor.

7.
Eur J Radiol ; 81(3): 423-9, 2012 Mar.
Artigo em Inglês | MEDLINE | ID: mdl-21237601

RESUMO

OBJECTIVE: To evaluate the feasibility of dual-energy CT (DECT) for monitoring dynamic changes in the renal corticomedullary sodium gradient in swine. MATERIAL AND METHODS: This study was approved by our Institutional Animal Care and Use Committee. Four water-restricted pigs were CT-scanned at 80 and 140 kVp at baseline and at 5 min intervals for 30 min during saline or furosemide diuresis. The renal cortical and medullary CT numbers were recorded. A DECT basis material decomposition method was used to quantify renal cortical and medullary sodium concentrations and medulla-to-cortex sodium ratios at each time point based on the measured CT numbers. The sodium concentrations and medulla-to-cortex sodium ratios were compared between baseline and at 30 min diuresis using paired Student t-tests. The medulla-to-cortex sodium ratios were considered to reflect the corticomedullary sodium gradient. RESULTS: At baseline prior to saline diuresis, the mean medullary and cortical sodium concentrations were 103.8±8.7 and 65.3±1.7 mmol/l, respectively, corresponding to a medulla-to-cortex sodium ratio of 1.59. At 30 min of saline diuresis, the medullary and cortical sodium concentrations decreased to 72.3±1.0 and 56.0±1.4 mmol/l, respectively, corresponding to a significantly reduced medulla-to-cortex sodium ratio of 1.29 (P<0.05). At baseline prior to furosemide diuresis, the mean medullary and cortical sodium concentrations were 110.5±3.6 and 66.7±4.1 mmol/l, respectively, corresponding to a medulla-to-cortex sodium ratio of 1.66. At 30 min of furosemide diuresis, the medullary and cortical sodium concentrations decreased to 68.5±0.3 and 58.9±4.0 mmol/l, respectively, corresponding to a significantly reduced medulla-to-cortex sodium ratio of 1.16 (P<0.05). One of the 4 pigs developed acute tubular necrosis likely related to prolonged hypoxia during intubation prior to the furosemide diuresis experiment. The medulla-to-cortex sodium ratio for this pig, which was excluded from the mean medulla-to-cortex ratio above, was 1.07 at baseline and 1.15 at 30 min following the administration of furosemide. CONCLUSION: DECT monitoring of dynamic changes in the renal corticomedullary sodium gradient after physiologic challenges is feasible in swine.


Assuntos
Necrose do Córtex Renal/diagnóstico por imagem , Córtex Renal/diagnóstico por imagem , Córtex Renal/metabolismo , Sódio/metabolismo , Tomografia Computadorizada por Raios X/métodos , Animais , Meios de Contraste/administração & dosagem , Diurese , Estudos de Viabilidade , Furosemida/administração & dosagem , Iohexol/administração & dosagem , Medula Renal/diagnóstico por imagem , Medula Renal/metabolismo , Projetos Piloto , Interpretação de Imagem Radiográfica Assistida por Computador , Suínos
8.
Radiology ; 261(3): 923-9, 2011 Dec.
Artigo em Inglês | MEDLINE | ID: mdl-21969665

RESUMO

PURPOSE: To determine whether flow velocity can be measured by using projection data from computed tomographic (CT) scans obtained during contrast material injection in a phantom model. MATERIALS AND METHODS: The authors constructed a 12.7-mm-diameter single-channel flow phantom with constant water flow velocity settings of 25.3, 43.9, and 70.5 cm/sec. For each flow velocity, serial axial scans were obtained with 16-section multidetector CT while a 10-mL bolus of contrast material was injected upstream of the imaging plane. For each bolus injection, the CT projection data from the scan with the sharpest increase in magnitude of detected contrast material was used for flow velocity measurements. Flow velocity was calculated as the ratio of distance between CT detector rows and the corresponding time lag in the contrast enhancement curves and was correlated with the reference velocities. Five separate contrast material injections and CT measurements were made for each flow velocity setting. RESULTS: The correlation coefficient between the CT measurements of flow velocity and the reference measurements was 0.98 (P < .05). The mean CT measurements of flow velocity were 34.2, 53.9, and 80.8 cm/sec for slow, moderate, and fast velocity settings, respectively, overestimating the corresponding actual flow velocities by 26%, 18%, and 13% and showing precision values (coefficients of variation) of 5.2%, 3.7%, and 6.6%. CONCLUSION: Flow velocity can be measured from row-to-row multidetector CT projectional data obtained during a single gantry revolution as a bolus of contrast material flows through a vascular phantom. With further development, this novel technique could potentially provide physiologic information to complement the anatomic CT angiographic findings of vascular disease.


Assuntos
Angiografia/métodos , Velocidade do Fluxo Sanguíneo , Meios de Contraste/farmacocinética , Iohexol/farmacocinética , Imagem Radiográfica a Partir de Emissão de Duplo Fóton/métodos , Tomografia Computadorizada por Raios X/métodos , Meios de Contraste/administração & dosagem , Humanos , Iohexol/administração & dosagem , Imagens de Fantasmas
9.
Radiology ; 255(2): 495-500, 2010 May.
Artigo em Inglês | MEDLINE | ID: mdl-20413762

RESUMO

PURPOSE: To retrospectively investigate the effects of furosemide on the visualization of renal medullary hyperattenuation at unenhanced computed tomography (CT). MATERIALS AND METHODS: This retrospective single-institution study was HIPAA compliant and approved by the institutional review board; requirement for informed consent was waived. This study identified 289 consecutive patients (152 men, 137 women; mean age, 59 years) without ureteral obstruction who underwent unenhanced scanning as part of CT urography; of these, 178 patients did not receive intravenous furosemide prior to imaging and 111 did. The presence of renal medullary hyperattenuation, renal stones, and bladder urine attenuation levels were recorded and compared between patients who did not receive furosemide prior to imaging and those who did by using the chi(2) and unpaired Student t tests. A multiple logistic regression model was used to evaluate independent predictors of visualization of renal medullary hyperattenuation. RESULTS: Renal medullary hyperattenuation was seen less commonly in patients who received furosemide (27 of 111, 24%) than in those who did not receive furosemide prior to imaging (79 of 178, 44%, P = .001). Bladder urine attenuation was lower in patients who received furosemide (-0.1 HU) compared with those who did not (6.4 HU, P < .001). A multiple logistic regression model revealed independent associations between the visualization of renal medullary hyperattenuation and the absence of furosemide administration (P = .002), younger age (P < .001), and presence of renal stones (P = .047). CONCLUSION: Furosemide administration prior to unenhanced CT is associated with decreased visualization of renal medullary hyperattenuation.


Assuntos
Diuréticos/administração & dosagem , Furosemida/administração & dosagem , Hematúria/diagnóstico por imagem , Medula Renal/diagnóstico por imagem , Tomografia Computadorizada por Raios X/métodos , Adolescente , Adulto , Idoso , Idoso de 80 Anos ou mais , Distribuição de Qui-Quadrado , Meios de Contraste , Feminino , Humanos , Iohexol , Modelos Logísticos , Masculino , Pessoa de Meia-Idade , Interpretação de Imagem Radiográfica Assistida por Computador , Estudos Retrospectivos
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