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1.
Artigo em Inglês | MEDLINE | ID: mdl-26382369

RESUMO

Feedback control schemes are a promising way to manipulate transport properties of driven colloidal suspensions. In the present article, we suggest a feedback scheme to enhance the collective transport of colloidal particles with repulsive interactions through a one-dimensional tilted washboard potential. The control is modeled by a harmonic confining potential, mimicking an optical "trap," with the center of this trap moving with the (instantaneous) mean particle position. Our theoretical analysis is based on the Smoluchowski equation combined with dynamical density functional theory for systems with hard-core or ultrasoft (Gaussian) interactions. For either type of interaction, we find that the feedback control can lead to an enhancement of the mobility by several orders of magnitude relative to the uncontrolled case. The largest effects occur for intermediate stiffness of the trap and large particle numbers. Moreover, in some regions of the parameter space the feedback control induces oscillations of the mean velocity. Finally, we show that the enhancement of mobility is robust against a small time delay in implementing the feedback control.

2.
Artigo em Inglês | MEDLINE | ID: mdl-25353768

RESUMO

Based on the Fokker-Planck equation we investigate the transport of an overdamped colloidal particle in a static, asymmetric periodic potential supplemented by a time-dependent, delayed feedback force, F(fc). For a given time t, F(fc) depends on the status of the system at a previous time t-τ(D), with τ(D) being a delay time, specifically on the delayed mean particle displacement (relative to some "switching position"). For nonzero delay times F(fc)(t) develops nearly regular oscillations, generating a net current in the system. Depending on the switching position, this current is nearly as large or even larger than that in a conventional open-loop rocking ratchet. We also investigate thermodynamic properties of the delayed nonequilibrium system and we suggest an underlying Langevin equation which reproduces the Fokker-Planck results.


Assuntos
Coloides/química , Retroalimentação , Modelos Químicos , Nanopartículas/química , Oscilometria/métodos , Reologia/métodos , Simulação por Computador , Difusão , Nanopartículas/ultraestrutura
3.
Artigo em Inglês | MEDLINE | ID: mdl-25615052

RESUMO

The waiting time distribution (WTD) is a common tool for analyzing discrete stochastic processes in classical and quantum systems. However, there are many physical examples where the dynamics is continuous and only approximately discrete, or where it is favourable to discuss the dynamics on a discretized and a continuous level in parallel. An example is the hindered motion of particles through potential landscapes with barriers. In the present paper we propose a consistent generalization of the WTD from the discrete case to situations where the particles perform continuous barrier crossing characterized by a finite duration. To this end, we introduce a recipe to calculate the WTD from the Fokker-Planck (Smoluchowski) equation. In contrast to the closely related first passage time distribution (FPTD), which is frequently used to describe continuous processes, the WTD contains information about the direction of motion. As an application, we consider the paradigmatic example of an overdamped particle diffusing through a washboard potential. To verify the approach and to elucidate its numerical implications, we compare the WTD defined via the Smoluchowski equation with data from direct simulation of the underlying Langevin equation and find full consistency provided that the jumps in the Langevin approach are defined properly. Moreover, for sufficiently large energy barriers, the WTD defined via the Smoluchowski equation becomes consistent with that resulting from the analytical solution of a (two-state) master equation model for the short-time dynamics developed previously by us [Phys. Rev. E 86, 061135 (2012)]. Thus, our approach "interpolates" between these two types of stochastic motion. We illustrate our approach for both symmetric systems and systems under constant force.

4.
Phys Rev E Stat Nonlin Soft Matter Phys ; 86(6 Pt 1): 061135, 2012 Dec.
Artigo em Inglês | MEDLINE | ID: mdl-23367921

RESUMO

We investigate the dynamics of a single, overdamped colloidal particle, which is driven by a constant force through a one-dimensional periodic potential. We focus on systems with large barrier heights where the lowest-order cumulants of the density field, that is, average position and the mean-squared displacement, show nontrivial (nondiffusive) short-time behavior characterized by the appearance of plateaus. We demonstrate that this "cage-like" dynamics can be well described by a discretized master equation model involving two states (related to two positions) within each potential valley. Nontrivial predictions of our approach include analytic expressions for the plateau heights and an estimate of the "de-caging time" obtained from the study of deviations from Gaussian behavior. The simplicity of our approach means that it offers a minimal model to describe the short-time behavior of systems with hindered dynamics.

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