Hierarchies of Frequentist Bounds for Quantum Metrology: From Cramér-Rao to Barankin.

We derive lower bounds on the variance of estimators in quantum metrology by choosing test observables that define constraints on the unbiasedness of the estimator. The quantum bounds are obtained by analytical optimization over all possible quantum measurements and estimators that satisfy the given constraints. We obtain hierarchies of increasingly tight bounds that include the quantum Cramér-Rao bound at the lowest order. In the opposite limit, the quantum Barankin bound is the variance of the locally best unbiased estimator in quantum metrology. Our results reveal generalizations of the quantum Fisher information that are able to avoid regularity conditions and identify threshold behavior in quantum measurements with mixed states, caused by finite data.

Scaling Laws for the Sensitivity Enhancement of Non-Gaussian Spin States.

We identify the large-N scaling of the metrological quantum gain offered by over-squeezed spin states that are accessible by one-axis twisting, as a function of the preparation time. We further determine how the scaling is modified by relevant decoherence processes and predict a discontinuous change of the quantum gain at a critical preparation time that depends on the noise. Our analytical results provide recipes for optimal and feasible implementations of quantum enhancements with non-Gaussian spin states in existing experiments, well beyond the reach of spin squeezing.

Optimal Observables and Estimators for Practical Superresolution Imaging.

Recent works identified resolution limits for the distance between incoherent point sources. However, it remains unclear how to choose suitable observables and estimators to reach these limits in practical situations. Here, we show how estimators saturating the Cramér-Rao bound for the distance between two thermal point sources can be constructed using an optimally designed observable in the presence of practical imperfections, such as misalignment, cross talk, and detector noise.

Interferometric Order Parameter for Excited-State Quantum Phase Transitions in Bose-Einstein Condensates.

Excited-state quantum phase transitions extend the notion of quantum phase transitions beyond the ground state. They are characterized by closing energy gaps amid the spectrum. Identifying order parameters for excited-state quantum phase transitions poses, however, a major challenge. We introduce a topological order parameter that distinguishes excited-state phases in a large class of mean-field models and can be accessed by interferometry in current experiments with spinor Bose-Einstein condensates. Our work opens a way for the experimental characterization of excited-state quantum phases in atomic many-body systems.

Metrological complementarity reveals the Einstein-Podolsky-Rosen paradox.

The Einstein-Podolsky-Rosen (EPR) paradox plays a fundamental role in our understanding of quantum mechanics, and is associated with the possibility of predicting the results of non-commuting measurements with a precision that seems to violate the uncertainty principle. This apparent contradiction to complementarity is made possible by nonclassical correlations stronger than entanglement, called steering. Quantum information recognises steering as an essential resource for a number of tasks but, contrary to entanglement, its role for metrology has so far remained unclear. Here, we formulate the EPR paradox in the framework of quantum metrology, showing that it enables the precise estimation of a local phase shift and of its generating observable. Employing a stricter formulation of quantum complementarity, we derive a criterion based on the quantum Fisher information that detects steering in a larger class of states than well-known uncertainty-based criteria. Our result identifies useful steering for quantum-enhanced precision measurements and allows one to uncover steering of non-Gaussian states in state-of-the-art experiments.

Metrological Detection of Multipartite Entanglement from Young Diagrams.

We characterize metrologically useful multipartite entanglement by representing partitions with Young diagrams. We derive entanglement witnesses that are sensitive to the shape of Young diagrams and show that Dyson's rank acts as a resource for quantum metrology. Common quantifiers, such as the entanglement depth and k-separability are contained in this approach as the diagram's width and height. Our methods are experimentally accessible in a wide range of atomic systems, as we illustrate by analyzing published data on the quantum Fisher information and spin-squeezing coefficients.

Superresolution Limits from Measurement Crosstalk.

Superresolution techniques based on intensity measurements after a spatial mode decomposition can overcome the precision of diffraction-limited direct imaging. However, realistic measurement devices always introduce finite crosstalk in any such mode decomposition. Here, we show that any nonzero crosstalk leads to a breakdown of superresolution when the number N of detected photons is large. Combining statistical and analytical tools, we obtain the scaling of the precision limits for weak, generic crosstalk from a device-independent model as a function of the crosstalk probability and N. The scaling of the smallest distance that can be distinguished from noise changes from N^{-1/2} for an ideal measurement to N^{-1/4} in the presence of crosstalk.

Multiparameter squeezing for optimal quantum enhancements in sensor networks.

Squeezing currently represents the leading strategy for quantum enhanced precision measurements of a single parameter in a variety of continuous- and discrete-variable settings and technological applications. However, many important physical problems including imaging and field sensing require the simultaneous measurement of multiple unknown parameters. The development of multiparameter quantum metrology is yet hindered by the intrinsic difficulty in finding saturable sensitivity bounds and feasible estimation strategies. Here, we derive the general operational concept of multiparameter squeezing, identifying metrologically useful states and optimal estimation strategies. When applied to spin- or continuous-variable systems, our results generalize widely-used spin- or quadrature-squeezing parameters. Multiparameter squeezing provides a practical and versatile concept that paves the way to the development of quantum-enhanced estimation of multiple phases, gradients, and fields, and for the efficient characterization of multimode quantum states in atomic and optical sensor networks.

Motional Fock states for quantum-enhanced amplitude and phase measurements with trapped ions.

The quantum noise of the vacuum limits the achievable sensitivity of quantum sensors. In non-classical measurement schemes the noise can be reduced to overcome this limitation. However, schemes based on squeezed or Schrödinger cat states require alignment of the relative phase between the measured interaction and the non-classical quantum state. Here we present two measurement schemes on a trapped ion prepared in a motional Fock state for displacement and frequency metrology that are insensitive to this phase. The achieved statistical uncertainty is below the standard quantum limit set by quantum vacuum fluctuations, enabling applications in spectroscopy and mass measurements.

Metrological Nonlinear Squeezing Parameter.

The well-known metrological linear squeezing parameters (such as quadrature or spin squeezing) efficiently quantify the sensitivity of Gaussian states. Yet, these parameters are insufficient to characterize the much wider class of highly sensitive non-Gaussian states. Here, we introduce a class of metrological nonlinear squeezing parameters obtained by analytical optimization of measurement observables among a given set of accessible (possibly nonlinear) operators. This allows for the metrological characterization of non-Gaussian quantum states of discrete and continuous variables. Our results lead to optimized and experimentally feasible recipes for a high-precision moment-based estimation of a phase parameter and can be used to systematically construct multipartite entanglement and nonclassicality witnesses for complex quantum states.

Sensitivity Bounds for Multiparameter Quantum Metrology.

We identify precision limits for the simultaneous estimation of multiple parameters in multimode interferometers. Quantum strategies to enhance the multiparameter sensitivity are based on entanglement among particles, modes, or combining both. The maximum attainable sensitivity of particle-separable states defines the multiparameter shot-noise limit, which can be surpassed without mode entanglement. Further enhancements up to the multiparameter Heisenberg limit are possible by adding mode entanglement. Optimal strategies that saturate the precision bounds are provided.

Hyper- and hybrid nonlocality.

The controlled generation and identification of quantum correlations, usually encoded in either qubits or continuous degrees of freedom, builds the foundation of quantum information science. Recently, more sophisticated approaches, involving a combination of two distinct degrees of freedom, have been proposed to improve on the traditional strategies. Hyperentanglement describes simultaneous entanglement in more than one distinct degree of freedom, whereas hybrid entanglement refers to entanglement shared between a discrete and a continuous degree of freedom. In this work we propose a scheme that allows us to combine the two approaches, and to extend them to the strongest form of quantum correlations. Specifically, we show how two identical, initially separated particles can be manipulated to produce Bell nonlocality among their spins, among their momenta, as well as across their spins and momenta. We discuss possible experimental realizations with atomic and photonic systems.

Frequentist and Bayesian Quantum Phase Estimation.

Frequentist and Bayesian phase estimation strategies lead to conceptually different results on the state of knowledge about the true value of an unknown parameter. We compare the two frameworks and their sensitivity bounds to the estimation of an interferometric phase shift limited by quantum noise, considering both the cases of a fixed and a fluctuating parameter. We point out that frequentist precision bounds, such as the Cramér-Rao bound, for instance, do not apply to Bayesian strategies and vice versa. In particular, we show that the Bayesian variance can overcome the frequentist Cramér-Rao bound, which appears to be a paradoxical result if the conceptual difference between the two approaches are overlooked. Similarly, bounds for fluctuating parameters make no statement about the estimation of a fixed parameter.

Robust Asymptotic Entanglement under Multipartite Collective Dephasing.

We derive an analytic solution for the ensemble-averaged collective dephasing dynamics of N noninteracting atoms in a fluctuating homogeneous external field. The obtained Kraus map is used to specify families of states whose entanglement properties are preserved at all times under arbitrary field orientations, even for states undergoing incoherent evolution. Our results apply to arbitrary spectral distributions of the field fluctuations.

Probing polariton dynamics in trapped ions with phase-coherent two-dimensional spectroscopy.

We devise a phase-coherent three-pulse protocol to probe the polariton dynamics in a trapped-ion quantum simulation. In contrast to conventional nonlinear signals, the presented scheme does not change the number of excitations in the system, allowing for the investigation of the dynamics within an N-excitation manifold. In the particular case of a filling factor one (N excitations in an N-ion chain), the proposed interaction induces coherent transitions between a delocalized phonon superfluid and a localized atomic insulator phase. Numerical simulations of a two-ion chain demonstrate that the resulting two-dimensional spectra allow for the unambiguous identification of the distinct phases, and the two-dimensional line shapes efficiently characterize the relevant decoherence mechanism.

Generic features of the dynamics of complex open quantum systems: statistical approach based on averages over the unitary group.

We obtain exact analytic expressions for a class of functions expressed as integrals over the Haar measure of the unitary group in d dimensions. Based on these general mathematical results, we investigate generic dynamical properties of complex open quantum systems, employing arguments from ensemble theory. We further generalize these results to arbitrary eigenvalue distributions, allowing a detailed comparison of typical regular and chaotic systems with the help of concepts from random matrix theory. To illustrate the physical relevance and the general applicability of our results we present a series of examples related to the fields of open quantum systems and nonequilibrium quantum thermodynamics. These include the effect of initial correlations, the average quantum dynamical maps, the generic dynamics of system-environment pure state entanglement and, finally, the equilibration of generic open and closed quantum systems.

Detecting nonclassical system-environment correlations by local operations.

We develop a general strategy for the detection of nonclassical system-environment correlations in the initial states of an open quantum system. The method employs a dephasing map which operates locally on the open system and leads to an experimentally accessible witness for genuine quantum correlations, measuring the Hilbert-Schmidt distance between pairs of open system states. We further derive the expectation value of the witness for various random matrix ensembles modeling generic features of complex quantum systems. This expectation value is shown to be proportional to a measure for the quantum discord which reduces to the concurrence for pure initial states.