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1.
Sci Rep ; 13(1): 16273, 2023 Sep 28.
Artigo em Inglês | MEDLINE | ID: mdl-37770517

RESUMO

Vortex matter in layered high-[Formula: see text] superconductors, including iron-pnictides, undergo several thermodynamic phase transitions due to the complex interplay of pinning energy, thermal energy and elastic energy. Moreover, the presence of anisotropy makes their vortex physics even more intriguing. Here, we report a detailed vortex dynamics study, using dc magnetization measurements, in a triclinic iron-pnictide superconductor (Ca[Formula: see text]La[Formula: see text])[Formula: see text](Pt[Formula: see text]As[Formula: see text])(Fe[Formula: see text]As[Formula: see text])[Formula: see text], with a superconducting transition temperature, T[Formula: see text] [Formula: see text] 31 K. A second magnetization peak (SMP) feature is observed for magnetic field perpendicular (H[Formula: see text]c) and parallel (H[Formula: see text]ab) to the crystal plane. However, its fundamental origin is quite different in both directions. For H[Formula: see text]c, the SMP can be well explained using an elastic-to-plastic vortex creep crossover, using collective creep theory. In addition, a possible rhombic-to-square vortex lattice phase transition is also observed for fields in between the onset-field and peak-field related to the SMP. On the other hand, for H[Formula: see text]ab, a clear signature of an order-disorder vortex phase transition is observed in the isothermal M(H) measurements at T [Formula: see text] 6 K. The disordered phase exhibits the characteristics of entangled pinned vortex-liquid. We construct a comprehensive vortex phase diagram by displaying characteristic temperatures and magnetic fields for both crystal geometries in this unique superconducting compound. Our study sheds light on the intricate vortex dynamics and pinning in an iron-pnictide superconductor with triclinic symmetry.

2.
Sci Rep ; 12(1): 20359, 2022 Nov 27.
Artigo em Inglês | MEDLINE | ID: mdl-36437284

RESUMO

We performed magnetization measurements in a single crystal of the anisotropic bilayer pnictide superconductor KCa[Formula: see text]Fe[Formula: see text]As[Formula: see text]F[Formula: see text], with [Formula: see text] [Formula: see text] 34 K, for [Formula: see text] [Formula: see text] [Formula: see text]-axis and [Formula: see text] [Formula: see text] [Formula: see text]-planes. A second magnetization peak (SMP) was observed in the isothermal M(H) curves measured below 16 K for [Formula: see text] [Formula: see text] [Formula: see text]-planes. A peak in the temperature variation of the critical current density, [Formula: see text](T), at 16 K, strongly suggests the emergence of Josephson vortices at lower temperatures, which leads to the SMP in the sample. In addition, it is noticed that the appearance of Josephson vortices below 16 K renders easy magnetic flux penetration. A detailed vortex dynamics study suggests that the SMP can be explained in terms of elastic pinning to plastic pinning crossover. Furthermore, contrary to the common understanding, the temperature variation of the first peak field, [Formula: see text], below and above 16 K, behaves non-monotonically. A highly disordered vortex phase, governed by plastic pinning, has been observed between 17 and 23 K, within a field region around an extremely large first peak field. Pinning force scaling suggests that the point defects are the dominant source of pinning for H [Formula: see text] [Formula: see text]-planes, whereas, for H [Formula: see text] [Formula: see text]-axis, point defects in addition to surface defects are at play. Such disorder contributes to the pinning due to the variation in charge carrier mean free path, [Formula: see text] -pinning. Moreover, the large [Formula: see text] observed in our study is consistent with the literature, which advocates this material for high magnetic field applications.

3.
J Phys Condens Matter ; 29(20): 205401, 2017 May 24.
Artigo em Inglês | MEDLINE | ID: mdl-28346216

RESUMO

The oxyborate Fe3O2BO3 presents a charge density wave (CDW) transition close to room temperature. As we show here, this is associated with a well defined anomaly in the specific heat. Below this transition, when applying in a single crystal of Fe3O2BO3 a DC voltage above a temperature dependent threshold, a high current is liberated in this material. We study the conduction in single crystals of Fe3O2BO3 with voltage applied parallel and perpendicular to the crystallographic c axis direction. The observed currents are attributed to the depinning of charge ordered domains above a threshold voltage V T2 that gives rise to a collective conduction due to coherent domains. Compliance limited DC data shows that above a lower threshold voltage depinning is smooth and follows a power law scaling. Similar depinning with power law scaling is also revealed in the AC conductivity.

4.
J Phys Condens Matter ; 25(49): 496009, 2013 Dec 11.
Artigo em Inglês | MEDLINE | ID: mdl-24214902

RESUMO

The phase transition in CuCrO2 to an ordered magnetic state is studied with bulk measurements and elastic and inelastic neutron scattering techniques. The reported onset of spontaneous electric polarization at T = 23.5 K coincides with the appearance, on cooling, of elastic magnetic scattering. At higher temperatures long range magnetic correlations gradually develop but they are dynamic. The ground state is characterized by three-dimensional long range magnetic ordering but along the c direction the correlation length remains limited to ∼200 Å.

5.
J Phys Condens Matter ; 24(48): 486001, 2012 Dec 05.
Artigo em Inglês | MEDLINE | ID: mdl-23137933

RESUMO

Among double perovskites, the interpretation of the magnetic, thermal and transport properties of Sr(2)YRuO(6) remains a challenge. Characterization using different techniques reveals a variety of features that are not understood, described as anomalous, and yields contradictory values for several relevant parameters. We solved this situation through detailed susceptibility, specific heat, thermal expansion and x-ray diffraction measurements, including a quantitative correlation of the parameters characterizing the so-called anomalies. The emergence of short-range magnetic correlations, surviving well above the long-range transition, naturally accounts for the observed unconventional behavior of this compound. High resolution x-ray powder diffraction and thermal expansion results conclusively show that the magnetic and thermal responses are driven by lattice changes, providing a comprehensive scenario in which the interplay between the spin and structural degrees of freedom plays a relevant role.

6.
J Phys Condens Matter ; 19(18): 186226, 2007 May 08.
Artigo em Inglês | MEDLINE | ID: mdl-21691007

RESUMO

We report a detailed study of the electric transport and magnetic properties of the La(5/8-y)Nd(y)Ca(3/8)MnO(3) manganite system. Substitution of La(3+) by smaller Nd(3+) ions reduces the mean ionic radius of the A-site ion. We have studied samples in the entire range between La-rich and Nd-rich compounds (0.1

7.
Phys Rev Lett ; 87(14): 147201, 2001 Oct 01.
Artigo em Inglês | MEDLINE | ID: mdl-11580673

RESUMO

We observe for the first time a structural phase transition in the oxyborate Fe3O2BO3 which occurs along three leg ladders present in this material. X-ray diffraction shows that this transition at 283 K is associated with a new phase where atomic displacements occur in alternate directions perpendicular to the axis and within the plane of the ladders. Magnetic data show that these displacements lead to the formation of singlet pairs which dissociate close to the structural transition. Anomalies in the transport properties also occur close to 283 K showing that the structural transition is related to a charge ordering phenomenon in a low dimensional structure.

8.
Phys Rev B Condens Matter ; 41(7): 4056-4061, 1990 Mar 01.
Artigo em Inglês | MEDLINE | ID: mdl-9994224
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