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1.
Nat Commun ; 13(1): 3630, 2022 Jun 24.
Artigo em Inglês | MEDLINE | ID: mdl-35750676

RESUMO

Research into practical applications of magnetic skyrmions, nanoscale solitons with interesting topological and transport properties, has traditionally focused on two dimensional (2D) thin-film systems. However, the recent observation of novel three dimensional (3D) skyrmion-like structures, such as hopfions, skyrmion strings (SkS), skyrmion bundles, and skyrmion braids, motivates the investigation of new designs, aiming to exploit the third spatial dimension for more compact and higher performance spintronic devices in 3D or curvilinear geometries. A crucial requirement of such device schemes is the control of the 3D magnetic structures via charge or spin currents, which has yet to be experimentally observed. In this work, we utilise real-space imaging to investigate the dynamics of a 3D SkS within a nanowire of Co8Zn9Mn3 at room temperature. Utilising single current pulses, we demonstrate current-induced nucleation of a single SkS, and a toggle-like positional switching of an individual Bloch point at the end of a SkS. The observations highlight the possibility to locally manipulate 3D topological spin textures, opening up a range of design concepts for future 3D spintronic devices.

2.
Nat Commun ; 12(1): 2723, 2021 May 11.
Artigo em Inglês | MEDLINE | ID: mdl-33976177

RESUMO

Magnetic skyrmions are topologically non-trivial, swirling magnetization textures that form lattices in helimagnetic materials. These magnetic nanoparticles show promise as high efficiency next-generation information carriers, with dynamics that are governed by their topology. Among the many unusual properties of skyrmions is the tendency of their direction of motion to deviate from that of a driving force; the angle by which they diverge is a materials constant, known as the skyrmion Hall angle. In magnetic multilayer systems, where skyrmions often appear individually, not arranging themselves in a lattice, this deflection angle can be easily measured by tracing the real space motion of individual skyrmions. Here we describe a reciprocal space technique which can be used to determine the skyrmion Hall angle in the skyrmion lattice state, leveraging the properties of the skyrmion lattice under a shear drive. We demonstrate this procedure to yield a quantitative measurement of the skyrmion Hall angle in the room-temperature skyrmion system FeGe, shearing the skyrmion lattice with the magnetic field gradient generated by a single turn Oersted wire.

3.
Nat Commun ; 11(1): 1726, 2020 Apr 07.
Artigo em Inglês | MEDLINE | ID: mdl-32265449

RESUMO

Magnetic skyrmions are topologically nontrivial particles with a potential application as information elements in future spintronic device architectures. While they are commonly portrayed as two dimensional objects, in reality magnetic skyrmions are thought to exist as elongated, tube-like objects extending through the thickness of the host material. The study of this skyrmion tube state (SkT) is vital for furthering the understanding of skyrmion formation and dynamics for future applications. However, direct experimental imaging of skyrmion tubes has yet to be reported. Here, we demonstrate the real-space observation of skyrmion tubes in a lamella of FeGe using resonant magnetic x-ray imaging and comparative micromagnetic simulations, confirming their extended structure. The formation of these structures at the edge of the sample highlights the importance of confinement and edge effects in the stabilisation of the SkT state, opening the door to further investigation into this unexplored dimension of the skyrmion spin texture.

4.
J Phys Condens Matter ; 31(28): 285803, 2019 Jul 17.
Artigo em Inglês | MEDLINE | ID: mdl-30933932

RESUMO

We present the results of x-ray scattering and muon-spin relaxation ([Formula: see text]SR) measurements on the iron-pnictide compound FeCrAs. Polarized non-resonant magnetic x-ray scattering results reveal the 120° periodicity expected from the suggested three-fold symmetric, non-collinear antiferromagnetic structure. [Formula: see text]SR measurements indicate a magnetically ordered phase throughout the bulk of the material below [Formula: see text] K. There are signs of fluctuating magnetism in a narrow range of temperatures above [Formula: see text] involving low-energy excitations, while at temperatures well below [Formula: see text] behaviour characteristic of freezing of dynamics is observed, likely reflecting the effect of disorder in our polycrystalline sample. Using density functional theory we propose a distinct muon stopping site in this compound and assess the degree of distortion induced by the implanted muon.

5.
Phys Rev Lett ; 105(8): 087203, 2010 Aug 20.
Artigo em Inglês | MEDLINE | ID: mdl-20868129

RESUMO

We report the direct measurement of antiferromagnetic spin polarization at the oxygen sites in the multiferroic TbMn2O5, through resonant soft x-ray magnetic scattering. This supports recent theoretical models suggesting that the oxygen spin polarization is key to the magnetoelectric coupling mechanism. The spin polarization is observed through a resonantly enhanced diffraction signal at the oxygen K edge at the commensurate antiferromagnetic wave vector. Using the fdmnes code we have accurately reproduced the experimental data. We have established that the resonance arises through the spin polarization on the oxygen sites hybridized with the square based pyramid Mn3+ ions. Furthermore we have discovered that the position of the Mn3+ ion directly influences the oxygen spin polarization.

6.
Rev Sci Instrum ; 81(7): 073904, 2010 Jul.
Artigo em Inglês | MEDLINE | ID: mdl-20687739

RESUMO

We report the design and construction of a novel soft x-ray diffractometer installed at Diamond Light Source. The beamline endstation RASOR is constructed for general users and designed primarily for the study of single crystal diffraction and thin film reflectivity. The instrument is comprised of a limited three circle (theta, 2theta, and chi) diffractometer with an additional removable rotation (phi) stage. It is equipped with a liquid helium cryostat, and post-scatter polarization analysis. Motorized motions are provided for the precise positioning of the sample onto the diffractometer center of rotation, and for positioning the center of rotation onto the x-ray beam. The functions of the instrument have been tested at Diamond Light Source, and initial test measurements are provided, demonstrating the potential of the instrument.

7.
J Phys Condens Matter ; 22(3): 036003, 2010 Jan 27.
Artigo em Inglês | MEDLINE | ID: mdl-21386301

RESUMO

We report the observation of a modulated structure and a ferromagnetic insulating state in a high quality single crystal of a nine-layer BaRuO(3). Using x-ray scattering, the modulated satellites were observed to double the unit cell along the c-axis at low temperature. The ferromagnetic insulating state is confirmed by magnetic and resistivity measurements. Analyzing the peak profiles from the modulation and host structure respectively, showed a lattice distortion at T∼55 K. These findings elucidate the intimate relationship between ferromagnetism and lattice distortion in a nine-layer BaRuO(3).

8.
J Phys Condens Matter ; 21(48): 485601, 2009 Dec 02.
Artigo em Inglês | MEDLINE | ID: mdl-21832526

RESUMO

Despite being one of the oldest known magnetic materials, and the classic mixed valence compound, thought to be charge ordered, the structure of magnetite below the Verwey transition is complex and the presence and role of charge order is still being debated. Here, we present resonant x-ray diffraction data at the iron K-edge on forbidden (0, 0, 2n+1)(C) and superlattice [Formula: see text] reflections. Full linear polarization analysis of the incident and scattered light was conducted in order to explore the origins of the reflections. Through simulation of the resonant spectra we have confirmed that a degree of charge ordering takes place, while the anisotropic tensor of susceptibility scattering is responsible for the superlattice reflections below the Verwey transition. We also report the surprising result of the conversion of a significant proportion of the scattered light from linear to nonlinear polarization.

9.
Phys Rev Lett ; 103(20): 207602, 2009 Nov 13.
Artigo em Inglês | MEDLINE | ID: mdl-20366013

RESUMO

The magnetic structures which endow TbMnO(3) with its multiferroic properties have been reassessed on the basis of a comprehensive soft x-ray resonant scattering (XRS) study. The selectivity of XRS facilitated separation of the various contributions (Mn L(2) edge, Mn 3d moments; Tb M(4) edge, Tb 4f moments), while its variation with azimuth provided information on the moment direction of distinct Fourier components. When the data are combined with a detailed group theory analysis, a new picture emerges of the ferroelectric transition at 28 K. Instead of being driven by the transition from a collinear to a noncollinear magnetic structure, as has previously been supposed, it is shown to occur between two noncollinear structures.

10.
J Synchrotron Radiat ; 12(Pt 4): 434-41, 2005 Jul.
Artigo em Inglês | MEDLINE | ID: mdl-15968119

RESUMO

The use of softer-energy X-rays produced by synchrotron radiation for diffraction is an area of current interest. In this paper, experiments exploiting resonant scattering at the L absorption edges of 3d transition metal elements are reported. Such energies, typically 500-1000 eV, are at the extreme limit of soft X-ray diffraction where absorption effects are so severe that the sample and diffractometer must be placed in a windowless high-vacuum vessel. In addition, the Ewald sphere is so small as to likely contain, at most, only a single Bragg reflection. Advantages of using such radiation for the study of weak diffraction effects such as anomalous scattering, charge ordering, magnetic diffraction and orbital ordering are reported.


Assuntos
Magnetismo/instrumentação , Modelos Químicos , Difração de Raios X/instrumentação , Difração de Raios X/métodos , Simulação por Computador , Desenho de Equipamento , Conformação Molecular , Difração de Raios X/tendências
11.
Phys Rev Lett ; 91(16): 167205, 2003 Oct 17.
Artigo em Inglês | MEDLINE | ID: mdl-14611437

RESUMO

We report the first direct resonant soft x-ray scattering observations of orbital ordering. We have studied the low temperature phase of La0.5Sr1.5MnO4, a compound that displays charge and orbital ordering. Previous claims of orbital ordering in such materials have relied on observations at the manganese K edge. These claims have been questioned in several theoretical studies. Instead we have employed resonant soft x-ray scattering at the manganese L(III) and L(II) edges which probes the orbital ordering directly. Energy scans at constant wave vector are compared to theoretical predictions and suggest that at all temperatures there are two separate contributions to the scattering: direct orbital ordering and strong cooperative Jahn-Teller distortions of the Mn3+ ions.

12.
Phys Rev Lett ; 90(18): 187201, 2003 May 09.
Artigo em Inglês | MEDLINE | ID: mdl-12786040

RESUMO

We have conducted the first soft x-ray diffraction experiments from a bulk single crystal, studying the bilayer manganite La2-2xSr1+2xMn2O7 with x=0.475 in which we were able to access the (002) Bragg reflection using soft x rays. The Bragg reflection displays a strong resonant enhancement at the L(III) and L(II) manganese absorption edges. We demonstrate that the resonant enhancement of the magnetic diffraction of the (001) is extremely large, indeed so large that it exceeds that of the nonresonant Bragg diffraction. Resonant soft x-ray scattering of 3d transition metal oxides is the only technique for the atomic selective measurement of spin, charge, and orbital correlations in materials, such as high temperature superconductors, colossal magnetoresistance manganites, and charge stripe nickelates.

13.
Ann Thorac Surg ; 64(5): 1527-8, 1997 Nov.
Artigo em Inglês | MEDLINE | ID: mdl-9386758
14.
Ann Thorac Surg ; 47(6): 838-40, 1989 Jun.
Artigo em Inglês | MEDLINE | ID: mdl-2757437

RESUMO

Thymectomy is an accepted therapeutic modality for patients with myasthenia gravis. The selection of patients for operation and the surgical approach are controversial. We reviewed 52 patients (aged 18 months to 82 years; mean age, 34 years) treated with transsternal radical thymectomy between 1972 and 1987. Patients were symptomatically staged according to the modified Osserman classification. There was one hospital death and postoperative follow-up was obtained on 51 patients. Improvement after thymectomy was observed in 3 of 11 patients (27%) in Osserman stage I, 16 of 25 patients (64%) in Osserman stage IIA, and 13 of 15 patients (86%) in combined Osserman stages IIB, III, and IV. Preoperative Osserman stage, patient sex, and thymic histology correlated with postoperative clinical response. Transsternal radical thymectomy is effective therapy for myasthenia gravis. Sustained improvement is obtained in patients with moderate and advanced disease. The majority of patients with ocular disease do not benefit from operation.


Assuntos
Miastenia Gravis/cirurgia , Timectomia/métodos , Adulto , Feminino , Seguimentos , Humanos , Masculino , Fatores de Tempo
15.
Aviat Space Environ Med ; 56(10): 1009-10, 1985 Oct.
Artigo em Inglês | MEDLINE | ID: mdl-4062766

RESUMO

A high performance aircraft test pilot who presented with acalculous cholecystitis was found to have a calcified omental hematoma adjacent to the gallbladder. Omental hematomas have not previously been linked to flight in high performance aircraft. Current prevailing hypotheses regarding etiologies of omental hematomas include rapid blood flow shifts and venous fragility. Forces encountered in high performance aircraft may increase the chance of omental hemorrhage.


Assuntos
Medicina Aeroespacial , Calcinose/etiologia , Hematoma/etiologia , Doenças Profissionais/etiologia , Omento , Adulto , Gravitação , Humanos , Masculino
16.
Am J Surg ; 148(6): 760-3, 1984 Dec.
Artigo em Inglês | MEDLINE | ID: mdl-6507747

RESUMO

A significant percentage of surgery performed for complications of gastroesophageal reflux at a major medical center has been performed for problems related to prior surgery. Our patients who required remedial surgery fell into three categories. Those with recurrent reflux generally fared well. Patients with dysphagia, gastric stasis, or both presented difficult problems. The key to success for these patients lies in choosing the operation best suited to the anatomic and physiologic situation as defined by preoperative contrast studies, pH monitoring, endoscopy, and selective gastric emptying studies.


Assuntos
Fundo Gástrico/cirurgia , Refluxo Gastroesofágico/cirurgia , Adulto , Estudos de Avaliação como Assunto , Feminino , Seguimentos , Humanos , Masculino , Métodos , Complicações Pós-Operatórias/cirurgia , Reoperação
17.
Arch Surg ; 119(10): 1208-9, 1984 Oct.
Artigo em Inglês | MEDLINE | ID: mdl-6477107

RESUMO

Secondary aortocolonic fistula is an uncommon complication of prosthetic aortic grafts; apparently there have been only two previously described long-term survivors. We describe a long-term survivor with this complication in which preoperative computed tomographic scanning and percutaneous abscess drainage allowed early diagnosis and intervention and contributed to optimal treatment and survival. Adherence to time-honored principles of abscess drainage and graft removal, followed by extra-anatomic bypass when indicated, are essential to successful treatment.


Assuntos
Doenças da Aorta/cirurgia , Doenças do Colo/cirurgia , Fístula/cirurgia , Abscesso/terapia , Doenças da Aorta/diagnóstico por imagem , Doenças da Aorta/etiologia , Prótese Vascular/efeitos adversos , Doenças do Colo/diagnóstico por imagem , Doenças do Colo/etiologia , Drenagem , Feminino , Fístula/diagnóstico por imagem , Fístula/etiologia , Humanos , Pessoa de Meia-Idade , Tomografia Computadorizada por Raios X
18.
South Med J ; 77(7): 857-9, 1984 Jul.
Artigo em Inglês | MEDLINE | ID: mdl-6740354

RESUMO

We have reviewed our experience with xeromammography over a five-year period in a setting where there is no protocol for mammographic screening. Only 8.9% of breast carcinomas were found by xeromammography alone, a ratio substantially smaller than that found in large screening programs. While 80% of the occult carcinomas were localized, only 47% of women with palpable disease had localized tumors. It appears that screening mammography is underused, and that more localized tumors would be detected if more mammograms were ordered.


Assuntos
Neoplasias da Mama/diagnóstico , Mamografia , Xeromamografia , Adulto , Biópsia , Estudos de Avaliação como Assunto , Feminino , Humanos , Pessoa de Meia-Idade , Estudos Retrospectivos
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