Coherence time characterization method for hard X-ray free-electron lasers.

Coherence time is one of the fundamental characteristics of light sources. Methods based on autocorrelation have been widely applied from optical domain to soft X-rays to characterize the radiation coherence time. However, for the hard X-ray regime, due to the lack of proper mirrors, it is extremely difficult to implement such autocorrelation scheme. In this paper, a novel approach for characterizing the coherence time of a hard X-ray free-electron laser (FEL) is proposed and validated numerically. A phase shifter is adopted to control the correlation between X-ray and microbunched electrons. The coherence time of the FEL pulse can be extracted from the cross-correlation. Semi-analytical analysis and three-dimensional time-dependent numerical simulations are presented to elaborate the details. A coherence time of 218.2 attoseconds for 6.92 keV X-ray FEL pulses is obtained in our simulation based on the configuration of Linac Coherent Light Source. This approach provides critical temporal coherence diagnostics for X-ray FELs, and is decoupled from machine parameters, applicable for any photon energy, radiation brightness, repetition rate and FEL pulse duration.

Attosecond Coherence Time Characterization in Hard X-Ray Free-Electron Laser.

One of the key challenges in scientific researches based on free-electron lasers (FELs) is the characterization of the coherence time of the ultra-fast hard x-ray pulse, which fundamentally influences the interaction process between x-rays and materials. Conventional optical methods, based on autocorrelation, are very difficult to realize due to the lack of mirrors. Here, we experimentally demonstrate a novel method which yields a coherence time of 174.7 attoseconds for the 6.92 keV FEL pulses at the Linac Coherent Light Source. In our experiment, a phase shifter is adopted to control the cross-correlation between x-ray and microbunched electrons. This approach provides critical diagnostics for the temporal coherence of x-ray FELs and is universal for general machine parameters; applicable for wide range of photon energy, radiation brightness, repetition rate and FEL pulse duration.