High-order harmonic generation from solid targets with 2 mJ pulses.

Harmonics up to the 18th order are generated from solid targets by focusing 2 mJ, 50 fs pulses at 800 nm to a spot size of 1.7 µm (FWHM). To our knowledge, this is the first demonstration of high-harmonic generation with a very short focal length paraboloid (f/1.4) and kilohertz laser system. The harmonics have a low divergence (<4°) compared to the driving beam and conversion efficiencies (>10(-7) per harmonic) comparable to gas harmonics. No contrast enhancement techniques are employed, and the system is capable of operating at 500 Hz.

Quasimonoenergetic electron beams with relativistic energies and ultrashort duration from laser-solid interactions at 0.5 kHz.

We investigate the production of electron beams from the interaction of relativistically-intense laser pulses with a solid-density SiO(2) target in a regime where the laser pulse energy is approximately mJ and the repetition rate approximately kHz. The electron beam spatial distribution and spectrum were investigated as a function of the plasma scale length, which was varied by deliberately introducing a moderate-intensity prepulse. At the optimum scale length of lambda/2, the electrons are emitted in a collimated beam having a quasimonoenergetic distribution that peaked at approximately 0.8 MeV. A highly reproducible structure in the spatial distribution exhibits an evacuation of electrons along the laser specular direction and suggests that the electron beam duration is comparable to that of the laser pulse. Particle-in-cell simulations which are in good agreement with the experimental results offer insights on the acceleration mechanism by the laser field.

Vacuum-free x-ray source based on ultrashort laser irradiation of solids.

A vacuum-free ultrafast laser-based x-ray source is demonstrated. Hard x-rays up to 80KeV are generated from Cu, Mo, Ag, Sn, and Ge targets in a laminar helium flow surrounded by atmosphere using tightly focused 33fs, 3mJ laser pulses. X-ray spectra, conversion efficiencies, and source sizes are presented. Six-fold efficiency improvement is observed, over similar sources found in the literature [1]. Source sizes determined for Cu and Mo show distinct dependences on laser pulse energy. It is also shown that the Cu source size has no dependence on the presence of the spectral band around the 8KeV K-shell lines.

Generation of hard X-rays using an ultrafast fiber laser system.

We report the first hard X-ray source driven by a femtosecond fiber laser. The high energy fiber CPA system incorporated a 65mum LMA fiber amplifying stage which provided 300-fs recompressed pulses and diffraction limited beam quality with M(2) < 1.07. A deformable mirror was used to optimize the wavefront and the spot size was focused down to 2.3 mum with an f/1.2 paraboloidal mirror. 50muJ was deposited on the nickel target with 2x10(15)-W/cm(2) focal intensity and a distinctive Ni K(alpha)-line (7.48 keV) emission was measured with 5x10(-8) energy conversion efficiency.

Demonstration of fiber-laser-produced plasma source and application to efficient extreme UV light generation.

Efficient generation of extreme UV (EUV) light at lambda = 13.5 nm from a bulk Sn target has been demonstrated by using a fiber laser. The conversion efficiency from the 1064 nm IR to the EUV was measured to be around 0.9% into 2pi steradians within a 2% bandwidth. To the best of our knowledge, this is the first time an all-fiber system was used to generate EUV or soft x rays.

Isolated attosecond pulses generated by relativistic effects in a wavelength-cubed focal volume.

Lasers that provide an energy encompassed in a focal volume of a few cubic wavelengths (lambda3) can create relativistic intensity with maximal gradients using minimal energy. With particle-in-cell simulations we found that single 200-as pulses could be produced efficiently in a lambda3 laser pulse reflection by means of deflection and phase compression caused by the coherent motion of the plasma electrons that emit these pulses. This novel technique is efficient (approximately 10%) and can produce single attosecond pulses from the millijoule to the joule level.

Following evolution of bacteriorhodopsin in its reactive excited state via stimulated emission pumping.

New information concerning the photochemical dynamics of bacteriorhodopsin (BR) is obtained by impulsively stimulating emission from the reactive fluorescent state. Depletion of the excited-state fluorescence leads to an equal reduction in production of later photoproducts. Accordingly, chromophores which are forced back to the ground state via emission do not continue on in the photocycle, conclusively demonstrating that the fluorescent state is a photocycle intermediate. The insensitivity of depletion dynamics to the "dump" pulse timing, throughout the fluorescent states lifetime, and the biological inactivity of the dumped population suggest that the fluorescent-state structure is constant, well-defined, and significantly different than that where crossing to the ground state takes place naturally. In conjunction with conclusions from comparing the photophysics of BR with those of synthetic analogues containing "locked" retinals, present results show that large-amplitude torsion around C13=C14 is required to go between the above structures.