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1.
Nano Lett ; 24(25): 7609-7615, 2024 Jun 26.
Artigo em Inglês | MEDLINE | ID: mdl-38861682

RESUMO

Long-wave infrared (LWIR) imaging, or thermal imaging, is widely applied in night vision and security monitoring. However, the widespread use of LWIR imagers is impeded by their bulky size, considerable weight, and high cost. While flat meta-optics present a potential solution to these limitations, existing pure LWIR meta-optics face constraints such as severe chromatic or coma aberrations. Here, we introduce an approach utilizing large-scale hybrid meta-optics to address these challenges and demonstrate the achromatic, coma-corrected, and polarization-insensitive thermal imaging. The hybrid metalens doublet is composed of a metasurface corrector and a refractive lens, featuring a full field-of-view angle surpassing 20° within the 8-12 µm wavelength range. Employing this hybrid metalens doublet, we showcase high-performance thermal imaging capabilities both indoors and outdoors, effectively capturing ambient thermal radiation. The proposed hybrid metalens doublet holds considerable promise for advancing miniaturized, lightweight, and cost-effective LWIR optical imaging systems.

2.
Nat Commun ; 15(1): 3055, 2024 Apr 09.
Artigo em Inglês | MEDLINE | ID: mdl-38594345

RESUMO

Providing additional degrees of freedom to manipulate light, spatiotemporal optical vortex (STOV) beams carrying transverse orbital angular momentum are of fundamental importance for spatiotemporal control of light-matter interactions. Unfortunately, existing methods to generate STOV are plagued by various limitations such as inefficiency, bulkiness, and complexity. Here, we theoretically propose and experimentally demonstrate a microscale singlet platform composed of a slanted nanograting to generate STOV. Leveraging the intrinsic topological singularity induced by C2 symmetry and z-mirror symmetry breaking of the slanted nanograting, STOV is generated through the Fourier transform of the spiral phase in the momentum-frequency space to the spatiotemporal domain. In experiments, we observe the space-time evolution of STOV carried by femtosecond pulses using a time-resolved interferometry technique and achieve a generation efficiency exceeding 40%. Our work sheds light on a compact and versatile platform for light pulse shaping, and paves the way towards a fully integrated system for spatiotemporal light manipulation.

3.
J Periodontal Res ; 59(2): 249-258, 2024 Apr.
Artigo em Inglês | MEDLINE | ID: mdl-38115631

RESUMO

OBJECTIVE: To assess the effects of amoxicillin and metronidazole with scaling and root planing (SRP) on periodontal parameters and glycemic control in patients with severe periodontitis and diabetes mellitus. BACKGROUND: Adjunctive antibiotics use is advantageous for treating periodontitis in patients with severe periodontitis and diabetes. However, the effects of adjunctive antibiotic use on hemoglobin A1c (HbA1c) levels remain unclear. METHODS: This short-term, randomized controlled trial enrolled patients with severe periodontitis and type 2 diabetes. The patients were randomly allocated to SPR only (i.e., control) or SPR + antibiotics (500 mg of amoxicillin and 200 mg of metronidazole, three times daily for 7 days) groups. Periodontal and hematological parameters were assessed at baseline and 3 months after treatment. Inter- and intra-group analyses were performed using Student's t-tests, Mann-Whitney U tests, and the binary logistic regression models. p-values of <.05 were considered statistically significant. RESULTS: This study enrolled 49 patients, with 23 and 26 patients in the SRP-only and SRP + antibiotics groups, respectively. The periodontal parameters improved significantly and similarly in both groups after treatment (p < .05). The SRP + antibiotics group had more sites of improvement than the SRP-only group when the initial probing depth was >6 mm. (698 [78.96%] vs. 545 [73.35%], p = .008). The HbA1c levels decreased in the SRP-only and SRP + antibiotics groups after treatment (0.39% and 0.53%, respectively). The multivariable binary logistic regression model demonstrated that antibiotics administration and a high baseline HbA1c level were associated with a greater reduction in the HbA1c level (odds ratio = 4.551, 95% confidence interval: 1.012-20.463; odds ratio = 7.162, 95% confidence interval: 1.359-37.753, respectively). CONCLUSIONS: SRP and SRP plus systemic antibiotics were beneficial for glycemic control. Adjunctive antibiotic use slightly improved the outcome for patients with severe periodontitis and poorly controlled diabetes.


Assuntos
Periodontite Crônica , Diabetes Mellitus Tipo 2 , Periodontite , Humanos , Metronidazol/uso terapêutico , Amoxicilina/uso terapêutico , Aplainamento Radicular , Diabetes Mellitus Tipo 2/complicações , Diabetes Mellitus Tipo 2/tratamento farmacológico , Controle Glicêmico , Hemoglobinas Glicadas , Resultado do Tratamento , Antibacterianos/uso terapêutico , Periodontite/complicações , Periodontite/tratamento farmacológico , Raspagem Dentária , Periodontite Crônica/tratamento farmacológico
4.
Opt Lett ; 48(17): 4709-4712, 2023 Sep 01.
Artigo em Inglês | MEDLINE | ID: mdl-37656592

RESUMO

Metasurfaces have recently emerged as a crucial tool because they achieve spherical-aberration-free focusing when exposed to normal incident light. Nevertheless, these metasurfaces often exhibit considerable coma when subjected to oblique incident light, thereby limiting their imaging field of view. In light of this, our study presents the design and an experimental demonstration of a polarization-insensitive, large-field-of-view metalens that uses a silicon metasurface. The metalens is specifically tailored to the long-wavelength infrared region and possesses a numerical aperture of 0.81, which is capable of focusing light at incident angles up to ±80°. Moreover, we successfully build a meta-optics camera by integrating the large field-of-view metalens on top of an image sensor, thus enabling wide-angle thermal imaging of practical scenes. This research provides new, to the best of our knowledge, insights for designing and realizing large-field-of-view optical systems and holds promise for applications in night vision imaging and security monitoring.

5.
Mol Oral Microbiol ; 38(4): 309-320, 2023 08.
Artigo em Inglês | MEDLINE | ID: mdl-37216657

RESUMO

INTRODUCTION: MicroRNAs (miRNAs), a type of non-coding RNA, have been demonstrated to be essential posttranscriptional modulators in oral diseases and inflammatory responses. However, the specific role of miR-27a-5p in periodontitis requires further investigation. In this study, we used both cellular and animal models to determine how miR-27a-5p affects the pathogenesis of periodontitis and its associated biological functions. METHODS: Quantitative real-time polymerase chain reaction and western blotting were used to analyze the expression of cytokines, phosphatase and tensin homolog deleted on chromosome ten (PTEN), and miR-27a-5p transcription. Investigation of alveolar bone resorption and inflammation of the periodontium in ligature-induced periodontitis in mice was performed using micro-computed tomography (micro-CT), hematoxylin-eosin (HE) staining, and tartrate-resistant acid phosphatase (TRAP) staining. The binding of miR-27a-5p and PTEN was predicted using the TargetScan database and experimentally confirmed using dual luciferase reporter gene assays. RESULTS: The inflamed gingiva showed lower levels of miR-27a-5p. Macrophages from miR-27a-5p-/- mice produced much higher quantities of pro-inflammatory cytokines owing to the stimulation of Porphyromonas gingivalis lipopolysaccharide, and miR-27a-5p-/- mice with ligature-induced periodontitis also exhibited more severe alveolar bone resorption and damage to the periodontium. Target validation assays identified PTEN as a direct target of bona. Blocking PTEN expression partially reduced inflammation, both in vitro and in vivo. CONCLUSIONS: miR-27a-5p alleviated the inflammatory response in periodontitis by targeting PTEN.


Assuntos
Reabsorção Óssea , MicroRNAs , Periodontite , Camundongos , Animais , Tensinas/genética , Microtomografia por Raio-X , MicroRNAs/genética , MicroRNAs/metabolismo , Inflamação , PTEN Fosfo-Hidrolase/genética , PTEN Fosfo-Hidrolase/metabolismo , Citocinas/genética , Periodontite/genética , Cromossomos/metabolismo , Reabsorção Óssea/genética
6.
Nano Lett ; 23(7): 2991-2997, 2023 Apr 12.
Artigo em Inglês | MEDLINE | ID: mdl-36971648

RESUMO

Spiral phase contrast imaging and bright-field imaging are two widely used modes in microscopy, providing distinct morphological information about objects. However, conventional microscopes are always unable to operate with these two modes at the same time and need additional optical elements to switch between them. Here, we present a microscopy setup that incorporates a dielectric metasurface capable of achieving spiral phase contrast imaging and bright-field imaging synchronously. The metasurface not only can focus the light for diffraction-limited imaging but also can perform a two-dimensional spatial differentiation operation by imparting an orbital angular momentum to the incident light field. This allows two spatially separated images to be simultaneously obtained, one containing high-frequency edge information and the other showing the entirety of the object. Combined with the advantages of planar architecture and ultrathin thickness of the metasurface, this approach is expected to provide support in the fields of microscopy, biomedicine, and materials science.

7.
Natl Sci Rev ; 10(1): nwac120, 2023 Jan.
Artigo em Inglês | MEDLINE | ID: mdl-36825119

RESUMO

Display and power supply have been two essential and independent cornerstones of modern electronics. Here, we report a lithium-plasmon-based low-powered dynamic color display with intrinsic dual functionality (plasmonic display and energy recycling unit) which is a result of the electric-field-driven transformation of nanostructured lithium metals. Dynamic color displays are enabled by plasmonic transformation through electrodeposition (electrostripping) of lithium metals during the charging (discharging) process, while the consumed energy for coloring can be retrieved in the inverse process respectively. Energy recycling of lithium metals brings energy consumption down to 0.390 mW cm-2 (0.105 mW cm-2) for the active (static) coloration state of a proof-of-concept display/battery device, which approaches nearly-zero-energy-consumption in the near-100%-energy-efficiency limit of commercial lithium batteries. Combining the subwavelength feature of plasmonics with effective energy recycling, the lithium-plasmon-based dynamic display offers a promising route towards next-generation integrated photonic devices, with the intriguing advantages of low energy consumption, a small footprint and high resolution.

8.
Nano Lett ; 23(6): 2436-2441, 2023 Mar 22.
Artigo em Inglês | MEDLINE | ID: mdl-36723626

RESUMO

The electron vortex beam (EVB)-carrying quantized orbital angular momentum (OAM) plays an essential role in a series of fundamental research. However, the radius of the transverse intensity profile of a doughnut-shaped EVB strongly depends on the topological charge of the OAM, impeding its wide applications in electron microscopy. Inspired by the perfect vortex in optics, herein, we demonstrate a perfect electron vortex beam (PEVB), which completely unlocks the constraint between the beam size and the beam's OAM. We design nanoscale holograms to generate PEVBs carrying different quanta of OAM but exhibiting almost the same beam size. Furthermore, we show that the beam size of the PEVB can be readily controlled by only modifying the design parameters of the hologram. The generation of PEVB with a customized beam size independent of the OAM can promote various in situ applications of free electrons carrying OAM in electron microscopy.

9.
Nat Nanotechnol ; 18(1): 71-78, 2023 Jan.
Artigo em Inglês | MEDLINE | ID: mdl-36471110

RESUMO

The growing interest to develop modern digital displays and colour printing has driven the advancement of colouration technologies with remarkable speed. In particular, metasurface-based structural colouration shows a remarkable high colour saturation, wide gamut palette, chiaroscuro presentation and polarization tunability. However, previous approaches cannot simultaneously achieve all these features. Here, we design and experimentally demonstrate a surface-relief plasmonic metasurface consisting of shallow nanoapertures that enable the independent manipulation of colour hue, saturation and brightness by individually varying the geometric dimensions and orientation of the nanoapertures. We fabricate microscale artworks using a reusable template-stripping technique that features photorealistic and stereoscopic impressions. In addition, through the meticulous arrangement of differently oriented nanoapertures, kaleidoscopic information states can be decrypted by particular combinations of incident and reflected polarized light.

10.
Sci Adv ; 8(43): eabq8314, 2022 Oct 28.
Artigo em Inglês | MEDLINE | ID: mdl-36288319

RESUMO

The ability to control the instantaneous state of light, from high-energy pulses down to the single-photon level, is an indispensable requirement in photonics. This has, for example, facilitated spatiotemporal probing and coherent control of ultrafast light-matter interactions, and enabled capabilities such as generation of exotic states of light with complexity, or at wavelengths, that are not easily accessible. Here, by leveraging the multifunctional control of light at the nanoscale offered by metasurfaces embedded in a Fourier transform setup, we present a versatile approach to synthesize ultrafast optical transients with arbitrary control over its complete spatiotemporal evolution. Our approach, supporting an ultrawide bandwidth with simultaneously high spectral and spatial resolution, enables ready synthesis of complex states of structured space-time wave packets. We expect our results to offer unique capabilities in coherent ultrafast light-matter interactions and facilitate applications in microscopy, communications, and nonlinear optics.

11.
Nano Lett ; 22(16): 6655-6663, 2022 Aug 24.
Artigo em Inglês | MEDLINE | ID: mdl-35925801

RESUMO

The miniaturization and integration of optoelectronic devices require progressive size reduction of active layers, resulting in less optical absorption and lower quantum efficiency. In this work, we demonstrate that introducing a metasurface made of hybrid organic-inorganic perovskite (HOIP) can significantly enhance broadband absorption and improve photon-to-electron conversion, which roots from exciting Mie resonances together with suppressing optical transmission. On the basis of the HOIP metasurface, a broadband photodetector has been fabricated where photocurrent boosts more than 10 times in the frequency ranging from ultraviolet to visible. The device response time is less than 5.1 µs at wavelengths 380, 532, and 710 nm, and the relevant 3 dB bandwidth is over 0.26 MHz. Moreover, this photodetector has been applied as a signal receiver for transmitting 2D color images in broadband optical communication. These results accentuate the practical applications of HOIP metasurfaces in novel optoelectronic devices for broadband optical communication.

12.
ACS Appl Mater Interfaces ; 14(8): 10805-10814, 2022 Mar 02.
Artigo em Inglês | MEDLINE | ID: mdl-35175726

RESUMO

With the development of high-performance supercapacitors, a conductive polymer (CP)-based pseudocapacitance electrode with good electrical conductivity and low processing costs holds a promising application prospect. As the core component of supercapacitors, the CP electrode with adjustable spacing, a high specific surface area, and a faster ion diffusion path has been extensively investigated. Herein, based on accurate top-down photolithography and electropolymerization approaches, we fabricate a CP-coated vertically aligned micropillar array (MPA) electrode. The electrode presents an overwhelming enhanced areal specific capacitance compared with that of a flat configuration, which is partially ascribed to an increased electroactive surface area, two rapid channels for ion diffusion and electron transfer, and enhanced electric field intensity that is provided by the MPA structure. Based on the fabricated CP-based MPA electrode, an asymmetric supercapacitor is assembled with two thiophene derivatives, presenting a high energy density and excellent cycling stability. A supercapacitor system cascading with three asymmetric supercapacitor devices further demonstrates the practical applications by driving the light-emitting diodes. This work provides a good reference for the further development of CP-based energy storage devices with high energy density and superior cycling stability.

13.
Light Sci Appl ; 10(1): 107, 2021 May 25.
Artigo em Inglês | MEDLINE | ID: mdl-34035215

RESUMO

Monochromatic light can be characterized by its three fundamental properties: amplitude, phase, and polarization. In this work, we propose a versatile, transmission-mode all-dielectric metasurface platform that can independently manipulate the phase and amplitude for two orthogonal states of polarization in the visible frequency range. For proof-of-concept experimental demonstration, various single-layer metasurfaces composed of subwavelength-spaced titanium-dioxide nanopillars are designed, fabricated, and characterized to exhibit the ability of polarization-switchable multidimensional light-field manipulation, including polarization-switchable grayscale nanoprinting, nonuniform cylindrical lensing, and complex-amplitude holography. We envision the metasurface platform demonstrated here to open new possibilities toward creating compact multifunctional optical devices for applications in polarization optics, information encoding, optical data storage, and security.

14.
Nat Commun ; 12(1): 2230, 2021 Apr 13.
Artigo em Inglês | MEDLINE | ID: mdl-33850114

RESUMO

The term Poincaré beam, which describes the space-variant polarization of a light beam carrying spin angular momentum (SAM) and orbital angular momentum (OAM), plays an important role in various optical applications. Since the radius of a Poincaré beam conventionally depends on the topological charge number, it is difficult to generate a stable and high-quality Poincaré beam by two optical vortices with different topological charge numbers, as the Poincaré beam formed in this way collapses upon propagation. Here, based on an all-dielectric metasurface platform, we experimentally demonstrate broadband generation of a generalized perfect Poincaré beam (PPB), whose radius is independent of the topological charge number. By utilizing a phase-only modulation approach, a single-layer spin-multiplexed metasurface is shown to achieve all the states of PPBs on the hybrid-order Poincaré Sphere for visible light. Furthermore, as a proof-of-concept demonstration, a metasurface encoding multidimensional SAM and OAM states in the parallel channels of elliptical and circular PPBs is implemented for optical information encryption. We envision that this work will provide a compact and efficient platform for generation of PPBs for visible light, and may promote their applications in optical communications, information encryption, optical data storage and quantum information sciences.

15.
Materials (Basel) ; 13(18)2020 Sep 08.
Artigo em Inglês | MEDLINE | ID: mdl-32911692

RESUMO

AlSi10Mg alloy branches were fabricated by selective laser melting (SLM), and the branches were employed to evaluate their effect on the mechanical properties. When the porous branches were compressed along its building direction, the tree column structures-type AlSi10Mg alloy branches collapsed twice, which had typical elastic, shear, collapse, and densification stages. The compressive stress concentration at the interface between the support and the porous body caused the fracture of the tree column structures-type AlSi10Mg alloy branches. The fracture surface indicated that the prepared tree-type branches were distributed with different shapes of dimples, and the Si content inside the dimples was higher than that of the edge. The morphology of the Al-Si eutectic structure formed by SLM and the stress concentration at the Al/Al-Si-eutectic interface affected the fracture morphology and Si content distribution.

16.
Nano Lett ; 20(4): 2791-2798, 2020 04 08.
Artigo em Inglês | MEDLINE | ID: mdl-32155076

RESUMO

As the two most representative operation modes in an optical imaging system, bright-field imaging and phase contrast imaging can extract different morphological information on an object. Developing a miniature and low-cost system capable of switching between these two imaging modes is thus very attractive for a number of applications, such as biomedical imaging. Here, we propose and demonstrate that a Fourier transform setup incorporating an all-dielectric metasurface can perform a two-dimensional spatial differentiation operation and thus achieve isotropic edge detection. In addition, the metasurface can provide two spin-dependent, uncorrelated phase profiles across the entire visible spectrum. Therefore, based on the spin-state of incident light, the system can be used for either diffraction-limited bright-field imaging or isotropic edge-enhanced phase contrast imaging. Combined with the advantages of planar architecture and ultrathin thickness of the metasurface, we envision this approach may open new vistas in the very interdisciplinary field of imaging and microscopy.


Assuntos
Microscopia de Contraste de Fase/instrumentação , Desenho de Equipamento , Análise de Fourier , Luz , Imagem Óptica/instrumentação , Fótons
17.
Optica ; 7(9)2020.
Artigo em Inglês | MEDLINE | ID: mdl-33655018

RESUMO

We realize a dielectric metasurface that enables full-color generation and ultrasmooth brightness variation. The reproduced artwork "Girl with a Pearl Earring" features photorealistic color representation and stereoscopic image impression, mimicking the texture of an oil-painting.

18.
Laser Photon Rev ; 14(9)2020.
Artigo em Inglês | MEDLINE | ID: mdl-33569085

RESUMO

Light beams carrying spin angular momentum (SAM) and orbital angular momentum (OAM) have created novel opportunities in the areas of optical communications, imaging, micromanipulation and quantum optics. However, complex optical setups are required to simultaneously manipulate, measure and analyze these states, which significantly limits system integration. Here, we introduce a novel detection approach for measuring multiple SAM and OAM modes simultaneously through a planar nanophotonic demultiplexer based on an all-dielectric metasurface. Coaxial light beams carrying multiple SAM and OAM states of light upon transmission through the demultiplexer are spatially separated into a range of vortex beams with different topological charge, each propagating along a specific wavevector. The broadband response, material dispersion and momentum conservation further enable the demultiplexer to achieve wavelength demultiplexing. We envision the ultracompact multifunctional architecture to enable simultaneous manipulation and measurement of polarization and spin encoded photon states with applications in integrated quantum optics and optical communications.

19.
Adv Mater ; 32(27): e1903787, 2020 Jul.
Artigo em Inglês | MEDLINE | ID: mdl-31566259

RESUMO

Recent advances in nanofabrication technologies have spurred many breakthroughs in the field of photonic metamaterials that provide efficient ways of manipulating light-matter interaction at subwavelength scales. As one of the most important applications, photonic metamaterials can be used to implement novel optical absorbers. First the morphology engineering of various photonic metamaterial absorbers is discussed, which is highly associated with impendence matching conditions and resonance modes of the absorbers, thus directly determines their absorption efficiency, operational bandwidth, incident angle, and polarization dependence. Then, the recent achievements of various interdisciplinary applications based on photonic metamaterial absorbers, including structural color generation, ultrasensitive optical sensing, solar steam generation, and highly responsive photodetection, are reviewed. This report is expected to provide an overview and vision for the future development of photonic metamaterial absorbers and their applications in novel nanophotonic systems.

20.
Nanoscale ; 11(22): 10646-10654, 2019 Jun 06.
Artigo em Inglês | MEDLINE | ID: mdl-31107482

RESUMO

Optical polarization topology is a spatially varying polarization structure, which usually exists around the polarization singularity. In three-dimensional (3D) space, optical polarization topologies mainly contain two fundamental structures, Möbius strip and twisted ribbon, depending on the parity of half-twist number. These spectacular topologies have been widely found in the existence of electric fields from multi-beam interference. Here, we propose and numerically demonstrate that, depending on the photonic spin state of light, an ultrathin all-dielectric metasurface can achieve efficient generation and transformation of two arbitrary 3D polarization topologies. The spin-controlled, tightly-focused Poincaré beams generated by the metasurface exhibit topologically stable 3D polarization topologies around the waist of the focal point. The preparation of such optical polarization topologies may have potential applications in compact complex beam engineering, optical signal multiplexing and optical fabrication of microstructures with nontrivial topology.

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