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1.
Small ; : e2309780, 2024 Mar 03.
Artigo em Inglês | MEDLINE | ID: mdl-38433392

RESUMO

The conventional sea water desalination technologies are not yet adopted worldwide, especially in the third world countries due to their high capital cost as well as large energy requirement. To solve this issue in a sustainable way an interfacial solar water evaporation device is designed and proposed in this article using the branches of Prunus serrulata (PB). The PB has abundant microchannels and shows excellent photothermal conversion capability after carbonization. Moreover, the easy access to raw materials and the facile fabrication process makes the solar water evaporating device very cost effective for seawater desalination application. Experiments show that in the presence of the fabricated evaporator the evaporation rate of water can reach 3.5 kg m-2  h-1 under 1 sun, which is superior to many similar experimental devices. In addition, its advantages, such as effective sewage purification capability, low cost, and environmental friendliness, make this evaporator highly competitive in the extensive promotion of this technology and can be considered as a new sustainable solution for seawater desalination with great application potential and prospects.

2.
Small Methods ; 8(2): e2300239, 2024 Feb.
Artigo em Inglês | MEDLINE | ID: mdl-37356086

RESUMO

2D semi-metallic hafnium ditelluride material is used in several applications such as solar steam generation, gas sensing, and catalysis owing to its strong near-infrared absorbance, high sensitivity, and distinctive electronic structure. The zero-bandgap characteristics, along with the thermal and dynamic stability of 2D-HfTe2, make it a desirable choice for developing long-wavelength-range photonics devices. Herein, the HfTe2 -nanosheets are prepared using the liquid-phase exfoliation method, and their superior nonlinear optical properties are demonstrated by the obtained modulation depth of 11.9% (800 nm) and 6.35% (1560 nm), respectively. In addition, the observed transition from saturable to reverse saturable absorption indicates adaptability of the prepared material in nonlinear optics. By utilizing a side polished fiber-based HfTe2 -saturable absorber (SA) inside an Er-doped fiber laser cavity, a mode-locked laser with 724 fs pulse width and 56.63 dB signal-to-noise ratio (SNR) is realized for the first time. The generated laser with this SA has the second lowest mode-locking pump threshold (18.35 mW), among the other 2D material based-SAs, thus paving the way for future laser development with improved efficiency and reduced thermal impact. Finally, employing this HfTe2 -SA, a highly stable single-frequency fiber laser (SNR ≈ 74.56 dB; linewidth ≈ 1.268 kHz) is generated for the first time, indicating its promising ultranarrow photonic application.

3.
Langmuir ; 38(43): 13187-13194, 2022 11 01.
Artigo em Inglês | MEDLINE | ID: mdl-36255348

RESUMO

Interfacial solar steam generation (ISSG) is considered as an excellent seawater desalination technology because of its electricity-independent nature, low cost, and portability. However, improving the water evaporation efficiency, simplifying the fabrication process, and reducing the overall cost of the evaporator are still challenging. Here, an efficient and sustainable solar water evaporator is fabricated with carbonized ginkgo biloba leaves as the structural basis of photothermal materials. The combination of the abundant capillary channels in ginkgo leaves paired with polyacrylamide (PAM) hydrogel accelerates water transportation and solar-driven evaporation. The fabricated evaporator shows excellent photothermal conversion capability and evaporates water at 2.39 kg m-2 h-1 under 1 sun irradiation. In addition, the device exhibits remarkable stability in simulated seawater and can effectively realize seawater desalination or sewage treatment. As a result, the system is promising for future highly efficient solar evaporation due to its environmental protection and low cost.


Assuntos
Energia Solar , Purificação da Água , Água , Luz Solar , Vapor
4.
ACS Appl Mater Interfaces ; 14(6): 7936-7948, 2022 Feb 16.
Artigo em Inglês | MEDLINE | ID: mdl-35119819

RESUMO

With the advancement of civilization, water purification, as well as management and disposal of ever-increasing municipal solid waste (MSW), and e-waste, have become global concerns. To address these issues in a sustainable way, a 3D solar evaporator has been proposed in this paper by repurposing recycled paper from MSW in the form of egg trays and waste dry toner (e-waste) using a facile fabrication method. The unique 3D porous structure, fibrous surface, superior water absorbing capability as well as low thermal conductivity of wastepaper-derived egg trays make them an excellent candidate for an efficient solar evaporator, while the waste toner powder coating significantly enhances the optical absorbance capacity. Under 1 sun illumination, the proposed solar evaporator demonstrates an excellent evaporation rate and efficiency of 1.3 kg/m2 h and 78.5%, respectively. Moreover, the competitive advantage of the 3D structure in collecting solar irradiance at various light incident angles in comparison to a 2D structure, excellent cycle stability, low processing temperature, and the use of low-cost waste materials enable its use for large-scale water purification systems.

5.
ACS Appl Mater Interfaces ; 13(51): 61518-61527, 2021 Dec 29.
Artigo em Inglês | MEDLINE | ID: mdl-34793123

RESUMO

Two-dimensional (2D) gallium sulfide (GaS) offers a plethora of exceptional electrical and optical properties, allowing it to be used in a wide range of applications, including photodetectors, hydrogen generation, and nonlinear optical devices. In this paper, ultrathin 2D GaS nanosheets are synthesized using the liquid-phase exfoliation method, and the structure, morphology, and chemical composition of the as-prepared nanosheets are extensively investigated. After depositing 2D GaS nanosheets on side polished fibers, successful saturable absorbers (SAs) are fabricated for the first time. The realized modulation depths are 10 and 5.3% at 1 and 1.5 µm, respectively, indicating the wideband saturable absorption performance of the prepared SAs. By integrating GaS-SAs into three different wavelength-based fiber laser cavities, stable mode-locked pulses are achieved, having pulse durations of 46.22 ps (1 µm), 614 fs (1.5 µm), and 1.02 ps (2 µm), respectively. Additionally, different orders of harmonic mode-locked pulses with the highest repetition rate of 0.55 GHz (45th order) and Q-switched pulses with the shortest pulse duration of 2.2 µs are obtained in the telecommunication waveband. These findings suggest that 2D GaS has a lot of potential for broadband ultrafast photonics in nonlinear photonics devices.

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