Wavelength scaling of terahertz pulse energies delivered by two-color air plasmas.

We address the long-standing problem of anomalous growth observed in the terahertz (THz) energy yield from air plasmas created by two-color laser pulses, as the fundamental wavelength λ0 is increased. Using two distinct optical parametric amplifiers (OPAs), we report THz energies scaling like λ0α with large exponents 5.6≤α≤14.3, which departs from the growth in λ02 expected from photocurrent theory. By means of comprehensive 3D simulations, we demonstrate that the changes in the laser beam size, pulse duration, and phase-matching conditions in the second-harmonic generation process when tuning the OPA's carrier wavelength can lead to these high scaling powers. The value of the phase angle between the two colors reached at the exit of the doubling crystal turns out to be crucial and even explains non-monotonic behaviors in the measurements.

Ultrabroadband terahertz spectroscopy of a liquid crystal.

Liquid crystals (LCs) are becoming increasingly important for applications in the terahertz frequency range. A detailed understanding of the spectroscopic parameters of these materials over a broad frequency range is crucial in order to design customized LC mixtures for improved performance. We present the frequency dependent index of refraction and the absorption coefficients of the nematic liquid crystal 5CB over a frequency range from 0.3 THz to 15 THz using a dispersion-free THz time-domain spectrometer system based on two-color plasma generation and air biased coherent detection (ABCD). We show that the spectra are dominated by multiple strong spectral features mainly at frequencies above 4 THz, originating from intramolecular vibrational modes of the weakly LC molecules.

Optical waveguide mode control by nanoslit-enhanced terahertz field.

In this Letter we propose a scheme providing control over an optical waveguide mode by a terahertz (THz) wave. The scheme is based on an optimization of the overlap between the optical waveguide mode and the THz field, with the THz field strength enhanced by the presence of a metallic nanoslit surrounding the waveguide. We find an optimum balance between the optical mode attenuation and Kerr-induced change in the propagation constant. The criterion for a π/2-cumulative phase shift, for instance for application in a Mach-Zehnder interferometer configuration, requires 10 kV/cm THz field, which in turn is estimated to result in a nonlinear change of the refractive index in the waveguide of 0.001. Our simulations prove that it is quite reasonable to observe the effect experimentally.

Terahertz field enhancement to the MV/cm regime in a tapered parallel plate waveguide.

We investigate field enhancement properties of a tapered parallel plate waveguide for ultrashort terahertz (THz) pulses. We use two independent methods, air biased coherent detection inside the waveguide and free-space electro-optic sampling, respectively, which enables a calibrated, quantitative measurement of the field strength at the output of the waveguide. Field enhancement factors greater than 20 are demonstrated and record-high field strengths of > 1.4 MV/cm are reached. We find an excellent agreement between the two independent methods of field measurement and a numerical 3D full-vectorial time-domain simulations.

Direct observation of sub-100 fs mobile charge generation in a polymer-fullerene film.

The formation of mobile charges in a roll-to-roll processed poly-3-hexylthiophene-fullerene bulk heterojunction film is observed directly by using transient terahertz spectroscopy with sub-100 fs temporal resolution. The transient terahertz ac conductivity reveals that 20% of the incident pump photons are converted into highly delocalized charges within the 40 fs, 3.1 eV pump pulse duration, which then rapidly becomes localized within 120 fs. Approximately 2/3 of these carriers subsequently decay, possibly into an exciton, on a 1 ps time scale.

Terahertz pulse propagation in the near field and the far field.

We present a detailed investigation of the propagation properties of beams of ultrashort terahertz (THz) pulses emitted from large-aperture (LA) antennas. The large area of the emitter is demonstrated to have substantial influence on the temporal pulse profile in both the near field and the far field. We perform a numerical analysis based on scalar and vectorial broadband diffraction theory and are able to distinguish between near-field and far-field contributions to the total THz signal. We find that the THz beam from a LA antenna propagates like a Gaussian beam and that the temporal profile of the THz pulse, measured in the near field, contains information about the temporal and spatial field distribution on the emitter surface, which is intrinsically connected to the carrier dynamics of the antenna substrate. As a result of pulse reshaping, focusing of the THz beam leads to a reduced relative pulse momentum, with implications in THz field-ionization experiments.

Photoexcited GaAs surfaces studied by transient terahertz time-domain spectroscopy.

The transmission characteristics of an air-GaAs interface and the transient absorption and index spectra of the thin, photoexcited surface layer are investigated subsequent to excitation by a femtosecond laser pulse. We find that the total phase change and transmission of a terahertz (THz) probe pulse are dominated by interface effects. This observation has important implications in the interpretation of THz time-domain spectroscopy data of absorbing media. We also observe that the THz pulse apparently arrives at the detector as much as 60 fs earlier when it is transmitted through an optically excited GaAs wafer. This effect is fully explained in terms of a frequency-dependent transmission and phase shift at the air-GaAs interface and is not associated with superluminal propagation.

Radiation patterns from lens-coupled terahertz antennas.

We report on investigations of the angular distribution of the radiation emitted from a terahertz antenna system equipped with a truncated spherical silicon lens. The pattern is calculated by wide-angle interference principles and Huygens-Fresnel diffraction theory. Experimental determination of the radiation pattern is performed by spatially resolved terahertz time-domain spectroscopy. Good agreement between theory and experiment is obtained, and we find that the terahertz beam can be represented by a Gaussian beam emitted from a circular aperture equal to the diameter of the lens.