Reversible optical tuning of GeSbTe phase-change metasurface spectral filters for mid-wave infrared imaging.

Tunable narrowband spectral filtering across arbitrary optical wavebands is highly desirable in a plethora of applications, from chemical sensing and hyperspectral imaging to infrared astronomy. Yet, the ability to reconfigure the optical properties, with full reversibility, of a solid-state large-area narrowband filter remains elusive. Existing solutions require either moving parts, have slow response times, or provide limited spectral coverage. Here, we demonstrate a 1-inch diameter continuously tunable, fully reversible, all-solid-state, narrowband phase-change metasurface filter based on a GeSbTe-225 (GST)-embedded plasmonic nanohole array. The passband of the presented device is ∼ 74 n m with ∼ 70 % transmittance and operates across the 3-5 µm thermal imaging waveband. Continuous, reconfigurable tuning is achieved by exploiting intermediate GST phases via optical switching with a single nanosecond laser pulse, and material stability is verified through multiple switching cycles. We further demonstrate multispectral thermal imaging in the mid-wave infrared using our active phase-change metasurfaces. Our results pave the way for highly functional, reduced power, compact hyperspectral imaging systems and customizable optical filters for real-world system integration.

High-efficiency flexible multilevel photon sieves by single-step laser-based fabrication and optical analysis.

Over the past several decades, the need for high-resolution, high-efficiency, lightweight, high-contrast focusing optics has continued to increase due to their applications in fields such as astronomy, spectroscopy, free-space optical communications, defense, and remote sensing. In recent years, photon sieve planar diffractive optics, which are essentially Fresnel zone plates with the rings broken into individual "pinhole" apertures, have been developed on flexible, lightweight polyimide substrates. However, transmission efficiencies have continuously been very low (∼1%-11%) until this work, thus impeding the widespread use of photon sieves in practical applications. Here, we present flexible, lightweight, four- and eight-level phase photon sieves with 25.7% and 49.7% transmission efficiency, respectively, up to five times greater than that of any other photon sieve reported thus far. Additionally, these sieves were fabricated via a single step pulsed laser ablation method. The total time to fabricate a ∼3 cm2 photon sieve via the single-step fabrication was tens of seconds, giving the technique a significant advantage over traditional photolithography used to generate multilevel structures. Analytical analysis of the photon sieve was carried out via the finite-difference time-domain (FDTD) method and was in very good agreement with experimental results. We have also calculated via FDTD modeling the behavior of higher-level photon sieves for further enhanced efficiencies, and analytically show an estimated upper bound on photon sieve efficiency of 70% within the first focal plane null in the limit of increasing step number, and the data presented herein provide a relationship between efficiency and step number. Additionally, this process of multilevel diffractive lens fabrication can be extended to multilevel Fresnel zone plates, which have not previously been demonstrated by this process. The results presented in this work represent a new step in high-resolution diffractive optics, showing efficiencies suitable for widespread applications in addition to drastically reducing the cost and complexity of fabricating multilevel focusing elements.

Flexible binary phase photon sieves on polyimide substrates by laser ablation.

A binary phase diffractive optical element photon sieve is fabricated by direct laser ablation of a thin, flexible polyimide substrate with a nanosecond-pulsed ultraviolet laser. The binary phase photon sieve operates at 633 nm and was designed with 19 rings and a focal length of 400 mm. The total time to fabricate the photon sieves was tens of seconds. The surface properties of the laser-processed areas are examined, and the optical performance of the photon sieve is characterized and compared to FDTD simulations. By optimizing the laser fluence and travel distance between laser pulses, features with sub-wavelength surface roughness were achieved. The photon sieve showed good focusing ability with suppressed side-lobes. When the fractional area of photon sieve pinholes was made to approach 50%, the binary sieve diffraction efficiency approached 11%, matching the highest value reported in the literature for a photon sieve. Thus, this Letter demonstrates both high efficiency and lightweight diffractive optics suitable for space satellite and other applications, with capabilities for low cost and high throughput fabrication.

Fabrication of photon sieves by laser ablation and optical properties.

In this work, we demonstrate the feasibility and performance of photon sieve diffractive optical elements fabricated via a direct laser ablation process. Pulses of 50 ns width and wavelength 1064 nm from an ytterbium fiber laser were focused to a spot diameter of approximately 35 µm. Using a galvanometric scan head writing at 100 mm/s, a 30.22 mm2 photon sieve operating at 633 nm wavelength with a focal length of 400 mm was fabricated. The optical performance of the sieve was characterized and is in strong agreement with numerical simulations, producing a focal spot size full-width at half-maximum (FWHM) of 45.12 ± 0.74 µm with a photon sieve minimum pinhole diameter of 62.2 µm. The total time to write the photon sieve pattern was 28 seconds as compared to many hours using photolithography methods. We also present, for the first time to our knowledge in the literature, thorough characterization of the influence of angle of incidence, temperature, and illumination wavelength on photon sieve performance. Thus, this work demonstrates the potential for a high speed, low cost fabrication method of photon sieves that is highly customizable and capable of producing sieves with low or high numerical apertures.