Measurement of nonlinear refractive indices of bulk and liquid crystals by nonlinear chirped interferometry.

The nonlinear refractive indices (n2) of a selection of bulk (LiB3O5, KTiOAsO4, MgO:LiNbO3, LiGaS2, ZnSe) and liquid (E7, MLC2132) crystals are measured at 1030 nm in the sub-picosecond regime (200 fs) by nonlinear chirped interferometry. The reported values provide key parameters for the design of near- to mid-infrared parametric sources, as well as all-optical delay lines.

Reconfigurable design of a thermo-optically addressed liquid-crystal phase modulator by a neural network.

We present a machine learning approach to program the light phase modulation function of an innovative thermo-optically addressed, liquid-crystal based, spatial light modulator (TOA-SLM). The designed neural network is trained with a little amount of experimental data and is enabled to efficiently generate prescribed low-order spatial phase distortions. These results demonstrate the potential of neural network-driven TOA-SLM technology for ultrabroadband and large aperture phase modulation, from adaptive optics to ultrafast pulse shaping.

Spectral coherence properties of continuum generation in bulk crystals.

The stability of the phase difference between two white-light continua, generated from the same 180-fs pulses at ≃1035 nm, is assessed by a modified Bellini-Hänsch interferometer. Mutual spectral phase stability is studied and quantified as a function of several parameters: pulse energy, position of the nonlinear crystal with respect to the beam waist and interaction length. Our results show that intrapulse decoherence may significantly contribute to the measured CEP noise floor. In addition, spectrally-resolved intensity-to-phase coupling coefficients are measured and stability regions are identified.

Femtosecond laser-induced damage threshold of nematic liquid crystals at 1030 nm.

The laser-induced damage threshold (LIDT) of nematic liquid crystals is investigated in the femtosecond regime at ≃1030nm. The thickness and breakdown of freely suspended thin films (≃100nm) of different mixtures (MLC2073, MLC2132, and E7) is monitored in real time by spectral-domain interferometry. The duration of laser pulses was varied from 180 fs to 1.8 ps for repetition rates ranging from single shot to 1 MHz. The dependence of the LIDT with pulse duration suggests a damage mechanism dominated by ionization mechanisms at low repetition rate and by linear absorption at high repetition rate. In the single-shot regime, LIDTs exceeding 1J/cm2 are found for the three investigated mixtures. The LIDT of polyvinyl alcohol is also investigated by the same method.

Biomimicry of iridescent, patterned insect cuticles: comparison of biological and synthetic, cholesteric microcells using hyperspectral imaging.

Biological systems inspire the design of multifunctional materials and devices. However, current synthetic replicas rarely capture the range of structural complexity observed in natural materials. Prior to the definition of a biomimetic design, a dual investigation with a common set of criteria for comparing the biological material and the replica is required. Here, we deal with this issue by addressing the non-trivial case of insect cuticles tessellated with polygonal microcells with iridescent colours due to the twisted cholesteric organization of chitin fibres. By using hyperspectral imaging within a common methodology, we compare, at several length scales, the textural, structural and spectral properties of the microcells found in the two-band cuticle of the scarab beetle Chrysina gloriosa with those of the polygonal texture formed in flat films of cholesteric liquid crystal oligomers. The hyperspectral imaging technique offers a unique opportunity to reveal the common features and differences in the spectral-spatial signatures of biological and synthetic samples at a 6-nm spectral resolution over 400 nm-1000 nm and a spatial resolution of 150 nm. The biomimetic design of chiral tessellations is relevant to the field of non-specular properties such as deflection and lensing in geometric phase planar optics.

Relativistic-intensity near-single-cycle light waveforms at kHz repetition rate.

The development of ultra-intense and ultra-short light sources is currently a subject of intense research driven by the discovery of novel phenomena in the realm of relativistic optics, such as the production of ultrafast energetic particle and radiation beams for applications. It has been a long-standing challenge to unite two hitherto distinct classes of light sources: those achieving relativistic intensity and those with pulse durations approaching a single light cycle. While the former class traditionally involves large-scale amplification chains, the latter class places high demand on the spatiotemporal control of the electromagnetic laser field. Here, we present a light source producing waveform-controlled 1.5-cycle pulses with a 719 nm central wavelength that can be focused to relativistic intensity at a 1 kHz repetition rate based on nonlinear post-compression in a long hollow-core fiber. The unique capabilities of this source allow us to observe the first experimental indications of light waveform effects in laser wakefield acceleration of relativistic energy electrons.

Dispersion of 20 fs pulses through band edges of cholesteric liquid crystals.

We demonstrate the ability to manipulate ultrashort pulses in cholesteric liquid crystals in the linear regime. We present an extensive analysis of the spectral changes undergone by 20fs pulses when propagating through band edges of cholesteric liquid crystals. The accurate quantification of the introduced optical dispersion opens the way to controlled stretching and compression of ultrashort pulses. The behaviors of cholesteric liquid crystal films with different thickness, bandgap and structural parameters (monotonic pitch versus pitch-gradient films) are compared. A statistical approach is disclosed to fidelize and deepen the set of experimental investigations.

Nanoscale hyperspectral imaging of tilted cholesteric liquid crystal structures.

Ongoing research on chiral liquid crystals takes advantage of the peculiar behavior of twisted structures subject to curvature. We demonstrate the fine tunability of the characteristics of the bandgap of a cholesteric structure in which the orientation of the helix axis spatially changes. To date, the spectral resolution of the order of 6 nm, herein reached by hyperspectral imaging, has not been solved in tilted helices. A correlation between spectral shifts and spatial twists is thus made possible.

Shear-enhanced diffraction from thin permanent gratings in dye-doped nematic liquid crystal cells.

Permanent gratings are recorded in planar-aligned dye-doped nematic liquid crystal cells under visible light illumination. By increasing the irradiation intensity and exposure time, several diffraction orders of the recorded gratings are obtained in the Raman-Nath diffraction regime. By applying a dynamic transverse shear on one of the confining plates of the cell, an enhancement of the diffraction efficiency is achieved, which follows the period of the grating. By microscope inspection under static displacement of the upper plate, surface gratings formed by the dye adsorption are revealed in both the front and rear windows of the cell, indicating that the diffraction amplification originates from a coherent superposition of the diffracted orders when the gratings are displaced half a period. The effect provides self-matched amplification of diffraction with a simple cell, a single photo-inscription stage, and elementary displacement steps.

Dynamical optical response of nematic liquid crystal cells through electrically driven Fréedericksz transition: influence of the nematic layer thickness.

A dynamical optical characterization of planar nematic liquid-crystal cells electrically driven through the Fréedericksz transition is presented. Our method involves applying voltage steps with different starting voltage close to the Fréedericksz threshold. Measurements are performed on cells with various thickness, from a few microns up to 180µm, and highlight the transient molecular disorder occurring close to the Fréedericksz transition. We show that the transient disorder affects the molecular arrangement mainly in the reorientational plane of the splay motion induced by the planar cell geometry. Moreover, a disorder quantification in terms of optical transmission losses and temporal dynamics enables us to picture the Fréedericksz transition. This characterization provides the identification of the electrical driving conditions for which the effect of the reorientational disorder is minimized. When comparing cells with various thicknesses, it results that thick cells are characterized by a much smoother transition with respect to the conventional step-like Fréedericksz transition of the thin cells, hence, thick cells can be dynamically driven over a large range of voltages, even below the Fréedericksz threshold. The results are discussed in view of novel electro-optical applications of thick layers of nematics. As an example, the experimental conditions for realizing a rapid birefringence scan and the achievement of a large and tunable group delay for femtosecond pulses are presented.

Tunable angular shearing interferometer based on wedged liquid crystal cells.

The concept of a liquid crystal wedge as a tunable angular shearing interferometer is introduced and demonstrated to combine both high stability and high tunability. Different wedges are fabricated from planar aligned nematic liquid crystal cells with thickness gradients. These wedges are shown to produce stable interferograms from the polarization interference between the ordinary and extraordinary waves propagating in different directions at the output of the cell. The fringe periods, ranging from 70 µm to 1.25 mm, can be precisely controlled by a low voltage. Despite the wedge-shaped structure, no inhomogeneity has been detected when the wedge is driven adiabatically and the interferograms are uniform over regions as large as 5×5 mm. Moreover, dynamical measurements show that the wedges behave as a succession of multiple cells with different thickness, giving rise to a moving front of stabilizing fringes when driven dynamically. All the observations show that the device is suitable for large beam size and tunable shearing interferometry, with attractive features for applications such as phase sensing, photoalignment or photolithography.

Continuously tunable femtosecond delay-line based on liquid crystal cells.

We introduce a new device for group and phase delay steering of femtosecond pulse trains that makes use of cascaded, electrically driven, nematic liquid-crystal cells. Based on this approach we demonstrate a continuously tunable optical delay line. The simple collinear implementation with no moving parts enables to shape the achievable temporal range with sub-femtosecond accuracy. By appropriately choosing the bias voltages applied to the cascaded cells, the imparted group delay can be made either positive or negative and precisely adjusted. Moreover, independent control of the group delay and the phase of femtosecond pulses is demonstrated.

Anticorrelated Emission of High Harmonics and Fast Electron Beams From Plasma Mirrors.

We report for the first time on the anticorrelated emission of high-order harmonics and energetic electron beams from a solid-density plasma with a sharp vacuum interface-plasma mirror-driven by an intense ultrashort laser pulse. We highlight the key role played by the nanoscale structure of the plasma surface during the interaction by measuring the spatial and spectral properties of harmonics and electron beams emitted by a plasma mirror. We show that the nanoscale behavior of the plasma mirror can be controlled by tuning the scale length of the electron density gradient, which is measured in situ using spatial-domain interferometry.

Spatial-domain interferometer for measuring plasma mirror expansion.

We present a practical spatial-domain interferometer for characterizing the electronic density gradient of laser-induced plasma mirrors with sub-30-femtosecond temporal resolution. Time-resolved spatial imaging of an intensity-shaped pulse reflecting off an expanding plasma mirror induced by a time-delayed pre-pulse allows us to measure characteristic plasma gradients of 10-100 nm with an expansion velocity of 10.8 nm/ps. Spatial-domain interferometry (SDI) can be generalized to the ultrafast imaging of nm to µm size laser-induced phenomena at surfaces.

Passive coherent combining of CEP-stable few-cycle pulses from a temporally divided hollow fiber compressor.

We demonstrate a simple and robust passive coherent combining technique for temporal compression of millijoule energy laser pulses down to few-cycle duration in a gas-filled hollow fiber. High combining efficiency is achieved by using carefully oriented calcite plates for temporal pulse division and recombination. Carrier-envelope phase (CEP)-stable, 6-fs, 800-nm pulses with more than 0.6 mJ energy are routinely generated. This method could aid in the energy scaling of CEP-stable hollow-fiber compressor systems.

Carrier-envelope-phase stable, high-contrast, double chirped-pulse-amplification laser system.

We present the first carrier-envelope-phase stable chirped-pulse amplifier (CPA) featuring high temporal contrast for relativistic intensity laser-plasma interactions at 1 kHz repetition rate. The laser is based on a double-CPA architecture including cross-polarized wave (XPW) filtering technique and a high-energy grism-based compressor. The 8 mJ, 22 fs pulses feature 10⁻¹¹ temporal contrast at -20 ps and a carrier-envelope-phase drift of 240 mrad root mean square.

Carrier-envelope phase stability of hollow fibers used for high-energy few-cycle pulse generation.

We investigated the carrier-envelope phase (CEP) stability of hollow-fiber compression for high-energy few-cycle pulse generation. Saturation of the output pulse energy is observed at 0.6 mJ for a 260 µm inner-diameter, 1 m long fiber, statically filled with neon. The pressure is adjusted to achieve output spectra supporting sub-4-fs pulses. The maximum output pulse energy can be increased to 0.8 mJ by either differential pumping (DP) or circularly polarized input pulses. We observe the onset of an ionization-induced CEP instability, which saturates beyond input pulse energies of 1.25 mJ. There is no significant difference in the CEP stability with DP compared to static-fill.

Energy-scalable temporal cleaning device for femtosecond laser pulses based on cross-polarized wave generation.

We report on a compact energy-scalable device for generating high-fidelity femtosecond laser pulses based on spatial filtering through a hollow-core fiber followed by a nonlinear crystal for cross-polarized wave (XPW) generation. This versatile device is suited for temporal pulse cleaning over a wide range of input energies (from 0.1 to >10 mJ) and is successfully qualified on different ultrafast laser systems. Full characterization of the XPW output is presented. In particular, we demonstrate the generation of 1.6 mJ energy pulses starting from 11 mJ input pulse energy. The temporal contrast of the pulses is enhanced by more than 4 orders of magnitude. In addition, pulse shortening from 40 fs down to 15 fs Fourier-transform limit yields an overall peak-power transmission of up to 50%. This device not only serves as an integrated pulse contrast filter inside an ultrafast laser amplifier but also as a simple back-end solution for temporal post-compression of amplified pulses.

Generation of high-fidelity few-cycle pulses at 2.1 µm via cross-polarized wave generation.

We demonstrate the generation of temporally clean few-cycle pulses at 2.1 µm by shortening of 6-optical-cycle pulses via cross-polarized wave (XPW) generation in BaF(2), CaF(2) and CVD-Diamond crystals. By combining spectra and single-shot third-order intensity cross-correlation traces in a novel Bayesian pulse retrieval technique, we measured pulse durations of 20 fs, corresponding to 2.8 optical cycles. Our results show that XPW generation in the infrared could provide a high-fidelity source of few-cycle pulses for strong-field physics applications. It could also serve as an injector for high-peak power ultrafast mid-IR wavelength parametric amplifiers.

Carrier-envelope phase stabilization and control using a transmission grating compressor and an AOPDF.

Carrier-envelope phase (CEP) stabilization of a femtosecond chirped-pulse amplification system featuring a compact transmission grating compressor is demonstrated. The system includes two amplification stages and routinely generates phase-stable (approximately 250 mrad rms) 2 mJ, 25 fs pulses at 1 kHz. Minimizing the optical pathway in the compressor enables phase stabilization without feedback control of the grating separation or beam pointing. We also demonstrate for the first time to the best of our knowledge, out-of-loop control of the CEP using an acousto-optic programmable dispersive filter inside the laser chain.