Extreme magnetoresistance at high-mobility oxide heterointerfaces with dynamic defect tunability.

Magnetic field-induced changes in the electrical resistance of materials reveal insights into the fundamental properties governing their electronic and magnetic behavior. Various classes of magnetoresistance have been realized, including giant, colossal, and extraordinary magnetoresistance, each with distinct physical origins. In recent years, extreme magnetoresistance (XMR) has been observed in topological and non-topological materials displaying a non-saturating magnetoresistance reaching 103-108% in magnetic fields up to 60 T. XMR is often intimately linked to a gapless band structure with steep bands and charge compensation. Here, we show that a linear XMR of 80,000% at 15 T and 2 K emerges at the high-mobility interface between the large band-gap oxides γ-Al2O3 and SrTiO3. Despite the chemically and electronically very dissimilar environment, the temperature/field phase diagrams of γ-Al2O3/SrTiO3 bear a striking resemblance to XMR semimetals. By comparing magnetotransport, microscopic current imaging, and momentum-resolved band structures, we conclude that the XMR in γ-Al2O3/SrTiO3 is not strongly linked to the band structure, but arises from weak disorder enforcing a squeezed guiding center motion of electrons. We also present a dynamic XMR self-enhancement through an autonomous redistribution of quasi-mobile oxygen vacancies. Our findings shed new light on XMR and introduce tunability using dynamic defect engineering.

Nanopatterning of oxide 2-dimensional electron systems using low-temperature ion milling.

We present a 'top-down' patterning technique based on ion milling performed at low-temperature, for the realization of oxide two-dimensional electron system devices with dimensions down to 160 nm. Using electrical transport and scanning Superconducting QUantum Interference Device measurements we demonstrate that the low-temperature ion milling process does not damage the 2DES properties nor creates oxygen vacancies-related conducting paths in the STO substrate. As opposed to other procedures used to realize oxide 2DES devices, the one we propose gives lateral access to the 2DES along the in-plane directions, finally opening the way to coupling with other materials, including superconductors.

Unveiling unconventional magnetism at the surface of Sr2RuO4.

Materials with strongly correlated electrons often exhibit interesting physical properties. An example of these materials is the layered oxide perovskite Sr2RuO4, which has been intensively investigated due to its unusual properties. Whilst the debate on the symmetry of the superconducting state in Sr2RuO4 is still ongoing, a deeper understanding of the Sr2RuO4 normal state appears crucial as this is the background in which electron pairing occurs. Here, by using low-energy muon spin spectroscopy we discover the existence of surface magnetism in Sr2RuO4 in its normal state. We detect static weak dipolar fields yet manifesting at an onset temperature higher than 50 K. We ascribe this unconventional magnetism to orbital loop currents forming at the reconstructed Sr2RuO4 surface. Our observations set a reference for the discovery of the same magnetic phase in other materials and unveil an electronic ordering mechanism that can influence electron pairing with broken time reversal symmetry.

Imaging quantum fluctuations near criticality.

A quantum phase transition (QPT) occurs between two competing phases of matter at zero temperature, driven by quantum fluctuations. Though the presence of these fluctuations is well established, they have not been locally imaged in space and their local dynamics has not been studied so far. We use a scanning superconducting quantum interference device to image quantum fluctuations in the vicinity of the QPT from a superconductor to an insulator. We find fluctuations of the diamagnetic response in both space and time that survive well below the transition temperature, demonstrating their quantum nature. The fluctuations appear as telegraph-like noise with a range of characteristic times and a non-monotonic temperature dependence, revealing unexpected quantum granularity. The lateral dimension of these fluctuations grows towards criticality, offering a new measurable length scale. Our results provide physical insight about the reorganization of phases across a QPT, with implications for any theoretical description. This paves a new route for future quantum information applications.

Spatiotemporal vortex matter oscillations in Bi2Sr2CaCu2O8+delta crystals.

We observed an oscillatory behavior, both in space and time, of the induction in Bi2Sr2CaCu2O8+delta crystals exposed to a steady magnetic field. This new "flux waves" phenomenon appears near the order-disorder vortex phase transition, under specific conditions of temperature and induction gradient. A theoretical description of this effect is based on two coupled equations: the Landau-Khalatnikov dynamic equation for the order parameter of the vortex phase transition and the diffusion equation for the time evolution of the magnetic induction. A linear stability analysis of these equations predicts an oscillatory instability characterized by a period and wavelength in accordance with the experimental results.

Dynamic order-to-metastable-disorder vortex matter transition in Bi2Sr2CaCu2O8+delta.

Magneto-optical measurements of transient vortex states in Bi2Sr2CaCu2O8+delta show enhanced effects of metastability in prism-shaped as compared to platelet crystals including a significant shift of the second magnetization peak and qualitatively different dynamics. In contrast to platelets, where dislocations are generated only at the sample edges, we propose that in prism samples the dislocations are generated dynamically in the entire sample due to distributed surface barriers. As a result, a dynamic phase transition from a Bragg glass to a metastable disordered phase may occur well below the thermodynamic transition field.

Flux-flow resistivity anisotropy in the instability regime of the a-b plane of epitaxial superconducting YBa2Cu3O7-delta thin films.

Measurements of the nonlinear flux-flow resistivity rho and the critical vortex velocity vphi* at high voltage bias close to the instability regime predicted by Larkin and Ovchinnikov (Z. Eksp. Teor. Fiz 68, 1915 (1975) [Sov. Phys. JETP 41, 960 (1976)]) are reported along the node and antinode directions of the d-wave order parameter in the a-b plane of epitaxial YBa2Cu3O7-delta films. In this pinning-free regime, rho and vphi* are found to be anisotropic with values in the node direction larger on average by 10% than in the antinode direction. The anisotropy of rho is almost independent of temperature and field. We attribute the observed results to the anisotropic quasiparticle distribution on the Fermi surface of YBa2Cu3O7-delta.