Electro-optic 3D snapshot of a laser wakefield accelerated kilo-ampere electron bunch.

Laser wakefield acceleration, as an advanced accelerator concept, has attracted great attentions for its ultrahigh acceleration gradient and the capability to produce high brightness electron bunches. The three-dimensional (3D) density serves as an evaluation metric for the particle bunch quality and is intrinsically related to the applications of an accelerator. Despite its significance, this parameter has not been experimentally measured in the investigation of laser wakefield acceleration. We report on an electro-optic 3D snapshot of a laser wakefield electron bunch at a position outside the plasma. The 3D shape of the electron bunch was detected by simultaneously performing optical transition radiation imaging and electro-optic sampling. Detailed 3D structures to a few micrometer levels were reconstructed using a genetic algorithm. The electron bunch possessed a transverse size of less than 30 micrometers. The current profile shows a multi-peak structure. The main peak had a duration of < 10 fs and a peak current > 1 kA. The maximum electron 3D number density was ~ 9 × 1021 m -3. This research demonstrates a feasible way of 3D density monitoring on femtosecond kilo-ampere electron bunches, at any position of a beam transport line for relevant applications.

Modular supersonic nozzle for the stable laser-driven electron acceleration.

The sharp density down-ramp injection (shock injection) mechanism produces the quasi-monoenergetic electron beam with a bunch duration of tens of femtoseconds via laser wakefield acceleration. The stability of the accelerated electron beam strongly depends on the stability of the laser beam and the shock structure produced by the supersonic gas nozzle. In this paper, we report the study of a newly designed modular supersonic nozzle with a flexible stilling chamber and a converging-diverging structure. The performance of the nozzle is studied both numerically and experimentally with the computational fluid dynamics simulation and the Mach-Zehnder interferometry method. The simulation results and the experimental measurements are well consistent, and both prove the effectiveness of the stilling chamber in stabilizing the gas flow.

Notable improvements on LWFA through precise laser wavefront tuning.

Laser wakefield acceleration (LWFA) continues to grow and awaken interest worldwide, especially as in various applications it approaches performance comparable to classical accelerators. However, numerous challenges still exist until this can be a reality. The complex non-linear nature of the process of interaction between the laser and the induced plasma remains an obstacle to the widespread LWFA use as stable and reliable particle sources. It is commonly accepted that the best wavefront is a perfect Gaussian distribution. However, experimentally, this is not correct and more complicated ones can potentially give better results. in this work, the effects of tuning the laser wavefront via the controlled introduction of aberrations are explored for an LWFA accelerator using the shock injection configuration. Our experiments show the clear unique correlation between the generated beam transverse characteristics and the different input wavefronts. The electron beams stability, acceleration and injection are also significantly different. We found that in our case, the best beams were generated with a specific complex wavefront. A greater understanding of electron generation as function of the laser input is achieved thanks to this method and hopes towards a higher level of control on the electrons beams by LWFA is foreseen.

Laser-driven multi-MeV high-purity proton acceleration via anisotropic ambipolar expansion of micron-scale hydrogen clusters.

Multi-MeV high-purity proton acceleration by using a hydrogen cluster target irradiated with repetitive, relativistic intensity laser pulses has been demonstrated. Statistical analysis of hundreds of data sets highlights the existence of markedly high energy protons produced from the laser-irradiated clusters with micron-scale diameters. The spatial distribution of the accelerated protons is found to be anisotropic, where the higher energy protons are preferentially accelerated along the laser propagation direction due to the relativistic effect. These features are supported by three-dimensional (3D) particle-in-cell (PIC) simulations, which show that directional, higher energy protons are generated via the anisotropic ambipolar expansion of the micron-scale clusters. The number of protons accelerating along the laser propagation direction is found to be as high as 1.6 [Formula: see text] [Formula: see text] 10[Formula: see text]/MeV/sr/shot with an energy of 2.8 [Formula: see text] MeV, indicating that laser-driven proton acceleration using the micron-scale hydrogen clusters is promising as a compact, repetitive, multi-MeV high-purity proton source for various applications.

Highly stable sub-nanosecond Nd:YAG pump laser for optically synchronized optical parametric chirped-pulse amplification.

We developed an optically synchronized highly stable frequency-doubled Nd:YAG laser with sub-nanosecond pulse duration. The 1064 nm seed pulses generated by soliton self-frequency shift in a photonic crystal fiber from Ti:sapphire oscillator pulses were stabilized by controlling input pulse polarization. The seed pulses were amplified to 200 mJ by diode-pumped amplifiers with a high stability of only <0.2% (rms). With an external LBO doubler, the system generated 330 ps green pulse energy of 130 mJ at 532 nm with a conversion efficiency of 65%. The pulse duration was further extended to 490 ps by adjusting Nd:YAG crystal temperature. To the best of our knowledge, these results present a longer pulse duration with higher stability than previous Nd:YAG lasers with sub-nanosecond optical synchronization.

Relativistic flying forcibly oscillating reflective diffraction grating.

Relativistic flying forcibly oscillating reflective diffraction gratings are formed by an intense laser pulse (driver) in plasma. The mirror surface is an electron density singularity near the joining area of the wake wave cavity and the bow wave; it moves together with the driver laser pulse and undergoes forced oscillations induced by the field. A counterpropagating weak laser pulse (source) is incident at grazing angles, being efficiently reflected and enriched by harmonics. The reflected spectrum consists of the source pulse base frequency and its harmonics, multiplied by a large factor due to the double Doppler effect.

New algorithm using L1 regularization for measuring electron energy spectra.

Retrieving the spectrum of physical radiation from experimental measurements typically involves using a mathematical algorithm to deconvolve the instrument response function from the measured signal. However, in the field of signal processing known as "Source Separation" (SS), which refers to the process of computationally retrieving the separate source components that generate an overlapping signal on the detector, the deconvolution process can become an ill-posed problem and crosstalk complicates the separation of the individual sources. To overcome this problem, we have designed a magnetic spectrometer for inline electron energy spectrum diagnosis and developed an analysis algorithm using techniques applicable to the problem of SS. An unknown polychromatic electron spectrum is calculated by sparse coding using a Gaussian basis function and an L1 regularization algorithm with a sparsity constraint. This technique is verified by using a specially designed magnetic field electron spectrometer. We use Monte Carlo simulations of the detector response to Maxwellian input energy distributions with electron temperatures of 5.0 MeV, 10.0 MeV, and 15.0 MeV to show that the calculated sparse spectrum can reproduce the input spectrum with an optimum energy bin width automatically selected by the L1 regularization. The spectra are reproduced with a high accuracy of less than 4.0% error, without an initial value. The technique is then applied to experimental measurements of intense laser accelerated electron beams from solid targets. Our analysis concept of spectral retrieval and automatic optimization of energy bin width by sparse coding could form the basis of a novel diagnostic method for spectroscopy.

Experimental investigation on the temporal contrast of pre-pulses by post-pulses in a petawatt laser facility.

We experimentally explore the generation of pre-pulses by post-pulses, created through internal reflection in the optical components, by the nonlinear process associated with the B-integral in the laser chain of the petawatt (PW) facility J-KAREN-P. At a large time delay between the main and the post-pulses, we have found that the pre-pulses are not generated from their counterpart post-pulses at an identical time difference before the main pulse, and the temporal shapes of the pre-pulses are greatly distorted asymmetrically. We have also observed that the peak intensities of the pre-pulses are drastically suppressed compared to the expected value at a small time delay. We briefly describe the origins of the pre-pulses generated by the post-pulses and demonstrate the removal of the pre-pulses by switching to optical components with a small wedge angle at our PW laser facility.

Light source based on a 100†mm-long monolithic undulator magnet with a very short 4†mm-period length.

A novel method to fabricate undulator magnets of a-few-millimetre-period length is being explored. Plate-type magnets, 100 mm-long with 4 mm-period length, have been successfully fabricated. They produce an undulator field of approximately 3 kG at a gap of 1.6 mm. Prototype undulators based on this technology have been constructed. Field measurements and characterization show that the quality of the undulator field of these plate magnets is sufficient for an undulator light source, and the calculated spectrum shows that the fundamental radiation emitted from this field is quite satisfactory. Test experiments for light generation using a real electron beam have been carried out at a test accelerator at the Research Center for Electron Photon Science (ELPH), Tohoku University, Japan, which is able to realize optics conditions to accept a very short gap of ∼1.6 mm. First observation and characterization of blue light was successfully accomplished.

High-contrast high-intensity repetitive petawatt laser.

We report the generation of 63 J of broadband pulse energies at 0.1 Hz from the J-KAREN-P laser, which is based on an OPCPA/Ti:sapphire hybrid architecture. Pulse compression down to 30 fs indicates a peak power of over 1 PW. High temporal contrast of 1012 prior to the main pulse has been demonstrated with 10 J output energy. High intensities of 1022 W/cm2 on target by focusing a 0.3 PW laser with an f/1.3 off-axis parabolic mirror have been achieved. Fundamental processes of laser matter interaction at over 1022 W/cm2 intensities belong to a new branch of science that will be the principal research task of our infrastructure.

Approaching the diffraction-limited, bandwidth-limited Petawatt.

J-KAREN-P is a high-power laser facility aiming at the highest beam quality and irradiance for performing state-of-the art experiments at the frontier of modern science. Here we approached the physical limits of the beam quality: diffraction limit of the focal spot and bandwidth limit of the pulse shape, removing the chromatic aberration, angular chirp, wavefront and spectral phase distortions. We performed accurate measurements of the spot and peak fluence after an f/1.3 off-axis parabolic mirror under the full amplification at the power of 0.3 PW attenuated with ten high-quality wedges, resulting in the irradiance of ~1022 W/cm2 and the Strehl ratio of ~0.5.

Ion pinhole imaging diagnostics on fast ion source in femtosecond laser plasma of cluster targets.

The spatial configuration of the ion source generated under femtosecond laser interaction with clusters is investigated. While intense laser pulses (36 fs, 60 mJ, intensity of 4 × 1017 W/cm2) propagated in CO2 cluster (~0.22 µm in diameter) media, the shape of the obtained plasma ion source was registered for the first time by means of pinhole imaging method. The remarkable decrease in fast ion yield in the vicinity of the assumed best laser focus near the gas cluster jet axis is observed. Such observed anisotropy of the ion source is suggested to originate from the influence of the laser prepulse destroying clusters in advance to the arrival of the main pulse. The assumption is confirmed by optical shadowgraphy images of the plasma channel and is important for further development of an efficient laser-plasma-based fast ion source. Following the observed geometry of the ion source, the laser intensity limit allowing to accelerate ions to ~100 keV energy range was estimated.

Decomposition of powerful axisymmetrically polarized laser pulses in underdense plasma.

Interaction of relativistically intense axisymmetrically polarized (radially or azimuthally polarized) laser pulses (RIAPLP) with underdense plasma is shown experimentally and theoretically to be essentially different from the interaction of conventional Gaussian pulses. The difference is clearly observed in distinct spectra of the side-scattered laser light for the RIAPLP and Gaussian pulses, as well as in the appearance of a spatially localized strong side emission of second harmonic of the laser pulse in the case of RIAPLP. According to our analysis based on three-dimensional particle-in-cell simulations, this is a result of instability in the propagation of RIAPLP in uniform underdense plasma.

Revealing the second harmonic generation in a femtosecond laser-driven cluster-based plasma by analyzing shapes of Ar XVII spectral lines.

We present experiments dealing with a femtosecond laser-driven cluster-based plasma, where by analyzing the nonlinear phenomenon of satellites of spectral lines of Ar XVII, we revealed the nonlinear phenomenon of the generation of the second harmonic of the laser frequency. For performing this analysis we developed new results in the theory of satellites of spectral lines. From such lineshape analysis we found, in particular, that the efficiency of converting the short (40 fs) intense (3x10¹8 W/cm²) incident laser light into the second harmonic was 2%. This result is in the excellent agreement with the 2-Dimensional Particle-In-Cell (2D PIC) simulation that we also performed. There is also an order of magnitude agreement between the thresholds for the SHG found from the line shape analysis and from the 2D PIC simulations.

A laser-plasma-produced soft X-ray laser at 89 eV generates DNA double-strand breaks in human cancer cells.

While it has been expected that X-ray laser will be widely applied to biomedical studies, this has not been achieved to date and its biological effects such as DNA damage have not been evaluated. As a first step for its biological application, we developed a culture cell irradiation system, particularly designed for a plasma-driven soft X-ray laser pulse, to investigate whether the soft X-ray laser is able to induce DNA double strand breaks (DSBs) in living cells or not. The human adenocarcimona cell line A549 was irradiated with the soft X-ray laser at a photon energy of 89 eV and the repair focus formation of the DSBs was assessed by immunofluorescence staining with antiphosphorylated DNA-PKcs (p-DNA-PKcs), ATM (p-ATM) and γ-H2AX antibody. The p-DNA-PKcs, ATM, and γ-H2AX foci were clearly identified after soft X-ray laser irradiation. Furthermore, the increase in the X-ray laser shot number, even from a single shot, results in the increase in p-DNA-PKcs foci. These results are the first evidence that the 89 eV soft X-ray laser is able to induce DSB in living cells. Our study demonstrated that this irradiation system is a useful tool for investigating the radiobiological effect of soft X-ray laser.

Observation and theory of X-ray mirages.

The advent of X-ray lasers allowed the realization of compact coherent soft X-ray sources, thus opening the way to a wide range of applications. Here we report the observation of unexpected concentric rings in the far-field beam profile at the output of a two-stage plasma-based X-ray laser, which can be considered as the first manifestation of a mirage phenomenon in X-rays. We have developed a method of solving the Maxwell-Bloch equations for this problem, and find that the experimentally observed phenomenon is due to the emergence of X-ray mirages in the plasma amplifier, appearing as phase-matched coherent virtual point sources. The obtained results bring a new insight into the physical nature of amplification of X-ray radiation in laser-induced plasma amplifiers and open additional opportunities for X-ray plasma diagnostics and extreme ultraviolet lithography.

Soft x-ray free-electron laser imaging by LiF crystal and film detectors over a wide range of fluences.

LiF crystal and film detectors were used to measure the far-field fluence profile of a self-amplified spontaneous-emission free-electron laser beam and diffraction imaging with high spatial resolution. In these measurements the photoluminescence (PL) response of LiF crystal and film was compared over a wide range of soft x-ray fluences. It was found that the soft x-ray fluence dependences of LiF crystal and film differ. At low fluence, the LiF crystal shows higher PL response compared to LiF film, while this comparison is the opposite at higher fluence. Accurate measurement of LiF crystal and film PL response is important for precise characterization of the spatial, spectral, and coherence features of x-ray beams across the full profile and in localized areas. For such measurements, crucial LiF detector attributes are high spatial resolution and high dynamic range.

High-power γ-ray flash generation in ultraintense laser-plasma interactions.

When high-intensity laser interaction with matter enters the regime of dominated radiation reaction, the radiation losses open the way for producing short pulse high-power γ-ray flashes. The γ-ray pulse duration and divergence are determined by the laser pulse amplitude and by the plasma target density scale length. On the basis of theoretical analysis and particle-in-cell simulations with the radiation friction force incorporated, optimal conditions for generating a γ-ray flash with a tailored overcritical density target are found.

Proton acceleration to 40 MeV using a high intensity, high contrast optical parametric chirped-pulse amplification/Ti:sapphire hybrid laser system.

Using a high-contrast (10(10):1) and high-intensity (10(21) W/cm(2)) laser pulse with the duration of 40 fs from an optical parametric chirped-pulse amplification/Ti:sapphire laser, a 40 MeV proton bunch is obtained, which is a record for laser pulse with energy less than 10 J. The efficiency for generation of protons with kinetic energy above 15 MeV is 0.1%.

Optical features of a LiF crystal soft X-ray imaging detector irradiated by free electron laser pulses.

Optical features of point defects photoluminescence in LiF crystals, irradiated by soft X-ray pulses of the Free Electron Laser with wavelengths of 17.2 - 61.5 nm, were measured. We found that peak of photoluminescence spectra lies near of 530 nm and are associated with emission of F3+ centers. Our results suggest that redistribution of photoluminescence peak intensity from the red to the green part of the spectra is associated with a shortening of the applied laser pulses down to pico - or femtosecond durations. Dependence of peak intensity of photoluminescence spectra from the soft X-ray irradiation fluence was measured and the absence of quenching phenomena, even at relatively high fluencies was found, which is very important for wide applications of LiF crystal X-ray imaging detectors.