Distributed quantum sensing of multiple phases with fewer photons.

Distributed quantum metrology has drawn intense interest as it outperforms the optimal classical counterparts in estimating multiple distributed parameters. However, most schemes so far have required entangled resources consisting of photon numbers equal to or more than the parameter numbers, which is a fairly demanding requirement as the number of nodes increases. Here, we present a distributed quantum sensing scenario in which quantum-enhanced sensitivity can be achieved with fewer photons than the number of parameters. As an experimental demonstration, using a two-photon entangled state, we estimate four phases distributed 3 km away from the central node, resulting in a 2.2 dB sensitivity enhancement from the standard quantum limit. Our results show that the Heisenberg scaling can be achieved even when using fewer photons than the number of parameters. We believe our scheme will open a pathway to perform large-scale distributed quantum sensing with currently available entangled sources.

Testing multiple hypotheses on the colour change of treefrogs in response to various external conditions.

Amphibians are famous for their ability to change colours. And a considerable number of studies have investigated the internal and external factors that affect the expression of this phenotypic plasticity. Evidence to date suggests that thermoregulation and camouflage are the main pressures that influence frogs' adaptive colour change responses. However, certain gaps in our knowledge of this phenomenon remain, namely: (i) how do frogs adjust their colour in response to continuously changing external conditions?; (ii) what is the direction of change when two different functions of colour (camouflage and thermoregulation) are in conflict?; (iii) does reflectance in the near-infrared region show thermally adaptive change?; and (iv) is the colour change ability of each frog an individual trait (i.e., consistent within an individual over time)? Using Dryophytes japonicus (Hylidae, Hyla), we performed a series of experiments to answer the above questions. We first showed that frogs' responses to continuously-changing external conditions (i.e., background colour and temperature) were not linear and limited to the range they experience under natural conditions. Second, when a functional conflict existed, camouflage constrained the adaptive response for thermoregulation and vice versa. Third, though both temperature and background colour induced a change in near-infrared reflectance, this change was largely explained by the high correlation between colour (reflectance in the visible spectrum) and near-infrared reflectance. Fourth, within-individual variation in colour change capacity (i.e., the degree of colour change an individual can display) was lower than inter-individual variation, suggesting individuality of colour change capacity; however, we also found that colour change capacity could change gradually with time within individuals. Our results collectively reveal several new aspects of how evolution shapes the colour change process and highlight how variation in external conditions restricts the extent of colour change in treefrogs.

Entangling three identical particles via spatial overlap.

Quantum correlations between identical particles are at the heart of quantum technologies. Several studies with two identical particles have shown that the spatial overlap and indistinguishability between the particles are necessary for generating bipartite entanglement. On the other hand, researches on the extension to more than two-particle systems are limited by the practical difficulty to control multiple identical particles in laboratories. In this work, we propose schemes to generate two fundamental classes of genuine tripartite entanglement, i.e., GHZ and W classes, which are experimentally demonstrated using linear optics with three identical photons. We also show that the tripartite entanglement class decays from the genuine entanglement to the full separability as the particles become more distinguishable from each other. Our results support the prediction that particle indistinguishability is a fundamental element for entangling identical particles.

Demonstration of Complete Information Trade-Off in Quantum Measurement.

While an information-disturbance trade-off in quantum measurement has been at the core of foundational quantum physics and constitutes a basis of secure quantum information processing, recently verified reversibility of a quantum measurement requires to refine it toward a complete version of information trade-off in quantum measurement. Here we experimentally demonstrate a trade-off relation among all information contents, i.e., information gain, disturbance, and reversibility in quantum measurement. By exploring quantum measurements applied on a photonic qutrit, we observe that the information of a quantum state is split into three distinct parts accounting for the extracted, disturbed, and reversible information. We verify that such different parts of information are in trade-off relations not only pairwise but also triplewise all at once, and find that the triplewise relation is tighter than any of the pairwise relations. Finally, we realize optimal quantum measurements that inherently preserve quantum information without loss of information, which offer wider applications in measurement-based quantum information processing.

Sub-10 nm Precision Engineering of Solid-State Defects via Nanoscale Aperture Array Mask.

Engineering a strongly interacting uniform qubit cluster would be a major step toward realizing a scalable quantum system for quantum sensing and a node-based qubit register. For a solid-state system that uses a defect as a qubit, various methods to precisely position defects have been developed, yet the large-scale fabrication of qubits within the strong coupling regime at room temperature continues to be a challenge. In this work, we generate nitrogen vacancy (NV) color centers in diamond with sub-10 nm scale precision using a combination of nanoscale aperture arrays (NAAs) with a high aspect ratio of 10 and a secondary E-beam hole pattern used as an ion-blocking mask. We perform optical and spin measurements on a cluster of NV spins and statistically investigate the effect of the NAAs during an ion-implantation process. We discuss how this technique is effective for constructing a scalable system.

Habitat ephemerality affects the evolution of contrasting growth strategies and cannibalism in anuran larvae.

Ephemeral streams are challenging environments for tadpoles; thus, adaptive features that increase the survival of these larvae should be favored by natural selection. In this study, we compared the adaptive growth strategies of Bombina orientalis (the oriental fire-bellied toad) tadpoles from ephemeral streams with those of such tadpoles from non-ephemeral streams. Using a common garden experiment, we tested the interactive effects of location (ephemeral vs. non-ephemeral), food availability, and growing density on larval period, weight at metamorphosis, and cannibalism. We found that tadpoles from ephemeral streams underwent a shorter larval period compared with those from non-ephemeral streams but that this difference was contingent on food availability. The observed faster growth is likely to be an adaptive response because tadpoles in ephemeral streams experience more biotic/abiotic stressors, such as desiccation risk and limited resources, compared with those in non-ephemeral streams, with their earlier metamorphosis potentially resulting in survival benefits. As a trade-off for their faster growth, tadpoles from ephemeral streams generally had a lower body weight at metamorphosis compared with those from non-ephemeral streams. We also found lower cannibalism rates among tadpoles from ephemeral streams, which can be attributed to the indirect fitness costs of cannibalizing their kin. Our study demonstrates how ephemeral habitats have affected the evolutionary change in cannibalistic behaviors in anurans and provides additional evidence that natural selection has mediated the evolution of growth strategies of tadpoles in ephemeral streams.

Implementation of a 3 × 3 directionally-unbiased linear optical multiport.

Linear optical multiports are widely used in photonic quantum information processing. Naturally, these devices are directionally-biased since photons always propagate from the input ports toward the output ports. Recently, the concept of directionally-unbiased linear optical multiports was proposed. These directionally-unbiased multiports allow photons to propagate along a reverse direction, which can greatly reduce the number of required linear optical elements for complicated linear optical quantum networks. Here, we report an experimental demonstration of a 3 × 3 directionally-unbiased linear optical fiber multiport using an optical tritter and mirrors. Compared to the previous demonstration using bulk optical elements which works only with light sources with a long coherence length, our experimental directionally-unbiased 3 × 3 optical multiport does not require a long coherence length since it provides negligible optical path length differences among all possible optical trajectories. It can be a useful building block for implementing large-scale quantum walks on complex graph networks.

Quantum enhanced multiple-phase estimation with multi-mode N00N states.

Quantum metrology can achieve enhanced sensitivity for estimating unknown parameters beyond the standard quantum limit. Recently, multiple-phase estimation exploiting quantum resources has attracted intensive interest for its applications in quantum imaging and sensor networks. For multiple-phase estimation, the amount of enhanced sensitivity is dependent on quantum probe states, and multi-mode N00N states are known to be a key resource for this. However, its experimental demonstration has been missing so far since generating such states is highly challenging. Here, we report generation of multi-mode N00N states and experimental demonstration of quantum enhanced multiple-phase estimation using the multi-mode N00N states. In particular, we show that the quantum Cramer-Rao bound can be saturated using our two-photon four-mode N00N state and measurement scheme using a 4 × 4 multi-mode beam splitter. Our multiple-phase estimation strategy provides a faithful platform to investigate multiple parameter estimation scenarios.

Extended Spatially Localized Perturbation GAN (eSLP-GAN) for Robust Adversarial Camouflage Patches.

Deep neural networks (DNNs), especially those used in computer vision, are highly vulnerable to adversarial attacks, such as adversarial perturbations and adversarial patches. Adversarial patches, often considered more appropriate for a real-world attack, are attached to the target object or its surroundings to deceive the target system. However, most previous research employed adversarial patches that are conspicuous to human vision, making them easy to identify and counter. Previously, the spatially localized perturbation GAN (SLP-GAN) was proposed, in which the perturbation was only added to the most representative area of the input images, creating a spatially localized adversarial camouflage patch that excels in terms of visual fidelity and is, therefore, difficult to detect by human vision. In this study, the use of the method called eSLP-GAN was extended to deceive classifiers and object detection systems. Specifically, the loss function was modified for greater compatibility with an object-detection model attack and to increase robustness in the real world. Furthermore, the applicability of the proposed method was tested on the CARLA simulator for a more authentic real-world attack scenario.

Inotodiol From Inonotus obliquus Chaga Mushroom Induces Atypical Maturation in Dendritic Cells.

Dendritic cells (DCs) have the ability to stimulate naïve T cells that coordinate subsequent adaptive response toward an inflammatory response or tolerance depending on the DC differentiation level. Inotodiol, a lanostane triterpenoid found in Inonotus obliquus (wild Chaga mushroom), is a natural compound with a wide range of biological activities. In this study, we investigated whether inotodiol promotes the maturation of bone marrow-derived DCs (BMDCs) and inotodiol-treated BMDCs induce T cell activation. Inotodiol increased the expression of surface maturation markers, including MHC-I, MHC-II, CD86, and CD40, on BMDCs without affecting the production of various cytokines, including TNF-α and IL-12p40 in these cells. T cells primed with inotodiol-treated BMDCs proliferated and produced IL-2, without producing other cytokines, including IL-12p40 and IFN-γ. Injection of inotodiol into mice induced maturation of splenic DCs and IL-2 production, and the administration of inotodiol and inotodiol-treated BMDCs induced the proliferation of adoptively transferred CD8+ T cells in vivo. The phosphatidylinositol-3-kinase inhibitor wortmannin abrogated the upregulation of Akt phosphorylation and CD86 and MHC-II expression induced by inotodiol. However, inotodiol failed to induce phosphorylation of the IκB kinase and degradation of IκB-α, and increased expression of CD86 induced by inotodiol was not blocked by an IκB kinase inhibitor. These results suggest that inotodiol induces a characteristic type of maturation in DCs through phosphatidylinositol-3-kinase activation independent of NF-κB, and inotodiol-treated DCs enhance T cell proliferation and IL-2 secretion.

A Distributed Black-Box Adversarial Attack Based on Multi-Group Particle Swarm Optimization.

Adversarial attack techniques in deep learning have been studied extensively due to its stealthiness to human eyes and potentially dangerous consequences when applied to real-life applications. However, current attack methods in black-box settings mainly employ a large number of queries for crafting their adversarial examples, hence making them very likely to be detected and responded by the target system (e.g., artificial intelligence (AI) service provider) due to its high traffic volume. A recent proposal able to address the large query problem utilizes a gradient-free approach based on Particle Swarm Optimization (PSO) algorithm. Unfortunately, this original approach tends to have a low attack success rate, possibly due to the model's difficulty of escaping local optima. This obstacle can be overcome by employing a multi-group approach for PSO algorithm, by which the PSO particles can be redistributed, preventing them from being trapped in local optima. In this paper, we present a black-box adversarial attack which can significantly increase the success rate of PSO-based attack while maintaining a low number of query by launching the attack in a distributed manner. Attacks are executed from multiple nodes, disseminating queries among the nodes, hence reducing the possibility of being recognized by the target system while also increasing scalability. Furthermore, we utilize Multi-Group PSO with Random Redistribution (MGRR-PSO) for perturbation generation, performing better than the original approach against local optima, thus achieving a higher success rate. Additionally, we propose to efficiently remove excessive perturbation (i.e, perturbation pruning) by utilizing again the MGRR-PSO rather than a standard iterative method as used in the original approach. We perform five different experiments: comparing our attack's performance with existing algorithms, testing in high-dimensional space in ImageNet dataset, examining our hyperparameters (i.e., particle size, number of clients, search boundary), and testing on real digital attack to Google Cloud Vision. Our attack proves to obtain a 100% success rate on MNIST and CIFAR-10 datasets and able to successfully fool Google Cloud Vision as a proof of the real digital attack by maintaining a lower query and wide applicability.

Diamond photonic crystal mirror with a partial bandgap by two 2D photonic crystal layers.

In this study, photonic crystals with a partial bandgap are demonstrated in the visible region using single-crystal diamonds. Quasi-three-dimensional photonic crystal structures are fabricated in the surface of the single-crystal diamonds using a tetrahedron Faraday cage that enables angled dry etching in three directions simultaneously. The reflection spectra can be controlled by varying the lattice constant of the photonic crystals. In addition, nitrogen-vacancy center single-photon sources are implanted on top of the diamond photonic crystals, and doubled collection efficiency from the light sources is achieved.

Entangling bosons through particle indistinguishability and spatial overlap.

Particle identity and entanglement are two fundamental quantum properties that work as major resources for various quantum information tasks. However, it is still a challenging problem to understand the correlation of the two properties in the same system. While recent theoretical studies have shown that the spatial overlap between identical particles is necessary for nontrivial entanglement, the exact role of particle indistinguishability in the entanglement of identical particles has never been analyzed quantitatively before. Here, we theoretically and experimentally investigate the behavior of entanglement between two bosons as spatial overlap and indistinguishability simultaneously vary. The theoretical computation of entanglement for generic two bosons with pseudospins is verified experimentally in a photonic system. Our results show that the amount of entanglement is a monotonically increasing function of both quantities. We expect that our work provides an insight into deciphering the role of the entanglement in quantum networks that consist of identical particles.

In-Depth Investigation of the Correlation between Organic Semiconductor Orientation and Energy-Level Alignment Using In Situ Photoelectron Spectroscopy.

Organic semiconductors (OSCs) are of interest for replacing traditional Si-based semiconductors as their flexibility and transparency enable new applications. The properties of OSC materials greatly depend on their orientation and molecular arrangement, which are strongly dependent on the underlying substrate material. Hence, in this study, in situ ultraviolet photoelectron spectroscopy (UPS) is used to elucidate the effect of the substrate on OSC orientation. Two types of OSCs, namely those with shape anisotropy (pentacene, dinaphtho[2,3-b:2',3'-f]thieno[3,2-b]thiophene, and dibenzothiopheno[6,5-b:6',5'-f]thieno[3,2-b]thiophene) and those with shape isotropy (N,N'-di(1-naphthyl)-N,N'-diphenyl-(1,1'-biphenyl)-4,4'-diamine, tris(4-carbazoyl-9-ylphenyl)amine, and [6,6]-phenyl C71 butyric acid methyl ester), are deposited on different electrode materials. The differences in the UPS spectra of these materials are observed directly. In general, the orientation of anisotropic OSC molecules significantly depends on the substrate properties, while that of the isotropic ones do not. All the anisotropic OSC molecules grown on poly(3,4-ethylenedioxythiophene)-polystyrenesulfonate (PEDOT:PSS) electrodes show a greater degree of molecular ordering than those grown on Au and multiwalled carbon nanotube/PEDOT:PSS electrodes. The molecular arrangements within the OSC/electrode structures are reflected in the energy-level shifts in the corresponding UPS spectra and hence in the electronic configurations. The results of this study should aid the design and synthesis of OSC materials with configurations suitable for organic electronic devices.

Prey with hidden colour defences benefit from their similarity to aposematic signals.

Some camouflaged animals hide colour signals and display them only transiently. These hidden colour signals are often conspicuous and are used as a secondary defence to warn or startle predators (deimatic displays) and/or to confuse them (flash displays). The hidden signals used in these displays frequently resemble typical aposematic signals, so it is possible that prey with hidden signals have evolved to employ colour patterns of a form that predators have previously learned to associate with unprofitability. Here, we tested this hypothesis by conducting two experiments that examined the effect of predator avoidance learning on the efficacy of deimatic and flash displays. We found that the survival benefits of both deimatic and flash displays were substantially higher against predators that had previously learned to associate the hidden colours with unprofitability than against naive predators. These findings help explain the phenological patterns we found in 1568 macro-lepidopteran species on three continents: species with hidden signals tend to occur later in the season than species without hidden signals.

Reference-frame-independent, measurement-device-independent quantum key distribution using fewer quantum states.

Reference-frame-independent quantum key distribution (RFI-QKD) provides a practical way to generate secret keys between two remote parties without sharing common reference frames. On the other hand, measurement-device-independent QKD (MDI-QKD) offers a high level of security, as it is immune to all quantum hacking attempts to measurement devices. The combination of these two QKD protocols, i.e., RFI-MDI-QKD, is one of the most fascinating QKD protocols, since it holds advantages of both practicality and security. For further practicality of RFI-MDI-QKD, it is beneficial to reduce the implementation complexity. Here, we show that RFI-MDI-QKD can be implemented using fewer quantum states than those of its original proposal. We find that, in principle, the number of quantum states for one of the parties can be reduced from six to three without compromising security. Compared to conventional RFI-MDI-QKD where both parties transmit six quantum states, it significantly simplifies the implementation of the QKD protocol. We also verify the feasibility of the scheme with a proof-of-principle experiment.

Origins of High Performance and Degradation in the Mixed Perovskite Solar Cells.

The origins of the high device performance and degradation in the air are the greatest issues for commercialization of perovskite solar cells. Here this study investigates the possible origins of the mixed perovskite cells by monitoring defect states and compositional changes of the perovskite layer over the time. The results of deep-level transient spectroscopy analysis reveal that a newly identified defect formed by Br atoms exists at deep levels of the mixed perovskite film, and its defect state shifts when the film is aged in the air. The change of the defect state is originated from loss of the methylammonium molecules of the perovskite layer, which results in decreased JSC , deterioration of the power conversion efficiency and long-term stability of perovskite solar cells. The results provide a powerful strategy to diagnose and manage the efficiency and stability of perovskite solar cells.

Informationally symmetrical Bell state preparation and measurement.

Bell state measurement (BSM) plays crucial roles in photonic quantum information processing. The standard linear optical BSM is based on Hong-Ou-Mandel interference where two photons meet and interfere at a beamsplitter (BS). However, a generalized two-photon interference is not based on photon-photon interaction, but interference between two-photon probability amplitudes. Therefore, it might be possible to implement BSM without interfering photons at a BS. Here, we investigate a linear optical BSM scheme which does not require two photon overlapping at a BS. By unleashing the two photon coexistence condition, it can be symmetrically divided into two parties. The symmetrically dividable property suggests an informationally symmetrical BSM between remote parties without a third party. We also present that our BSM scheme can be used for Bell state preparation between remote parties without a third party. Since our BSM scheme can be easily extended to multiple photons, it can be useful for various quantum communication applications.