Chiral phonons: circularly polarized Raman spectroscopy and ab initio calculations in a chiral crystal tellurium.

Recently, phonons with chirality (chiral phonons) have attracted significant attention. Chiral phonons exhibit angular and pseudoangular momenta. In circularly polarized Raman spectroscopy, the peak split of the Γ 3 mode is detectable along the principal axis of the chiral crystal in the backscattering configuration. In addition, peak splitting occurs when the pseudoangular momenta of the incident and scattered circularly polarized light are reversed. Until now, chiral phonons in binary crystals have been observed, whereas those in unary crystals have not been observed. Here, we observe chiral phonons in a chiral unary crystal Te. The pseudoangular momentum of the phonon is obtained in Te by an ab initio calculation. From this calculation, we verified the conservation law of pseudoangular momentum in Raman scattering. From this conservation law, we determined the handedness of the chiral crystals. We also evaluated the true chirality of the phonons using a measure with symmetry similar to that of an electric toroidal monopole.

Chirality-Induced Spin Polarization over Macroscopic Distances in Chiral Disilicide Crystals.

A spin-polarized state is examined under charge current at room temperature without magnetic fields in chiral disilicide crystals NbSi_{2} and TaSi_{2}. We found that a long-range spin transport occurs over ten micrometers in these inorganic crystals. A distribution of crystalline grains of different handedness is obtained via location-sensitive electrical transport measurements. The sum rule holds in the conversion coefficient in the current-voltage characteristics. A diamagnetic nature of the crystals supports that the spin polarization is not due to localized electron spins but due to itinerant electron spins. A large difference in the strength of antisymmetric spin-orbit interaction associated with 4d electrons in Nb and 5d ones in Ta is oppositely correlated with that of the spin polarization. A robust protection of the spin polarization occurs over long distances in chiral crystals.

Chirality-Induced Spin-Polarized State of a Chiral Crystal CrNb_{3}S_{6}.

Chirality-induced spin transport phenomena are investigated at room temperature without magnetic fields in a monoaxial chiral dichalcogenide CrNb_{3}S_{6}. We found that spin polarization occurs in these chiral bulk crystals under a charge current flowing along the principal c axis. Such phenomena are detected as an inverse spin Hall signal which is induced on the detection electrode that absorbs polarized spin from the chiral crystal. The inverse response is observed when applying the charge current into the detection electrode. The signal sign reverses in the device with the opposite chirality. Furthermore, the spin signals are found over micrometer length scales in a nonlocal configuration. Such a robust generation and protection of the spin-polarized state is discussed based on a one-dimensional model with an antisymmetric spin-orbit coupling.

Spin-Wave Chirality and Its Manifestations in Antiferromagnets.

As first demonstrated by Tang and Cohen in chiral optics, the asymmetry in the rate of electromagnetic energy absorption between left and right enantiomers is determined by an optical chirality density. Here, we demonstrate that this effect can exist in magnetic spin systems. By constructing a formal analogy with electrodynamics, we show that in antiferromagnets with broken chiral symmetry, the asymmetry in local spin-wave energy absorption is proportional to a spin-wave chirality density, which is a direct counterpart of optical zilch. We propose that injection of a pure spin current into an antiferromagnet may serve as a chiral symmetry breaking mechanism, since its effect in the spin-wave approximation can be expressed in terms of additional Lifshitz invariants. We use linear response theory to show that the spin current induces a nonequilibrium spin-wave chirality density.

The effect of doping a molecular spin ladder with non-magnetic impurities.

Since carrier doping of two-leg spin ladders can theoretically induce a superconductive state, investigation of such systems is of great use in the study of superconductivity. In this paper, we report the successful creation of a non-magnetic impurity doped into a two-leg molecular spin ladder and the characterization of its magnetic properties.

Tuning magnetotransport through a magnetic kink crystal in a chiral helimagnet.

We consider magnetotransport properties in a conducting chiral helimagnet, where the magnetic kink crystal (MKC) is formed under weak magnetic field applied perpendicular to the helical axis. The MKC behaves as a magnetic superlattice potential and results in Bragg scattering of conduction electrons. Tuning of the weak magnetic field enables us to control the size of the superlattice Brillouin zone and gives rise to a series of divergent resistivity anomalies originating from resonant Bragg scatterings. We discuss as well a nontrivial magnetic structure in the resonant states realized in the subsystem of the itinerant electrons.