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1.
Nat Commun ; 14(1): 5117, 2023 Aug 23.
Artigo em Inglês | MEDLINE | ID: mdl-37612287

RESUMO

Understanding how 1.5 °C pathways could adjust in light of new adverse information, such as a reduced 1.5 °C carbon budget, or slower-than-expected low-carbon technology deployment, is critical for planning resilient pathways. We use an integrated assessment model to explore potential pathway adjustments starting in 2025 and 2030, following the arrival of new information. The 1.5 °C target remains achievable in the model, in light of some adverse information, provided a broad portfolio of technologies and measures is still available. If multiple pieces of adverse information arrive simultaneously, average annual emissions reductions near 3 GtCO2/yr for the first five years following the pathway adjustment, compared to 2 GtCO2/yr in 2020 when the Covid-19 pandemic began. Moreover, in these scenarios of multiple simultaneous adverse information, by 2050 mitigation costs are 4-5 times as high as a no adverse information scenario, highlighting the criticality of developing a wide range of mitigation options, including energy demand reduction options.

2.
Science ; 380(6649): 1014-1016, 2023 06 09.
Artigo em Inglês | MEDLINE | ID: mdl-37289874

RESUMO

Looking at policies instead of promises shows that global climate targets may be missed by a large margin.


Assuntos
Mudança Climática , Clima , Política Ambiental
3.
Nat Commun ; 13(1): 4304, 2022 08 16.
Artigo em Inglês | MEDLINE | ID: mdl-35973995

RESUMO

Scientifically rigorous guidance to policy makers on mitigation options for meeting the Paris Agreement long-term temperature goal requires an evaluation of long-term global-warming implications of greenhouse gas emissions pathways. Here we employ a uniform and transparent methodology to evaluate Paris Agreement compatibility of influential institutional emission scenarios from the grey literature, including those from Shell, BP, and the International Energy Agency. We compare a selection of these scenarios analysed with this methodology to the Integrated Assessment Model scenarios assessed by the Intergovernmental Panel on Climate Change. We harmonize emissions to a consistent base-year and account for all greenhouse gases and aerosol precursor emissions, ensuring a self-consistent comparison of climate variables. An evaluation of peak and end-of-century temperatures is made, with both being relevant to the Paris Agreement goal. Of the scenarios assessed, we find that only the IEA Net Zero 2050 scenario is aligned with the criteria for Paris Agreement consistency employed here. We investigate root causes for misalignment with these criteria based on the underlying energy system transformation.


Assuntos
Objetivos , Gases de Efeito Estufa , Mudança Climática , Aquecimento Global/prevenção & controle , Temperatura
4.
Geophys Res Lett ; 48(8): e2020GL091883, 2021 Apr 28.
Artigo em Inglês | MEDLINE | ID: mdl-34149115

RESUMO

Many nations responded to the corona virus disease-2019 (COVID-19) pandemic by restricting travel and other activities during 2020, resulting in temporarily reduced emissions of CO2, other greenhouse gases and ozone and aerosol precursors. We present the initial results from a coordinated Intercomparison, CovidMIP, of Earth system model simulations which assess the impact on climate of these emissions reductions. 12 models performed multiple initial-condition ensembles to produce over 300 simulations spanning both initial condition and model structural uncertainty. We find model consensus on reduced aerosol amounts (particularly over southern and eastern Asia) and associated increases in surface shortwave radiation levels. However, any impact on near-surface temperature or rainfall during 2020-2024 is extremely small and is not detectable in this initial analysis. Regional analyses on a finer scale, and closer attention to extremes (especially linked to changes in atmospheric composition and air quality) are required to test the impact of COVID-19-related emission reductions on near-term climate.

6.
J Phys Chem C Nanomater Interfaces ; 121(7): 3790-3796, 2017 Feb 23.
Artigo em Inglês | MEDLINE | ID: mdl-28316756

RESUMO

Cesium lead halide nanocrystals, CsPbX3 (X = Cl, Br, I), exhibit photoluminescence quantum efficiencies approaching 100% without the core-shell structures usually used in conventional semiconductor nanocrystals. These high photoluminescence efficiencies make these crystals ideal candidates for light-emitting diodes (LEDs). However, because of the large surface area to volume ratio, halogen exchange between perovskite nanocrystals of different compositions occurs rapidly, which is one of the limiting factors for white-light applications requiring a mixture of different crystal compositions to achieve a broad emission spectrum. Here, we use mixtures of chloride and iodide CsPbX3 (X = Cl, I) perovskite nanocrystals where anion exchange is significantly reduced. We investigate samples containing mixtures of perovskite nanocrystals with different compositions and study the resulting optical and electrical interactions. We report excitation transfer from CsPbCl3 to CsPbI3 in solution and within a poly(methyl methacrylate) matrix via photon reabsorption, which also occurs in electrically excited crystals in bulk heterojunction LEDs.

7.
Analyst ; 140(14): 4882-6, 2015 Jul 21.
Artigo em Inglês | MEDLINE | ID: mdl-25994201

RESUMO

The measurement of single particle size distributions of amyloid fibrils is crucial for determining mechanisms of growth and toxicity. Nanopore sensing is an attractive solution for this problem since it gives information on aggregates' shapes with relatively high throughput for a single particle technology. In this paper we study the translocation of lysozyme fibrils through quartz glass nanopores. We demonstrate that, under appropriate salt and pH conditions, lysozyme fibrils translocate through bare quartz nanopores without causing significant clogging. This enables us to measure statistics on tens of thousands of translocations of lysozyme fibrils with the same nanopore and track their development over a time course of aggregation spanning 24 h. Analysis of our events shows that the statistics are consistent with a simple bulk conductivity model for the passage of rods with a fixed cross sectional area through a conical glass nanopore.


Assuntos
Amiloide/química , Muramidase/química , Nanoporos
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