Dual-comb absorption spectroscopy of molecular CeO in a laser-produced plasma.

Broadband and high-resolution absorption spectra of molecular cerium oxide (CeO) are obtained in a laser-produced plasma using dual-comb spectroscopy. Simultaneous measurements of Ce and CeO are used to probe time-resolved dynamics of the system. A spectral resolution of 1.24 GHz (2.4 pm) over a bandwidth of 378.7-383.7 THz (781.1-791.5 nm) allows simultaneous detection of hundreds of closely spaced rotational transitions in complex CeO bands.

Burst-mode dual-comb spectroscopy.

We introduce a new, to the best of our knowledge, modality of dual-comb spectroscopy (DCS) that enables a simplified and powerful new approach for time-resolved measurements with increased acquisition rates. This "burst mode" form of DCS relies on the multiplexing of each probe pulse into a short train of pulses. With this approach we demonstrate a time-resolved series of absorption-based spectroscopic measurements of a laser-induced plasma using only a single laser ablation shot and identify 22 Nd lines not previously reported in the literature. The transmission spectra spanned 3.1 THz and were acquired at an effective acquisition rate of 25 kHz with 40 µs time resolution. This simple modification to ∼100MHz level dual-comb systems provides a flexible approach for studying transient and low-duty-cycle events such as laser-induced plasmas, combustion, and explosive reactions.

Time-resolved dual-comb measurement of number density and temperature in a laser-induced plasma.

We utilize time-resolved dual-comb spectroscopy to measure the temporal evolution of the population number densities and absorption excitation temperature of Fe in a laser-induced plasma. The spectra of three excited-state transitions of Fe around 533 nm are simultaneously measured at different time delays following laser ablation of a stainless steel sample. This Letter probes late-time behaviors of laser-induced ablation plumes during plasma cooling. The high spectral resolution and broad spectral coverage of the dual-comb technique, combined with the time-resolved measurement capability shown here, will aid in the characterization of laser induced plasmas, including species identification and molecule and particle formation that can occur at later times in the plasma evolution.

Multi-gigahertz repetition-rate-selectable passive harmonic mode locking of a fiber laser.

We demonstrate a passive harmonically mode-locked erbium-doped fiber laser that operates at selectable harmonics spanning from the 6th to the 928th, which corresponds to repetition rates ranging from 153 MHz to 22.2 GHz. The noteworthy laser output stability is attested by supermode suppression levels as large as 41 dB. The influence of a continuous wave background on harmonics stability is tested.

66 W average power from a microjoule-class sub-100 fs fiber oscillator.

Performance scaling of passively mode-locked ultrashort-pulse fiber oscillators in terms of average power, peak power, and pulse energy is demonstrated. A very-large-mode-area fiber laser in an all-positive group-velocity-dispersion ring cavity configuration with intracavity spectral filter, mode-locked by nonlinear polarization evolution, emits 66 W of average power at 76 MHz repetition rate, corresponding to 0.9 µJ pulse energy. The pulses are dechirped to 91 fs outside the cavity with an average power of 60 W remaining after the compressor. The generated pulse peak power is as high as 7 MW.

High-energy femtosecond photonic crystal fiber laser.

We report the generation of high-energy high-peak power pulses in an all-normal dispersion fiber laser featuring large-mode-area photonic crystal fibers. The self-starting chirped-pulse fiber oscillator delivers 11 W of average power at 15.5 MHz repetition rate, resulting in 710 nJ of pulse energy. The output pulses are dechirped outside the cavity from 7 ps to nearly transform-limited duration of 300 fs, leading to pulse peak powers as high as 1.9 MW. Numerical simulations reveal that pulse shaping is dominated by the amplitude modulation and spectral filtering provided by a resonant semiconductor saturable absorber.

Sub-80 fs dissipative soliton large-mode-area fiber laser.

We report on high-energy ultrashort pulse generation from an all-normal-dispersion large-mode-area fiber laser by exploiting an efficient combination of nonlinear polarization evolution (NPE) and a semiconductor-based saturable absorber mode-locking mechanism. The watt-level laser directly emits chirped pulses with a duration of 1 ps and 163 nJ of pulse energy. These can be compressed to 77 fs, generating megawatt-level peak power. Intracavity dynamics are discussed by numerical simulation, and the intracavity pulse evolution reveals that NPE plays a key role in pulse shaping.

High-energy femtosecond pulses from a dissipative soliton fiber laser.

We report the generation of sub-150 fs pulses from a passively mode-locked laser featuring a large-mode-area microstructure fiber. Reliable self-starting mode-locking is achieved using a fast semiconductor saturable absorber mirror. The laser generates 63 nJ chirped pulses at 22 MHz repetition rate for an average power of 1.4 W. The 2.2 ps output pulses are compressed outside the cavity to 150 fs.

Mode-locked Yb-doped Bragg fiber laser.

We report on a mode-locked fiber laser featuring an Yb-doped large-mode-area Bragg fiber and exploiting dissipative-soliton pulse shaping. Reliable self-starting mode-locking is achieved using a fast semiconductor saturable absorber mirror. The laser generates 30 nJ chirped pulses at 17 MHz repetition rate for an average power of 510 mW. The 3.2 ps output pulses are compressed outside the cavity to 440 fs.

High-power all-normal-dispersion femtosecond pulse generation from a Yb-doped large-mode-area microstructure fiber laser.

We report on an all-normal-dispersion mode-locked fiber laser based on a large-mode-area Yb-doped microstructure fiber and using a high nonlinear modulation depth semiconductor saturable absorber mirror. The laser delivers 3.3 W of average output power with positively chirped 5.5 ps pulses at a center wavelength of 1033 nm. The pulse repetition rate is 46.4 MHz, which results in an energy per pulse of 71 nJ. These pulses are extracavity dechirped down to 516 fs by using bulk gratings. The average power of the dechirped pulses is 2.3 W, which corresponds to a peak power of more than 96 kW.