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The assessment of microplastic (MP) pollution in urban areas is essential considering its abundance in freshwater, particularly due to urban wet weather discharge. The precise sources of MPs must be identified to better understand its characteristics. This study examines the relationship between MP pollution in detention basin sediments and land use in the investigated catchments. The study of stormwater management infrastructure, mainly in detention basins, has enabled the quantification of MP abundance in sediments conveyed by stormwater in urban areas. Sediment sampling was conducted in ten detention basins and one combined sewer overflow (CSO) structure in the Lyon metropolitan area, France. These basins correspond to stormwater outlets of representative urban catchment areas. MP extraction involves densimetric separation and organic matter degradation. MPs were then characterized using micro-Fourier infrared spectroscopy and siMPle software. This protocol identified MPs between 50 and 500 µm in the study sites. This study highlights the high abundance in the collected sediment samples, ranging from 2,525 to 1,218,82 MP kg-1 by dry weight sediment. The MPs found have a median size around 115 µm, making them very small MPs that are mainly composed of polypropylene followed by polyethylene and polystyrene or polyethylene terephthalate. The abundance of MPs in sediments is associated with the land use type. Catchments in predominantly industrial and commercial zones were more significantly polluted with MPs compared with those in predominantly agricultural or heterogeneous zones. Finally, statistical analyses revealed links between sedimentary and urban parameters and MPs concentrations. Several recommendations are given for future research, notably concerning the analyzing of stormwater sediments to understand the sources of MP pollution.
Assuntos
Microplásticos , Poluentes Químicos da Água , Microplásticos/análise , Plásticos/análise , Sedimentos Geológicos/química , Poluentes Químicos da Água/análise , Monitoramento Ambiental/métodosRESUMO
Crude oil leakages and spills (OLS) are some of the problems attributed to pipeline failures in the oil and gas industry's midstream sector. Consequently, they are monitored via several leakage detection and localisation techniques (LDTs) comprising classical methods and, recently, Internet of Things (IoT)-based systems via wireless sensor networks (WSNs). Although the latter techniques are proven to be more efficient, they are susceptible to other types of failures such as high false alarms or single point of failure (SPOF) due to their centralised implementations. Therefore, in this work, we present a hybrid distributed leakage detection and localisation technique (HyDiLLEch), which combines multiple classical LDTs. The technique is implemented in two versions, a single-hop and a double-hop version. The evaluation of the results is based on the resilience to SPOFs, the accuracy of detection and localisation, and communication efficiency. The results obtained from the placement strategy and the distributed spatial data correlation include increased sensitivity to leakage detection and localisation and the elimination of the SPOF related to the centralised LDTs by increasing the number of node-detecting and localising (NDL) leakages to four and six in the single-hop and double-hop versions, respectively. In addition, the accuracy of leakages is improved from 0 to 32 m in nodes that were physically close to the leakage points while keeping the communication overhead minimal.
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Elevated trace metal concentrations in sediments pose a major problem for the management of stormwater detention basins. These basins provide a nature-based solution to remove particulate pollutants through settling, but the resuspension of these contaminated deposits may impact the quality of both surface and groundwater. A better understanding of trace metal distribution will help to improve basin design and sediment management. This study aims to predict the distribution of trace metal contamination in a stormwater detention basin through (i) investigation of the correlation between metal content in sediments and their settling velocity, and (ii) the coupling of such correlation with a Lagrangian Discrete Phase Model (LDPM). The correlation between Fe, Cr, Cu, Ni, Pb contents and the settling velocity is firstly investigated, based on the sediments collected from 6 sites (inlet and 5 traps at the bottom of a detention basin situated in Chassieu, France) during 5 campaigns in 2017. Results show that Fe is strongly correlated to settling velocity and can be considered as a good indicator of trace metal contents. The derived correlation is then combined with a LDPM for the prediction of trace metal distribution, producing results consistent with in situ measurements. The proposed methodology can be applied for other stormwater basins (dry or wet). As described in this article, the interactions between hydrodynamics and sediment physico-chemical characteristics is crucial for the design and management of stormwater detention basins, allowing managers to target the highest contaminated sediments.
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In the past ten years, governments from the European Union have been encouraged to collect volume and quality data for all the effluent overflows from separated stormwater and combined sewer systems that result in a significant environmental impact on receiving water bodies. Methods to monitor and control these flows require improvements, particularly for complex Combined Sewer Overflow (CSO) structures. The DSM-flux (Device for Stormwater and combined sewer flows Monitoring and the control of pollutant fluxes) is a new pre-designed and pre-calibrated channel that provides appropriate hydraulic conditions suitable for measurement of overflow rates and volumes by means of one water level gauge. In this paper, a stage-discharge relation for the DSM-flux is obtained experimentally and validated for multiple inflow hydraulic configurations. Uncertainties in CSO discharges and volumes are estimated within the Guide to the expression of Uncertainty in Measurement (GUM) framework. Whatever the upstream hydraulic conditions are, relative uncertainties are lower than 15% and 2% for the investigated discharges and volumes, respectively.
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Cidades , Incerteza , Movimentos da Água , Monitoramento Ambiental , Chuva , EsgotosRESUMO
To characterize the spatio-temporal variation of sediment ecotoxicity in a retention/detention basin, a monitoring program using the Heterocypris incongruens bioassay was carried out for 72 months (5 years) on a field basin close to Lyon in France. Results showed that the variation of ecotoxicity is relatively small from one location of the basin to another, apart from sediment sampling collected in an open-air chamber located in basin supposed to collect gross pollutants and hydrocarbons. Regarding the temporal variation of ecotoxicity, the bioassays also showed a slight variation between 6 and 72 months. On the contrary, they highlighted the high ecotoxicity of the "fresh" sediments collected during rain events using sediment traps. Additional investigations are needed to understand the period of inflexion of ecotoxicity, occurring between 24 h and 6 months. These results can be used by practitioners of urban facilities and networks to improve maintenance strategies of retention/detention basins.
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Sedimentos Geológicos/química , Poluentes Químicos da Água/análise , Aliivibrio fischeri/efeitos dos fármacos , Aliivibrio fischeri/metabolismo , Animais , Bioensaio , Crustáceos/efeitos dos fármacos , Crustáceos/metabolismo , Ecotoxicologia , Monitoramento Ambiental , França , Hidrocarbonetos/análise , Chuva/químicaRESUMO
Urban activities generate surface deposits over impervious surfaces that can represent ecological and health hazards. Bacteriome genetic structures of deposits washed off during rainfall events, over an urban industrial watershed, were inferred from 16 S rRNA gene (rrs) sequences generated by high throughput sequencing. Deposits were sampled over a 4 year-period from a detention basin (DB). Major shifts, matching key management practices, in the structure of these urban bacteriomes, were recorded. Correlation analyses of rrs similarities between samples and their respective concentrations in chemical pollutants, markers of human fecal contaminations (HF183) and antimicrobial resistances (integrons), were performed. Harsher environmental constraints building up in the older deposits led to an increase number of rrs reads from extremophiles such as Acidibacter and Haliangium. Deposits accumulating in the decantation pit of the DB showed an increase in rrs reads from warm blooded intestinal tract bacteria such as Bacteroides and Prevotella. This enrichment matched higher concentrations of Bacteroides HF183 genotypes normally restricted to humans. Bacteriomes of urban deposits appeared good indicators of human-driven environmental changes. Their composition was found representative of their origin. Soil particles and rain appeared to be major contributors of the inferred bacterial taxa recovered from recent deposits.
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Bactérias/genética , Microbiologia da Água , Poluentes Químicos da Água/toxicidade , Poluição da Água , Bactérias/classificação , Bactérias/isolamento & purificação , Bacteroides/genética , Cidades , Monitoramento Ambiental , Prevotella/genética , RNA Bacteriano , RNA Ribossômico 16S , Reação em Cadeia da Polimerase em Tempo Real , Análise de Sequência de RNA , Microbiologia do Solo , Propriedades de Superfície , Movimentos da ÁguaRESUMO
H2S emission dynamics in sewers are conditioned by the mass transfer coefficient at the interface. This work aims at measuring the variation of the mass transfer coefficient with the hydraulic characteristics, with the objective of estimating H2S emission in gravity pipes, and collecting data to establish models independent of the system geometry. The ratio between the H2S and O2 mass transfer coefficient was assessed in an 8 L mixed reactor under different experimental conditions. Then, oxygen mass transfer measurements were performed in a 10 m long gravity pipe. The following ranges of experimental conditions were investigated: velocity flow [0-0.61 m.s-1], Reynolds number [0-23,333]. The hydrodynamic parameters at the liquid/gas interface were calculated by computational fluid dynamics (CFD). In the laboratory-scale reactor, the O2 mass transfer coefficient was found to depend on the stirring rate (rph) as follows: KL,O2 = 0.016 + 0.025 N3.85. A KL,H2S/KL,O2 ratio of 0.64 ± 0.24 was found, in accordance with previously published data. CFD results helped in refining this correlation: the mass transfer coefficient depends on the local interface velocity ui (m.h-1): KL,O2 = 0.016 + 1.02 × 10-5 ui3.85 In the gravity pipe device, KL,O2 also exponentially increased with the mean flow velocity. These trends were found to be consistent with the increasing level of turbulence.
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Esgotos/química , Sulfetos/química , Poluentes Químicos da Água/química , Gases/química , Gravitação , Modelos Teóricos , Transição de FaseRESUMO
Problems related to hydrogen sulfide may be serious for both network stakeholders and the public in terms of health, sustainability of the sewer structure and urban comfort. H2S emission models are generally theoretical and simplified in terms of environmental conditions. Although air transport characteristics in sewers must play a role in the fate of hydrogen sulfide, only a limited number of studies have investigated this issue. The aim of this study was to better understand H2S liquid to gas transfer by highlighting the link between the mass transfer coefficient and the turbulence in the air flow and the water flow. For experimental safety reasons, O2 was taken as a model compound. The oxygen mass transfer coefficients were obtained using a mass balance in plug flow. The mass transfer coefficient was not impacted by the range of the interface air-flow velocity values tested (0.55-2.28 m·s-1) or the water velocity values (0.06-0.55 m·s-1). Using the ratio between kL,O2 to kL,H2S, the H2S mass transfer behavior in a gravity pipe in the same hydraulic conditions can be predicted.
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Ar/análise , Oxigênio/química , Esgotos/química , Água/química , Gravitação , Sulfeto de Hidrogênio/química , Modelos Teóricos , Eliminação de Resíduos LíquidosRESUMO
The problems related to hydrogen sulfide in terms of deterioration of sewer networks, toxicity and odor nuisance have become very clear to the network stakeholders and the public. The hydraulic and (bio)chemical phenomena and parameters controlling sulfide formation, emission and their incidences in sewer networks are very complex. Recent research studies have been developed in gravity and pressure sewers and some transfer models have been published. Nevertheless, the models do not take into account all the physical phenomena influencing the emission process. After summing up the main scientific knowledge concerning the production, oxidation, transfer and emission processes, the present review includes: (i) a synthetic analysis of sulfide and hydrogen sulfide emission models in sewer networks, (ii) an estimation of their limit, (iii) perspectives to improve the modelling approach. It shows that sulfide formation and uptake models still need refinements especially for some phenomena such as liquid to gas mass transfer. Transfer models that have been published so far are purposely simplified and valid for simple systems. More efforts have to be undertaken in order to better understand the mechanisms and the dynamics of hydrogen sulfide production and emission in real conditions.
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Poluentes Atmosféricos/química , Modelos Químicos , Engenharia Sanitária , Esgotos/química , Sulfetos/química , Sulfeto de Hidrogênio/química , Odorantes/análise , Oxirredução , Temperatura , Eliminação de Resíduos Líquidos , Águas Residuárias/químicaRESUMO
The present paper aims to identify ways to reduce pollution injected by residents in the urban wastewater network system. Two approaches are considered. The first one uses flow and pollutant calculation to test whether a polluter can easily be identified in a neighborhood. The second approach uses a survey to examine what incentive would be most effective to influence residents' behavior. Hydrodynamic simulation results show that concentration profiles at the network outlet corresponding to all possible polluters are similar and thus do not point out specific resident source of pollution. Household-level survey results show that most socio-economic and public-good-related characteristics do not play a significant role in explaining choices to discard in the home wastewater network. Apart from the nature of the waste itself, by far the belief that the respondent has about neighbors' and relatives' discarding behavior is the main driver of the choice.
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Modelos Teóricos , Controles Informais da Sociedade , Águas Residuárias , Poluentes da Água/análise , Poluição da Água/prevenção & controle , Cidades , Difusão , Drenagem Sanitária , Humanos , Características de Residência , População UrbanaRESUMO
Sedimentation is a common but complex phenomenon in the urban drainage system. The settling mechanisms involved in detention basins are still not well understood. The lack of knowledge on sediment transport and settling processes in actual detention basins is still an obstacle to the optimization of the design and the management of the stormwater detention basins. In order to well understand the sedimentation processes, in this paper, a new boundary condition as an attempt to represent the sedimentation processes based on particle tracking approach is presented. The proposed boundary condition is based on the assumption that the flow turbulent kinetic energy near the bottom plays an important role on the sedimentation processes. The simulated results show that the proposed boundary condition appears as a potential capability to identify the preferential sediment zones and to predict the trapping efficiency of the basin during storm events.