Mid-infrared supercontinuum generation in silicon-germanium all-normal dispersion waveguides.

We demonstrate coherent supercontinuum generation spanning over an octave from a silicon germanium-on-silicon waveguide using ∼200fs pulses at a wavelength of 4 µm. The waveguide is engineered to provide low all-normal dispersion in the TM polarization. We validate the coherence of the generated supercontinuum via simulations, with a high degree of coherence across the entire spectrum. Such a generated supercontinuum could lend itself to pulse compression down to 22 fs.

Nonlinear light generation in topological nanostructures.

Topological photonics has emerged as a route to robust optical circuitry protected against disorder1,2 and now includes demonstrations such as topologically protected lasing3-5 and single-photon transport6. Recently, nonlinear optical topological structures have attracted special theoretical interest7-11, as they enable tuning of topological properties by a change in the light intensity7,12 and can break optical reciprocity13-15 to realize full topological protection. However, so far, non-reciprocal topological states have only been realized using magneto-optical materials and macroscopic set-ups with external magnets4,16, which is not feasible for nanoscale integration. Here we report the observation of a third-harmonic signal from a topologically non-trivial zigzag array of dielectric nanoparticles and the demonstration of strong enhancement of the nonlinear photon generation at the edge states of the array. The signal enhancement is due to the interaction between the Mie resonances of silicon nanoparticles and the topological localization of the electric field at the edges. The system is also robust against various perturbations and structural defects. Moreover, we show that the interplay between topology, bi-anisotropy and nonlinearity makes parametric photon generation tunable and non-reciprocal. Our study brings nonlinear topological photonics concepts to the realm of nanoscience.

Nonlinear Wavefront Control with All-Dielectric Metasurfaces.

Metasurfaces, two-dimensional lattices of nanoscale resonators, offer unique opportunities for functional flat optics and allow the control of the transmission, reflection, and polarization of a wavefront of light. Recently, all-dielectric metasurfaces reached remarkable efficiencies, often matching or out-performing conventional optical elements. The exploitation of the nonlinear optical response of metasurfaces offers a paradigm shift in nonlinear optics, and dielectric nonlinear metasurfaces are expected to enrich subwavelength photonics by enhancing substantially nonlinear response of natural materials combined with the efficient control of the phase of nonlinear waves. Here, we suggest a novel and rather general approach for engineering the wavefront of parametric waves of arbitrary complexity generated by a nonlinear metasurface. We design all-dielectric nonlinear metasurfaces, achieve a highly efficient wavefront control of a third-harmonic field, and demonstrate the generation of nonlinear beams at a designed angle and the generation of nonlinear focusing vortex beams. Our nonlinear metasurfaces produce phase gradients over a full 0-2π phase range with a 92% diffraction efficiency.

High-resolution chalcogenide fiber bundles for longwave infrared imaging.

A flexible chalcogenide fiber bundle (FB) with a resolution as high as ~31 lp/mm has been fabricated for delivering thermal images of objects at room temperature. The FB is composed of ~200,000 single fibers with a Ge-As-Te-Se glass core 15 µm in diameter and a polyetherimide (PEI) cladding 16.8 µm in diameter. These Ge-As-Te-Se/PEI fibers show good transparency in the 3-12 µm spectral region. The fabricated FB presents a filling factor of ~72% and a crosstalk of ~1%. High-quality thermal images of a human hand were obtained through the FB, demonstrating good potential of the FB for longwave infrared imaging in the areas such as medicine, industry and defense.

CMOS compatible fabrication of micro, nano convex silicon lens arrays by conformal chemical vapor deposition.

We present a novel CMOS-compatible fabrication technique for convex micro-nano lens arrays (MNLAs) with high packing density on the wafer scale. By means of conformal chemical vapor deposition (CVD) of hydrogenated amorphous silicon (a-Si:H) following patterning of silicon pillars via electron beam lithography (EBL) and plasma etching, large areas of a close packed silicon lens array with the diameter from a few micrometers down to a few hundred nanometers was fabricated. The resulting structure shows excellent surface roughness and high uniformity. The optical focusing properties of the lenses at infrared wavelengths were verified by experimental measurements and numerical simulation. This approach provides a feasible solution for fabricating silicon MNLAs compatible for next generation large scale, miniaturized optical imaging detectors and related optical devices.

Experimental demonstration of linearly polarized 2-10 µm supercontinuum generation in a chalcogenide rib waveguide.

This Letter reports the production of a supercontinuum extending from ≈2 µm to >10 µm generated using a chalcogenide buried rib waveguide pumped with 330 femtosecond pulses at 4.184 µm. This is, to the best of our knowledge, the broadest mid-infrared supercontinuum generated in any planar waveguide platform. Because the waveguide is birefringent, quasi-single-mode, and uses an optimized dispersion design, the supercontinuum is linearly polarized with an extinction ratio >100. Dual beam spectrophotometry is performed easily using this source.

Tailoring of the Brillouin gain for on-chip widely tunable and reconfigurable broadband microwave photonic filters.

An unprecedented Brillouin gain of 44 dB in a photonic chip enables the realization of broadly tunable and reconfigurable integrated microwave photonic filters. More than a decade bandwidth reconfigurability from 30 up to 440 MHz, with a passband ripple <1.9 dB is achieved by tailoring the Brillouin pump. The filter central frequency is continuously tuned up to 30 GHz with no degradation of the passband response, which is a major improvement over electronic filters. Furthermore, we demonstrate pump tailoring to realize multiple bandpass filters with different bandwidths and central frequencies, paving the way for multiple on-chip microwave filters and channelizers.

Producing air-stable monolayers of phosphorene and their defect engineering.

It has been a long-standing challenge to produce air-stable few- or monolayer samples of phosphorene because thin phosphorene films degrade rapidly in ambient conditions. Here we demonstrate a new highly controllable method for fabricating high quality, air-stable phosphorene films with a designated number of layers ranging from a few down to monolayer. Our approach involves the use of oxygen plasma dry etching to thin down thick-exfoliated phosphorene flakes, layer by layer with atomic precision. Moreover, in a stabilized phosphorene monolayer, we were able to precisely engineer defects for the first time, which led to efficient emission of photons at new frequencies in the near infrared at room temperature. In addition, we demonstrate the use of an electrostatic gate to tune the photon emission from the defects in a monolayer phosphorene. This could lead to new electronic and optoelectronic devices, such as electrically tunable, broadband near infrared lighting devices operating at room temperature.

Atomically thin optical lenses and gratings.

Two-dimensional (2D) materials have emerged as promising candidates for miniaturized optoelectronic devices due to their strong inelastic interactions with light. On the other hand, a miniaturized optical system also requires strong elastic light-matter interactions to control the flow of light. Here we report that a single-layer molybdenum disulfide (MoS2) has a giant optical path length (OPL), around one order of magnitude larger than that from a single-layer of graphene. Using such giant OPL to engineer the phase front of optical beams we have demonstrated, to the best of our knowledge, the world's thinnest optical lens consisting of a few layers of MoS2 less than 6.3 nm thick. By taking advantage of the giant elastic scattering efficiency in ultra-thin high-index 2D materials, we also demonstrated high-efficiency gratings based on a single- or few-layers of MoS2. The capability of manipulating the flow of light in 2D materials opens an exciting avenue towards unprecedented miniaturization of optical components and the integration of advanced optical functionalities. More importantly, the unique and large tunability of the refractive index by electric field in layered MoS2 will enable various applications in electrically tunable atomically thin optical components, such as micro-lenses with electrically tunable focal lengths, electrical tunable phase shifters with ultra-high accuracy, which cannot be realized by conventional bulk solids.

High-resolution chalcogenide fiber bundles for infrared imaging.

An ordered chalcogenide fiber bundle with a high resolution for infrared imaging was fabricated using a stack-and-draw approach. The fiber bundle consisted of about 810,000 single fibers with an As2S3 glass core of 9 µm in diameter and a polyetherimide (PEI) polymer cladding of 10 µm in diameter. The As2S3/PEI fibers showed good transparency in the 1.5-6.5 µm spectral region. It presented a resolution of ∼45 lp/mm and a crosstalk of ∼2.5%. Fine thermal images of a hot soldering iron tip were delivered through the fiber bundle.

High Q factor chalcogenide ring resonators for cavity-enhanced MIR spectroscopic sensing.

We report the characteristics of high Q factor chalcogenide ring resonators designed for sensing in the mid-infrared (MIR). The resonators consisted of an exposed Ge11.5As24Se64.5 core on a Ge11.5As24S64.5 bottom cladding and were fabricated in the racetrack coupled ring structure. Loaded Q factors at 5.2µm up to 58,000were obtained, corresponding to an intrinsic Q of 145,000 and a waveguide propagation loss of 0.84dB/cm.

Nonlinear diffraction in orientation-patterned semiconductors.

This work represents experimental demonstration of nonlinear diffraction in an orientation-patterned semiconducting material. By employing a new transverse geometry of interaction, three types of second-order nonlinear diffraction have been identified according to different configurations of quasi-phase matching conditions. Specifically, nonlinear Cerenkov diffraction is defined by the longitudinal quasi-phase matching condition, nonlinear Raman-Nath diffraction satisfies only the transverse quasi-phase matching condition, and nonlinear Bragg diffraction fulfils the full vectorial quasi-phase matching conditions. The study extends the concept of transverse nonlinear parametric interaction toward infrared frequency conversion in semiconductors. It also offers an effective nondestructive method to visualise and diagnose variations of second-order nonlinear coefficients inside semiconductors.

Positive and negative phototunability of chalcogenide (AMTIR-1) microdisk resonator.

We demonstrate externally photo-induced partially-reversible tuning of the resonance of a microdisk made of AMTIR-1 (Ge(33)As(12)Se(55)). We have achieved for the first time, to the best of our knowledge, both positive and negative shift in a microresonator with external tuning. A positive resonance shift of 1 nm and a negative resonance shift of 0.5 nm on a single microdisk has been measured. We have found that this phenomenon is due to initial photo-expansion of the microdisk followed by the photo-bleaching of the AMTIR-1. The observed shifts and the underlying phenomenon is controllable by varying the illumination power (i.e. the low power illumination suppresses the photobleaching process). We measure a loaded quality factor of 1.2x10(5) at 1550nm (limited by the measuring instrument). This holds promise for non-contact low power reversible-tunning of photonic circuit elements.

Multi-milliwatt mid-infrared supercontinuum generation in a suspended core chalcogenide fiber.

A low-loss suspended core As(38)Se(62) fiber with core diameter of 4.5 µm and a zero-dispersion wavelength of 3.5 µm was used for mid-infrared supercontinuum generation. The dispersion of the fiber was measured from 2.9 to 4.2 µm and was in good correspondence with the calculated dispersion. An optical parametric amplifier delivering 320 fs pulses with a peak power of 14.8 kW at a repetition rate of 21 MHz was used to pump 18 cm of suspended core fiber at different wavelengths from 3.3 to 4.7 µm. By pumping at 4.4 µm with a peak power of 5.2 kW coupled to the fiber a supercontinuum spanning from 1.7 to 7.5 µm with an average output power of 15.6 mW and an average power >5.0 µm of 4.7 mW was obtained.

Enhancing and inhibiting stimulated Brillouin scattering in photonic integrated circuits.

On-chip nonlinear optics is a thriving research field, which creates transformative opportunities for manipulating classical or quantum signals in small-footprint integrated devices. Since the length scales are short, nonlinear interactions need to be enhanced by exploiting materials with large nonlinearity in combination with high-Q resonators or slow-light structures. This, however, often results in simultaneous enhancement of competing nonlinear processes, which limit the efficiency and can cause signal distortion. Here, we exploit the frequency dependence of the optical density-of-states near the edge of a photonic bandgap to selectively enhance or inhibit nonlinear interactions on a chip. We demonstrate this concept for one of the strongest nonlinear effects, stimulated Brillouin scattering using a narrow-band one-dimensional photonic bandgap structure: a Bragg grating. The stimulated Brillouin scattering enhancement enables the generation of a 15-line Brillouin frequency comb. In the inhibition case, we achieve stimulated Brillouin scattering free operation at a power level twice the threshold.

1.8-10 µm mid-infrared supercontinuum generated in a step-index chalcogenide fiber using low peak pump power.

By pumping an 11-cm-long step-index chalcogenide fiber with ∼330 fs pulses at 4.0 µm from an optical parametric amplifier, mid-infrared supercontinuum generation spanning from ∼1.8 to ∼10 µm within a dynamic range of ±15 dB has been demonstrated at a relatively low power threshold of ∼3000 W.

Tunable wideband microwave photonic phase shifter using on-chip stimulated Brillouin scattering.

We present the first microwave photonic phase shifter using stimulated Brillouin scattering (SBS) on-chip. The unique ability of SBS to generate both narrowband gain and loss resonances allows us to achieve low ±1.5 dB amplitude fluctuations, which is a record for integrated devices, along with 240° continuously tunable phase shift. Contrary to previous SBS-based approaches, the phase shift tuning mechanism relies on tuning the power, not the frequency, of two SBS pumps, making it more suited to on-chip implementations. We finally demonstrate that SBS pump depletion leads to amplitude response fluctuations, as well as increasing the insertion loss of the phase shifter. Advantageously, shorter integrated platforms possess higher pump depletion thresholds compared to long fibers, thus offering greater potential for reducing the insertion loss.

Negligible nonlinear absorption in hydrogenated amorphous silicon at 1.55 µm for ultra-fast nonlinear signal processing.

Three-photon absorption (3PA) has been observed as the dominant mechanism for nonlinear absorption in wide-bandgap hydrogenated amorphous silicon (a-Si:H-W) at 1.55 µm. The nonlinear index n2 and 3PA coefficient were measured to be 22 × 10(-17)m(2)/W and 5.0 × 10(-26) m(3)/W(2) respectively at 1.55 µm by using the z-scan method. This indicates that the figure of merit (FOM) of this material is intensity dependent. A value FOM>60 is predicted at intensities below 0.5 GW/cm(2) which is the maximum practical intensity for high-bit-rate (>160 GB/s) alloptical signal processing. The nonlinear phase change in a-Si:H-W has been compared with other common nonlinear materials (c-Si, As(2)S(3), Ge(11.5)As(24)Se(64.5)) for a 2 cm long waveguide with a-Si:H-W showing the greatest potential for integrated devices for all-optical processing with a high nonlinear index and negligible nonlinear absorption at intensities < 0.5 GW/cm(2).

Adaptive optics enhanced direct laser writing of high refractive index gyroid photonic crystals in chalcogenide glass.

Chiral gyroid photonic crystals are fabricated in the high refractive index chalcogenide glass arsenic trisulfide with an adaptive optics enhanced direct laser writing system. The severe spherical aberration imparted when focusing into the arsenic trisulfide is mitigated with a defocus decoupled aberration compensation technique that reduces the level of aberration that must be compensated by over an order of magnitude. The fabricated gyroids are shown to have excellent uniformity after our adaptive optics method is employed, and the transmission spectra of the gyroids are shown to have good agreement with numerical simulations that are based on a uniform and diffraction limited fabrication resolution.

Relative contribution of stoichiometry and mean coordination to the fragility of Ge-As-Se glass forming liquids.

The structural relaxation properties of 34 compositions of Ge-As-Se glass forming liquids are investigated by differential scanning calorimetry (DSC). The fragility index (m) and activation energies for enthalpy relaxation (Ea) exhibit universal trends with respect to stoichiometry and mean coordination (⟨r⟩), respectively. The liquid fragility which defines the full temperature dependence of the relaxation processes shows no well defined trend with respect to ⟨r⟩ but instead is found to be closely determined by the excess or deficiency in selenium with respect to stoichiometry. The mean coordination on the other hand appears to be an accurate predictor of the activation energy near the glass transition where most constraints are still intact. No intermediate phase is observed in either case. These results emphasize that chemical effects rather than topological effects appear to control the wide ranging structural mobility of these glass forming liquids. The consequences of these findings in terms of the thermal stability of the corresponding glasses are discussed. It is similarly found that sub-Tg relaxation is controlled by stoichiometry rather than topology.