Ultra-compact synthesis of space-time wave packets.

Space-time wave packets (STWPs) are pulsed fields in which a strictly prescribed association between the spatial and temporal frequencies yields surprising and useful behavior. However, STWPs to date have been synthesized using bulky free-space optical systems that require precise alignment. We describe a compact system that makes use of a novel optical component: a chirped volume Bragg grating that is rotated by 45° with respect to the plane-parallel device facets. By virtue of this grating's unique structure, cascaded gratings resolve and recombine the spectrum without free-space propagation or collimation. We produce STWPs by placing a phase plate that spatially modulates the resolved spectrum between such cascaded gratings, with a device volume of 25 × 25 × 8 mm3, which is orders-of-magnitude smaller than previous arrangements.

Rotated chirped volume Bragg gratings for compact spectral analysis.

We introduce a new, to the best of our knowledge, optical component-a rotated chirped volume Bragg grating (r-CBG)-that spatially resolves the spectrum of a normally incident light beam in a compact footprint and without the need for subsequent free-space propagation or collimation. Unlike conventional chirped volume Bragg gratings in which both the length and width of the device must be increased to increase the bandwidth, by rotating the Bragg structure we sever the link between the length and width of a r-CBG, leading to a significantly reduced device footprint for the same bandwidth. We fabricate and characterize such a device in multiple spectral windows, we study its spectral resolution, and confirm that a pair of cascaded r-CBGs can resolve and then recombine the spectrum. Such a device can lead to ultracompact spectrometers and pulse modulators.

Intracavity spatial mode conversion by holographic phase masks.

Past beam-shaping techniques, developed to transform a Gaussian beam into other waveforms, rely on a wide selection of available tools ranging from physical apertures, diffractive optical elements, phase masks, free-form optics to spatial light modulators. However, these devices - whether active or passive - do not address the underlying monochromatic nature of their embedded phase profiles, while being hampered by the complex, high-cost manufacturing process and a restrictive laser-induced damage threshold. Recently, a new type of passive phase devices for beam transformation - referred to as holographic phase masks (HPMs), was developed to address these critical shortcomings. In this work, we demonstrated the first integration of HPMs into a laser cavity for the generation of arbitrary spatial modes. Our approach allowed for different phase patterns to be embedded into the outputs of a laser system, while preserving the spatial structure of its intracavity beams. The optical system further possessed a unique ability to simultaneously emit distinct spatial modes into separate beampaths, owning to the multiplexing capability of HPMs. We also confirmed the achromatic nature of these HPMs in a wavelength-tunable cavity, contrary to other known passive or active beam-shaping tools. The achromatism of HPMs, coupled to their ability to withstand up to kW level of average power, makes possible future developments in high-power broadband sources, capable of generating light beams with arbitrary phase distribution covering any desirable spectral regions from near ultraviolet to near infrared.

What is the maximum differential group delay achievable by a space-time wave packet in free space?

The group velocity of 'space-time' wave packets - propagation-invariant pulsed beams endowed with tight spatio-temporal spectral correlations - can take on arbitrary values in free space. Here we investigate theoretically and experimentally the maximum achievable group delay that realistic finite-energy space-time wave packets can achieve with respect to a reference pulse traveling at the speed of light. We find that this delay is determined solely by the spectral uncertainty in the association between the spatial frequencies and wavelengths underlying the wave packet spatio-temporal spectrum - and not by the beam size, bandwidth, or pulse width. We show experimentally that the propagation of space-time wave packets is delimited by a spectral-uncertainty-induced 'pilot envelope' that travels at a group velocity equal to the speed of light in vacuum. Temporal walk-off between the space-time wave packet and the pilot envelope limits the maximum achievable differential group delay to the width of the pilot envelope. Within this pilot envelope the space-time wave packet can locally travel at an arbitrary group velocity and yet not violate relativistic causality because the leading or trailing edge of superluminal and subluminal space-time wave packets, respectively, are suppressed once they reach the envelope edge. Using pulses of width ∼ 4 ps and a spectral uncertainty of ∼ 20 pm, we measure maximum differential group delays of approximately ±150 ps, which exceed previously reported measurements by at least three orders of magnitude.

Generation of 1 kHz, 2.3 mJ, 88 fs, 2.5 µm pulses from a Cr2+:ZnSe chirped pulse amplifier.

We demonstrate the generation of 2.3 mJ, 88 fs, 2.5 µm laser pulses at 1 kHz repetition rate from a three-stage chirped pulse amplifier employing Cr2+:ZnSe crystals as the active gain media. 5 µJ seed of the amplifier is obtained via intrapulse difference frequency generation in a bismuth triborate (BIBO) crystal from spectrally broadened Ti:Sapphire amplifier output. A multi-pass amplifier followed by two single-pass amplifiers pumped by Q-switched Ho:YAG lasers boost the pulse energy to 6.5 mJ, yielding 2.3 mJ, 88 fs pulses upon pulse compression. Our results show the highest peak power at 2.5 µm with 1 kHz repetition rate. Such a laser will be a powerful source for studying strong-field physics and extending high-harmonic generation towards the keV region.