Fabrication of freestanding photonic devices combining polymer films with microfabrication techniques and 3D printing.

We report a technological concept for freestanding photonic elements based on metamaterials fabricated on polymer films by clean-room processes and framed using 3D printing. A spin-coated cyclic olefin copolymer (TOPAS) of variable thickness down to one micrometer was used as the substrate onto which metamaterials were fabricated using optical lithography. We demonstrate the possibility of applying a second TOPAS layer to protect the device or to allow for stacking another metamaterial layer. To obtain freestanding elements, frames were 3D printed directly on top of the metamaterial before lift-off from the carrier wafer. This ensured maintaining the flatness of the elements. Both the cleanroom process and the 3D printing enabled the design and manufacturing of elements in different sizes and shapes, e.g., to adapt to specific experimental set-ups and holder geometries or to be compatible with standard optical mounts. While TOPAS is transparent for wavelengths from UV to the far infrared, except for a few infrared absorption lines, we illustrate the concept with the simulation and manufacturing of THz band-pass filters. The performance of the fabricated filters was assessed using THz time-domain spectroscopy. The process is scalable to other wavelength ranges and has the potential for upscaling in manufacturing.

Orbital angular momentum in the near-field of a fork grating.

Light beams with Orbital Angular Momentum (OAM) are explored in applications from microscopy to quantum communication, while the Talbot effect revives in applications from atomic systems to x-ray phase contrast interferometry. We evidence the topological charge of an OAM carrying THz beam in the near-field of a binary amplitude fork-grating by means of the Talbot effect, which we show to persist over several fundamental Talbot lengths. We measure and analyze the evolution of the diffracted beam behind the fork grating in Fourier domain to recover the typical donut-shaped power distribution, and we compare experimental data to simulations. We isolate the inherent phase vortex using the Fourier phase retrieval method. To complement the analysis, we assess the OAM diffraction orders of a fork grating in the far-field using a cylindrical lens.

Retrieving the Talbot length of arbitrary 2D gratings.

The Talbot effect has been revived in many fields of modern optics. As a key number of self-imaging, the fundamental Talbot length plays a crucial role in many applications. However, the inspection of the Talbot carpet for determining the Talbot length is applicable only if the 2D field distribution behind the grating is represented by a 1D cross section. In this Letter, we show an effective way to overcome this limitation to explore the self-imaging of gratings with complex 2D periodicities. For that purpose, the near-field diffraction is analyzed using the Pearson correlation coefficient of the intensity distribution in Fourier space. We report results on linear, ring, and spiral gratings.

Real-Time High Resolution THz Imaging with a Fiber-Coupled Photo Conductive Antenna and an Uncooled Microbolometer Camera.

We present a real-time THz imaging method using a commercial fiber-coupled photo conductive antenna as the THz source and an uncooled microbolometer camera for detection. This new combination of state-of-the-art components is very adaptable due to its compact and uncooled radiation source, whose fiber coupling allows for a flexible placement. Using a camera with high sensitivity renders real-time imaging possible. As a proof-of-concept, the beam shape of a THz Time Domain Spectrometer was measured. We demonstrate real time imaging at nine frames per second and show its potential for practical applications in transmission geometry covering both material science and security tasks. The results suggest that hidden items, complex structures and the moisture content of (biological) materials can be resolved. We discuss the limits of the current setup, possible improvements and potential (industrial) applications, and we outline the feasibility of imaging in reflection geometry or extending it to multi-spectral imaging using band pass filters.

Terahertz Birefringent Biomimetic Aerogels Based on Cellulose Nanofibers and Conductive Nanomaterials.

Biomimetic, lamellar, and highly porous transition-metal carbide (MXene) embedded cellulose nanofiber (CNF) aerogels are assembled by a facile bidirectional freeze-drying approach. The biopolymer aerogels have large-scale, parallel-oriented micrometer-sized pores and show excellent mechanical strength and flexibility, tunable electrical properties, and low densities (2.7-20 mg/cm3). The CNF, MXene, and lamellar pores are efficiently utilized to endow the aerogels with exceptionally high birefringence in the terahertz (THz) regime. Birefringence values as high as 0.09-0.27 at 0.4 THz are achieved, which is comparable to most commercial THz birefringent materials such as liquid crystals, which suffer from fast disintegration, high cost, and complicated preparation processes. Empirical modeling for different MXene contents and an experimental comparison with silver nanowire or carbon nanotube embedded CNF aerogels suggest that the intrinsic conductivity and content of embedded nanomaterials, the aerogel porosity, and the lamellar cell walls can affect the optical properties such as the THz birefringence and absorption. The determination of optical anisotropy in the biopolymer aerogels lays a foundation for further exploration of ultralight, freestanding, and low-cost biomimetic porous architecture-based THz devices.

Terahertz refractive index matching solution.

We report on the fabrication and characterisation of a terahertz (THz) refractive index matching solution (TeraSol) based on barium titanate (BaTiO3) particles and benzocyclobutene (BCB). The high refractive index of BaTiO3 in the THz range makes this material ideal for tuning the effective refractive index of the solution over a wide range. Exploiting the effective medium approximation, we are able to determine the concentration of BaTiO3 particles necessary to obtain target refractive index values between n = 1.8 and n = 5, optimised to match those of substrates widely used in the THz. TeraSol can dramatically reduce the reflections from the substrate during measurements with THz time domain spectroscopy at cryogenic and room temperature. These properties make TeraSol an appealing material for anti-reflective coatings.