RESUMO
The ability to distinguish multiple forms of plutonium from one another, such as oxide and metal, is paramount in areas of nuclear nonproliferation and international safeguards. In its metal form, plutonium can be readily used in a nuclear weapon, while oxide forms are associated with nuclear reactor fuel. Oxide-based plutonium forms emit neutrons with an energy spectrum that is significantly different from the fission neutrons that are emitted from plutonium metal. Organic scintillation detectors output pulses that are proportional to the neutron energy deposited, and therefore present a means of distinguishing these plutonium forms based on their energy spectra. In this work, metal and oxide forms of plutonium were measured using a handheld detection system based on an organic glass scintillator. Monte Carlo modeling of these experiments was performed to provide insight into the origin of the features in the observed light output spectra. Through analysis of multiple regions of these spectra, in a matter of minutes we were able to unambiguously discriminate oxide and metal plutonium forms from one another and from a plutonium-beryllium neutron source, which was considered for comparison because these sources are commonly used in industrial applications. The ability to discriminate weapons-usable material from nuclear reactor fuel has applications in nuclear treaty verification and safeguards.
RESUMO
This Letter details a measurement of the ionization yield (Q(y)) of 6.7 keV(40)Ar atoms stopping in a liquid argon detector. The Q(y) of 3.6-6.3 detected e(-)/keV, for applied electric fields in the range 240-2130 V/cm, is encouraging for the use of this detector medium to search for the signals from hypothetical dark matter particle interactions and from coherent elastic neutrino-nucleus scattering. A significant dependence of Q(y) on the applied electric field is observed and explained in the context of ion recombination.