Toward Fully Multiferroic van der Waals SpinFETs: Basic Design and Quantum Calculations.

Manipulating spin transport enhances the functionality of electronic devices, allowing them to surpass physical constraints related to speed and power. For this reason, the use of van der Waals multiferroics at the interface of heterostructures offers promising prospects for developing high-performance devices, enabling the electrical control of spin information. Our work focuses primarily on a mechanism for multiferroicity in two-dimensional van der Waals materials that stems from an interplay between antiferromagnetism and the breaking of inversion symmetry in certain bilayers. We provide evidence for spin-electrical couplings that include manipulating van der Waals multiferroic edges via external voltages and the subsequent control of spin transport including for fully multiferroic spin field-effect transistors.

Model for Nonrelativistic Topological Multiferroic Matter.

We provide a model capable of accounting for the multiferroicity in certain materials. The model's base is on free electrons and spin moments coupled within nonrelativistic quantum mechanics. The synergistic interplay between the magnetic and electric degrees of freedom that turns into the multiferroic phenomena occurs at a profound quantum mechanical level, conjured by Berry's phases and the quantum theory of polarization. Our results highlight the geometrical nature of the multiferroic order parameter that naturally leads to magnetoelectric domain walls, with promising technological potential.

Hopfion-Driven Magnonic Hall Effect and Magnonic Focusing.

Hopfions are localized and topologically nontrivial magnetic configurations that have received considerable attention in recent years. In this Letter, we use a micromagnetic approach to analyze the scattering of spin waves (SWs) by magnetic hopfions. Our results evidence that SWs experience an electromagnetic field generated by the hopfion and sharing its topological properties. In addition, SWs propagating along the hopfion symmetry axis are deflected by the magnetic texture, which acts as a convergent or divergent lens, depending on the SWs' propagation direction. Assuming that SWs propagate along the plane perpendicular to the symmetry axis, the scattering is closely related to the Aharonov-Bohm effect, allowing us to identify the magnetic hopfion as a scattering center.

Magnetostatic interaction between Bloch point nanospheres.

Three-dimensional topological textures have become a topic of intense interest in recent years. This work uses analytical and numerical calculations to determine the magnetostatic field produced by a Bloch point (BP) singularity confined in a magnetic nanosphere. It is observed that BPs hosted in a nanosphere generate magnetic fields with quadrupolar nature. This finding is interesting because it shows the possibility of obtaining quadrupole magnetic fields with just one magnetic particle, unlike other propositions considering arrays of magnetic elements to generate this kind of field. The obtained magnetostatic field allows us to determine the interaction between two BPs as a function of the relative orientation of their polarities and the distance between them. It is shown that depending on the rotation of one BP related to the other, the magnetostatic interaction varies in strength and character, being attractive or repulsive. The obtained results reveal that the BP interaction has a complex behavior beyond topological charge-mediated interaction.

Magnetic Otto Engine for an Electron in a Quantum Dot: Classical and Quantum Approach.

We studied the performance of classical and quantum magnetic Otto cycle with a working substance composed of a single quantum dot using the Fock-Darwin model with the inclusion of the Zeeman interaction. Modulating an external/perpendicular magnetic field, in the classical approach, we found an oscillating behavior in the total work extracted that was not present in the quantum formulation.We found that, in the classical approach, the engine yielded a greater performance in terms of total work extracted and efficiency than when compared with the quantum approach. This is because, in the classical case, the working substance can be in thermal equilibrium at each point of the cycle, which maximizes the energy extracted in the adiabatic strokes.

Magnonic Black Holes.

We show that the interaction between the spin-polarized current and the magnetization dynamics can be used to implement black-hole and white-hole horizons for magnons-the quanta of oscillations in the magnetization direction in magnets. We consider three different systems: easy-plane ferromagnetic metals, isotropic antiferromagnetic metals, and easy-plane magnetic insulators. Based on available experimental data, we estimate that the Hawking temperature can be as large as 1 K. We comment on the implications of magnonic horizons for spin-wave scattering and transport experiments, and for magnon entanglement.

The mechanism of Menshutkin reaction in gas and solvent phases from the perspective of reaction electronic flux.

The mechanism of Menshutkin reaction, NH(3) + CH(3)Cl = [CH(3)-NH(3)]+ + Cl-, has been thoroughly studied in both gas and solvent (H(2)O and cyclohexane) phase. It has been found that solvents favor the reaction, both thermodynamically and kinetically. The electronic activity that drives the mechanism of the reaction was identified, fully characterized, and associated to specific chemical events, bond forming/breaking processes, by means of the reaction electronic flux. This led to a complete picture of the reaction mechanism that was independently confirmed by natural bond-order analysis and the dual descriptor for chemical reactivity and selectivity along the reaction path.

Insights into the mechanism of an S(N)2 reaction from the reaction force and the reaction electronic flux.

The mechanism of a simple S(N)2 reaction, viz; OH(-) + CH(3)F = CH(3)OH + F(-) has been studied within the framework of reaction force and reaction electronic flux. We have computationally investigated three different types of reaction mechanisms with two different types of transition states, leading to two different products. The electronic transfer contribution of the reaction electronic flux was found to play a crucial role in this reaction. Natural bond order analysis and dual descriptor provide additional support for elucidating the mechanism of this reaction.

Current-induced exchange interactions and effective temperature in localized moment systems.

We study theoretically the spin dynamics of a magnetic dimer serving as a contact between two electrodes. We find that the spin-spin coupling in the dimer can be dramatically modified from its equilibrium value. We show that the interaction can be tuned in such a way that it effectively changes its sign. The calculations show that, for large enough bias, the exchange interaction can even be changed from antiferromagnetic to ferromagnetic. The physical principles behind this result can be used as a new tool to achieve magneto-electric effects in molecular magnet systems.

Dynamics and spontaneous coherence of magnons in ferromagnetic thin films.

A theory of the dynamics of the Bose-Einstein condensate of magnons is presented. It is shown that, despite magnon decay processes, ongoing during the condensate formation, the system manifests spontaneous quantum coherence with a pseudo-spin degree of freedom originated from the presence of two valleys in momentum space. Finally, a real space description of the condensed state is provided, revealing the condensate state as a spin density wave. The effective dynamics of the spinor condensate wavefunction is characterized, and it is shown to display Josephson-like relations.

Quantum tunneling in nanomagnetic systems with different uniaxial anisotropy order.

A study of macroscopic quantum tunneling (MQT) of the magnetic moment in systems with quadratic and higher order uniaxial anisotropy and Zeeman interaction is presented. By using the instanton technique, under the giant spin approximation, the escape rate or probability per unit of time Gamma that the system undergoes a transition between coherent or metastable states is calculated. Using an effective particle potential we also determine the escape temperature T(e)(T), which marks the transition from quantum tunneling to thermal activation. A discussion is presented about the different models and the behavior of the magnetic system under the tunneling regime.

Interlayer transport in bilayer quantum Hall systems.

Bilayer quantum Hall systems have a broken symmetry ground state at a filling factor which can be viewed either as an excitonic superfluid or as a pseudospin ferromagnet. We present a theory of interlayer transport in quantum Hall bilayers that highlights remarkable similarities and critical differences between transport in Josephson junction and ferromagnetic metal spin-transfer devices. Our theory is able to explain the size of the large but finite low-bias interlayer conductance and the voltage width of this collective transport anomaly.