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Complementary metal-oxide semiconductor (CMOS) image sensor sensitivity in the near-infrared spectrum is limited by the absorption length in silicon. To deal with that limitation, we evaluate the implementation of a polysilicon nano-grating inside a pixel, at the transistor gate level of a 90 nm standard CMOS process, through opto-electrical simulations. The studied pixel structure involves a polysilicon nano-grating, designed with the fabrication layer of the transistor gate, which does not require any modifications in the process flow. The diffraction effect of the nano-grating increases the length of the light path in the photosensitive area and thus increases the photoelectric conversion efficiency. The nano-grating is integrated in combination with deep trench isolations to reduce cross talk between pixels. Coupled optical and electrical simulations report 33% external quantum efficiency improvement and 7% cross talk reduction at 850 nm.
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Nanogap antennas are compelling structures for squeezing light into ultrasmall volumes. However, when gaps are shrunk to the nanometer scale, the mode losses dramatically increase. In this Letter, we report the conditions of critical coupling between the arrays of nanogap resonant metal-insulator-metal (MIM) antennas and free space. Adapting the antenna density, critical coupling is achievable for any thickness of insulator, from 100 down to 0.1 nm. The fundamental optical mode can be described as continuous transitions through three types of modes: a perfect MIM mode, coupling between the MIM mode and surface plasmon polariton, and a gap plasmon mode. We found that the space between adjacent antennas is an essential parameter to perform critical coupling for thinner gaps. These results pave the way towards understanding extreme confinement in nanogap antenna structures such as MIM or nanoparticle arrays.
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Physical properties of nanocrystals self-assembled into 3D superlattices called supracrystals are highly specific with unexpected behavior. The best example to support such a claim was given through STM/STS experiments at low temperature of very thick supracrystals (around 1000 layers) where it was possible to image the surpracrystal surface and study their electronic properties. From previous studies, we know the optical properties of Ag nanocrystals self-assembled in a hexagonal network two-dimensional (2D) or by forming small 3D superlattices (from around 2 to 7 layers) are governed by dipolar interactions. Here, we challenge to study the optical properties of Ag supracrystals film characterized by large thicknesses (from around 27 to 180 Ag nanocrystals layers). In such experimental conditions, according to the classical Beer-Lambert law, the absorption of Ag films is expected to be very large, and the film transmission is close to zero. Very surprisingly, we observe reduced transmission intensity with an increase of the notch line width, in the 300-800 nm wavelength range, as the supracrystal film thickness increased. By calculating the transmission through the supracrystal films, we deduced that the films were dominated by the presence of cracks with wetting layers existing at their bottoms. This result was also confirmed by optical micrographs. The cracks widths increased with increasing the film thickness leading to more complex wetting layers. We also demonstrated the formation of small Ag clusters at the nanocrystal surface. These results provide some implications toward the design of plasmonic materials.
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Nano-resonators can be used in photovoltaics to drastically improve the ability of the device to absorb light and generate photo-carriers, therefore enabling a reduction of the absorber volume. Conventionally, the harvest of the spectrally broad solar spectrum is achieved via the tedious engineering of multiple optical resonances. In this paper, we propose a breakthrough approach, which consists in reducing the solar spectral range with a spectral conversion layer to match only one resonance that can then be easily designed. We use a Maxwell solver and a ray-tracing code to optimize the nano-resonator and its spectral converter. We show that 66.2% optical efficiency can be theoretically achieved in less than 40 nm mean thick absorber while leading to device design enabling collection of photo-generated carriers.
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We present a theoretical study of guided-mode-resonance filters made of two sub-wavelength metallic gratings and a dielectric waveguide, with lateral geometries compatible with the size of infrared focal plane array pixels. Contrary to most of the studies described in the literature, we consider here a focused beam on finite-sized filters, and we investigate the optical properties of a mosaic of 30 µm-long filters. We demonstrate the spectral filtering ability and low crosstalk of such components. We also study the impact of an oblique beam onto a filtering mosaic. We finally discuss the opportunities offered by these results for a new generation of multispectral infrared cameras, and we give an example of a simple architecture.
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Plasmon lasers are a new class of coherent light sources that use metals for light localization and amplification. Access to this confined light that couples to the oscillating electrons of metal enables reducing the physical size and mode volume of the laser much below the diffraction limit. The race to demonstrate new plasmon nanolasers has enabled considerable progress over the last several years regarding nanocavity design, operating temperature, pumping conditions, and material efficiency of both plasmonic nanocavity and gain medium. This article discusses some of the latest developments of coherent nanoscopic light sources, in metallic and dielectric lasers, with a specific focus on plasmon nanolasers. We highlight recent advances in plasmon lasers through plasmonic nanoparticle arrays: beam directionality, wavelength tunability, multi-modal emission, and dark and bright modes lasing. We also discuss future prospects.
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We present a theoretical study of the mid-infrared guided mode resonance spectral filters made of two subwavelength metallic gratings and a dielectric waveguide under a focused beam with a finite spot size. This Letter shows that, at the resonant wavelength, the lateral extension of the electromagnetic field in the waveguide is close to the width of the beam. We compare the performance of filters using gratings with a one-slit pattern and gratings with a two-slit pattern, and we show that the latter gratings (biatom gratings) provide a higher transmission and a better limitation of field extension, due to an improved angular acceptance. These results open new perspectives for pixel-sized infrared filters.
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Hydrophobic Au nanocrystal assemblies (both ordered and amorphous) were dispersed in aqueous solution via the assistance of lipid vesicles. The intertwine between vesicles and Au assemblies was made possible through a careful selection of the length of alkyl chains on Au nanocrystals. Extinction spectra of Au assemblies showed two peaks that were assigned to a scattering mode that red-shifted with increasing the assembly size and an absorption mode associated with localized surface plasmon that was independent of their size. This plasmon fingerprint could be used as a probe for investigating the optical properties of such assemblies. Our water-soluble assemblies enable exploring a variety of potential applications including solar energy and biomedicine.
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This paper deals with the integration of metallic and dielectric nanostructured planar lenses into a pixel from a silicon based CMOS image sensor, for a monochromatic application at 1.064 µm. The first is a Plasmonic Lens, based on the phase delay through nanoslits, which has been found to be hardly compatible with current CMOS technology and exhibits a notable metallic absorption. The second is a dielectric Phase-Fresnel Lens integrated at the top of a pixel, it exhibits an Optical Efficiency (OE) improved by a few percent and an angle of view of 50°. The third one is a metallic diffractive lens integrated inside a pixel, which shows a better OE and an angle of view of 24°. The last two lenses exhibit a compatibility with a spectral band close to 1.064 µm.
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Symmetric metal-dielectric guided-mode resonators (GMR) can operate as infrared band-pass filters, thanks to high-transmission resonant peaks and good rejection ratio. Starting from matrix formalism, we show that the behavior of the system can be described by a two-mode model. This model reduces to a scalar formula and the GMR is described as the combination of two independent Fabry-Perot resonators. The formalism has then been applied to the case of asymmetric GMR, in order to restore the properties of the symmetric system. This result allows designing GMR-on-substrate as efficient as free-standing systems, the same high transmission maximum value and high quality factor being conserved.
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Optical Helmholtz resonators (OHRs) have been adapted from acoustics designs for light absorbing structures, exhibiting extreme light confinement. Here, extraordinary transmission of light is theoretically demonstrated through symmetric OHRs, comprising a cavity with two λ/500 narrow slits on either side. This device has appealing features to act as a spectral bandpass filter in the context of multispectral imaging, in particular its high angular tolerance because of the localized nature of the resonance. Besides, the cavity can be modeled as an inductor and the two slits can be modeled as capacitors, the whole design acting as a LC circuit thus preventing any harmonic features.
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We propose a design to confine light absorption in flat and ultra-thin amorphous silicon solar cells with a one-dimensional silver grating embedded in the front window of the cell. We show numerically that multi-resonant light trapping is achieved in both TE and TM polarizations. Each resonance is analyzed in detail and modeled by Fabry-Perot resonances or guided modes via grating coupling. This approach is generalized to a complete amorphous silicon solar cell, with the additional degrees of freedom provided by the buffer layers. These results could guide the design of resonant structures for optimized ultra-thin solar cells.
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We show that a periodic array of metal-insulator-metal resonators can be described as a high refractive index metamaterial. This approach permits to obtain analytically the optical properties of the structure and thus to establish conception rules on the quality factor or on total absorption. Furthermore, we extend this formalism to the combination of two independent resonators.
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Luz , Manufaturas , Nanopartículas Metálicas/química , Modelos Teóricos , Espalhamento de Radiação , Absorção , Simulação por Computador , Condutividade Elétrica , RefratometriaRESUMO
We present a modal method for the fast analysis of 2D-layered gratings. It combines exact discrete formulations of Maxwell equations in 2D space with polynomial approximations of the constitutive equations, and provides a sparse formulation of the eigenvalue equations. In specific cases, the use of sparse matrices allows us to calculate the electromagnetic response while solving only a small fraction of the eigenmodes. This significantly increases computational speed up to 100×, as shown on numerical examples of both dielectric and metallic subwavelength gratings.
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We theoretically study metal-dielectric structures made of bi-atomic metallic gratings coupled to a guided-mode dielectric resonator. The bi-atomic pattern grating allows tailoring of the Fourier spectrum of the inverse grating permittivity in order to adapt the frequency gap and obtain a flat dispersion band over a wide angular range. A significant enhancement (two-fold) of the angular tolerance as compared to a simply periodic structure is obtained.
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We demonstrate that almost 100% of incident photons can interact with a monolayer of scatterers in a symmetrical environment. Nearly perfect optical extinction through free-standing transparent nanorod arrays has been measured. The sharp spectral opacity window, in the form of a characteristic Fano resonance, arises from the coherent multiple scattering in the array. In addition, we show that nanorods made of absorbing material exhibit a 25-fold absorption enhancement per unit volume compared to unstructured thin film. These results open new perspectives for light management in high-Q, low volume dielectric nanostructures, with potential applications in optical systems, spectroscopy, and optomechanics.
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Modelos Químicos , Nanotubos/química , Fótons , Fenômenos Eletromagnéticos , Membranas Artificiais , Espalhamento de Radiação , Compostos de Silício/químicaRESUMO
We study experimentally and theoretically band-pass filters based on guided-mode resonances in free-standing metal-dielectric structures with subwavelength gratings. A variety of filters are obtained: polarizing filters with 1D gratings, and unpolarized or selective filters with 2D gratings, which are shown to behave as two crossed-1D structures. In either case, a high transmission (up to ≈ 79 %) is demonstrated, which represents an eight-fold enhancement compared to the geometrical transmission of the grating. We also show that the angular sensitivity strongly depends on the rotation axis of the sample. This behavior is explained with a detailed description of the guided-mode transmission mechanism.
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We retrieve the complex optical index of single-walled carbon nanotube (CNT) films in the 0.6-800 µm spectral range. Results are obtained from a complete set of optical measurements, reflection and transmission, of free-standing CNT films using time domain spectroscopy in the terahertz (THz) and Fourier transform infrared (IR) spectroscopy in the visible-IR. Based on a Drude-Lorentz model, our results reveal a global metallic behavior of the films in the IR, and confirm their high optical index in the THz range.
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In this Letter, we demonstrate experimentally that a patchwork of four metal-insulator-metal patches leads to an unpolarized wideband omnidirectional infrared absorption. Our structure absorbs 70% of the incident light on a 2.5 µm bandwidth at 8.5 µm. It paves the way to the design of wideband efficient plasmonic absorbers in the infrared spectrum.
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We investigate the mechanisms involved in the funneling of optical energy into subwavelength grooves etched on a metallic surface. The key phenomenon is unveiled thanks to the decomposition of the electromagnetic field into its propagative and evanescent parts. We unambiguously show that the funneling is not due to plasmonic waves flowing toward the grooves, but rather to the magnetoelectric interference of the incident wave with the evanescent field, this field being mainly due to the resonant wave escaping from the groove.