Simulations of the gain profile and performance of a diode side-pumped QCW Nd:YAG laser.

A design of a diode side-pumped Nd:YAG laser module and simulations of the gain distribution inside the active medium are presented in this paper. The code is based on a nonsequential ray-tracing Monte Carlo method for the light generated by the laser diodes. The fluorescence image of the active medium was analyzed in order to compare it with the simulations, which were found to be in good agreement with experimental data. The laser was tested in QCW mode and provided a maximum average power of 220 W while maintaining constant energy per pulse in the 100-1000 Hz range.

Mode-locked laser operation of Indium-modified Yb:KY(WO4)2 single crystal.

We report the first pulsed laser operation of an Indium-modified Yb:KY(WO4)2 crystal. Indium incorporation enlarges the broadening of the Yb3+ optical bands, reduces crystal lattice parameters and increases n(p) refractive index. A KY0.8In0.07Yb0.13(WO4)2 crystal pumped at 981 nm with a Ti-sapphire laser in a SESAM modulated resonator produces at 300 K self-starting and stable mode-locking. The shortest laser pulses achieved were centred at λ = 1041.1 nm, have a duration of 96 fs with average power of 134 mW and repetition rate of 103.5 MHz (1.3 nJ/pulse).

Femtosecond infrared intrastromal ablation and backscattering-mode adaptive-optics multiphoton microscopy in chicken corneas.

The performance of femtosecond (fs) laser intrastromal ablation was evaluated with backscattering-mode adaptive-optics multiphoton microscopy in ex vivo chicken corneas. The pulse energy of the fs source used for ablation was set to generate two different ablation patterns within the corneal stroma at a certain depth. Intrastromal patterns were imaged with a custom adaptive-optics multiphoton microscope to determine the accuracy of the procedure and verify the outcomes. This study demonstrates the potential of using fs pulses as surgical and monitoring techniques to systematically investigate intratissue ablation. Further refinement of the experimental system by combining both functions into a single fs laser system would be the basis to establish new techniques capable of monitoring corneal surgery without labeling in real-time. Since the backscattering configuration has also been optimized, future in vivo implementations would also be of interest in clinical environments involving corneal ablation procedures.

Wavefront retrieval of amplified femtosecond beams by second-harmonic generation.

We present a new approach for wavefront characterization of near transform-limited intense femtosecond beams using the angular and spectral dependences of the second-harmonic generation conversion efficiency in uniaxial crystals. The method is applied to different aberrated beams and results are compared with the measurements performed with a commercial sensor, finding very good agreement. The phase retrieval dependence with different parameters (e.g. crystal thickness) is discussed. Successful application to sharpen intensity profiles is also demonstrated.

Enhancement of filamentation postcompression by astigmatic focusing.

The energy scaling up of pulse postcompression is still an open issue. In this work we analyze the use of astigmatic focusing to improve the output pulses in a filamentation based postcompression setup. Unlike spherical conditions, astigmatic focusing enhances the output energy and the spectral broadening of the filament. This is due to the increase of critical power, allowing a considerable improvement of the postcompression energy and stability in a simple way. We demonstrated compression from FWHM 100 fs, 10 nm, 3 mJ input pulses to 13 fs, 142 nm, near 1 mJ pulses.

A new method for relative Sr determination in human teeth enamel.

We present a new method to determine Sr/Ca changes in hard dental tissues based on laser ablation and spectroscopic detection. By using femtosecond Laser Induced Breakdown Spectroscopy (fs-LIBS), we micro mapped the relative amount of strontium in the enamel of three human lower third molar. We also analyzed the Sr/Ca ratio along the striae of Retzius. Results show that microlibs allows detection of variation in relative Sr/Ca ratio through enamel. The same values of Sr/Ca ratio were found along a single stria. The method has a precision better than 95% and is sensitive enough to detect Sr/Ca ratio variations among striae and within stria. Fs-LIBS generates information in a fast and simple way that can be used by non-specialists to make inferences about diet or mobility in human populations and fossil hominids.

Spatio-temporal characterization of ultrashort pulses diffracted by circularly symmetric hard-edge apertures: theory and experiment.

We carry out a complete spatio-temporal characterization of the electric field of an ultrashort laser pulse after passing through a diffractive optical element composed of several binary amplitude concentric rings. Analytical expressions for the total diffraction field in the time and spectral domain are provided, using the Rayleigh-Sommerfeld formulation of the diffraction. These expressions are experimentally validated. The spatio-temporal amplitude and phase structure of the pulse are measured at different planes beyond the diffractive optical element using spatially-resolved spectral interferometry assisted by an optical fiber coupler (STARFISH). Our results allow corroborating theoretical predictions on the presence of multiple pulses or complex spectral distributions due to the diffraction-induced effects by the hard-edge ring apertures.

Femtosecond multi-filamentation control by mixture of gases: towards synthesised nonlinearity.

We have investigated femtosecond multi-filamentation process in a mixture of gases controlling the concentration of atoms versus molecules in the gas cell. The experimental results show that this control could provide a new freedom degree to deterministic spatial distribution control of the multiple filaments. Our simulation indicates surprisingly that only difference of the gases nonlinearity (referred to as "synthesised nonlinearity") is sufficient to be responsible for this control. This study opens the way to provide few-cycle pulses spatial distributed source for spatially encoded measurements and experiments.

Above-millijoule super-continuum generation using polarisation dependent filamentation in atoms and molecules.

We demonstrate for the first time that input polarisation control inducing one single filamentation is a very robust technique to accurately control the filamentation dynamics enhancing throughput energy of the supercontinuum generation up to 1.2 millijoule. Reaching the above-millijoule regime opens the way to post-compression of multi-terawatt laser pulses.

Temporal wavefront stability of an ultrafast high-power laser beam.

We measured the temporal dynamics of wavefront aberrations in a beam produced by a commercial ultrafast high-power laser with a research-prototype real-time Hartmann-Shack wavefront sensor. Measurements were performed at two different temporal rates for a 7 mm diameter. Results showed that changes in the wavefront aberrations were always lower than 1%. The main contribution to the total root-mean-square (RMS) wavefront error was due to the effects of low order aberrations (defocus and astigmatism), which persisted even after cavity realignment. The potential improvement in the beam quality after correction of the different aberration modes was also shown. Real-time measurements of laser aberrations while modifying cavity parameters might be a useful tool to improve the beam quality.

Non-collinear sum-frequency generation of femtosecond pulses in a micro-structured beta-BaB2O4 crystal.

Sum-frequency generation of femtosecond pulses by noncollinear phase matching in a micro-structured beta-BaB(2)O(4) crystal has been investigated. A 1D relief grating was recorded in the surface of a beta-BaB(2)O(4) crystal by direct irradiation with femtosecond pulses. Groove dimensions of 1 mum width and 200 nm depth were obtained for the recording parameters. This micro-structured crystal was used for generating ultraviolet pulses (265 nm) by noncollinear sum-frequency generation of the fundamental and the second harmonic of a Ti:Sapphire femtosecond laser system. Effective group-velocity matching between the incident pulses can be achieved for certain noncollinear processes in a compact way. The application of such device to intensity cross-correlation measurements of the second-harmonic pulse was shown.

Femtosecond laser disruption of filamentous cyanobacteria unveils dissimilar cellular stability between heterocysts and vegetative cells.

Filamentous cyanobacteria develop heterocysts in response to deprivation for combined nitrogen under aerobic conditions. The most prominent structural change in heterocysts is the biosynthesis of an envelope that restricts gas permeability, providing an appropriate micro-oxic environment for N2 fixation inside. The additional thickness of the differentiated cells, when compared to vegetative cells, makes filamentous cyanobacteria an attractive biological system to investigate cellular response against femtosecond laser processing. By irradiating the cyanobacterial filaments with 120 fs, 795 nm, 1 kHz pulses focused through a 100x microscope objective with a numerical aperture of 0.85, we have determined that the pulse energy threshold for an apparent disruption of the cell wall of vegetative cells is 13 +/- 4 nJ per pulse. A further increase in the pulse energy to 43 +/- 13 nJ causes the complete removal of vegetative cells. In contrast, the pulse energy threshold has to be augmented about three-fold for heterocyst envelope disruption or two-fold for complete removal of heterocysts. We propose that the singular cross-linked structure of the glycolipid multilayer of the envelope, required to restrict gas permeability, accounts for the remarked difference in the ablation energy threshold between vegetative cells and heterocysts.

Femtosecond laser written surface waveguides fabricated in Nd:YAG ceramics.

Near surface channel waveguides have been fabricated in Neodymium doped YAG ceramics by using IR femtosecond laser irradiation at the low frequency regime. Single mode guidance has been demonstrated with propagation losses of ~1 dB/cm. Time resolved confocal micro-luminescence experiments have been used to determine the spectroscopic properties of the Nd(3+) laser ions in the channel waveguide as well as to elucidate the waveguide formation processes.

Synthesis of ceramic nanoparticles by ultrafast laser ablation of solid targets in water.

We report production of nanoparticles of several advanced ceramics (Si3N4, SiC, AlN, and Al2O3) by ablation with femtosecond laser pulses of solid targets submerged in deionized water. The products withstand comparison with commercial nanoparticle suspensions obtained by other techniques as they are analyzed by means of transmission electron microscopy. As compared with metal nanoparticles produced with the same technique, we have found that the overall dependence of mean sizes and distribution widths on the laser fluence is similar. We explain why it is difficult to synthetize very small (<5 nm) and monodisperse particles in terms of ablation mechanism and discuss the aplicability of the technique for industrial production.

Ab initio calculation of the double ionization of helium in a few-cycle laser pulse beyond the one-dimensional approximation.

We present ab initio computations of the ionization of two-electron atoms by short pulses of intense linearly polarized Ti:sapphire laser radiation beyond the one-dimensional approximation. In the model the electron correlation is included in its full dimensionality, while the center-of-mass motion is restricted along the polarization axis. Our results exhibit a rich double ionization quantum dynamics in the direction transversal to the field polarization, which is neglected in the previous models based on the one-dimensional approximation.

Non-linear Young's double-slit experiment.

The Young's double slit experiment is recreated using intense and short laser pulses. Our experiment evidences the role of the non-linear Kerr effect in the formation of interference patterns. In particular, our results evidence a mixed mechanism in which the zeroth diffraction order of each slit are mainly affected by self-focusing and self-phase modulation, while the higher orders propagate linearly. Despite of the complexity of the general problem of non-linear propagation, we demonstrate that this experiment retains its simplicity and allows for a geometrical interpretation in terms of simple optical paths. In consequence, our results may provide key ideas on experiments on the formation of interference patterns with intense laser fields in Kerr media.

Hydrogen atom interacting with a multifrequency laser field: ionization and harmonic generation.

The response of a hydrogen atom submitted to a multiharmonic laser field is studied. The relative phases of the harmonic components are critical both for atomic ionization and high-order harmonic generation. In the phase-locked case under adequate interference conditions, the inhibition of ionization is followed by an increase of the intensities of the generated harmonics.

Lithium ionization by a strong laser field.

We study ab initio computations of the interaction of lithium with a strong laser field. Numerical solutions of the time-dependent fully correlated three-particle Schrodinger equation restricted to the one-dimensional soft-core approximation are presented. Our results show a clear transition from nonsequential to sequential double ionization for increasing intensities. Nonsequential double ionization is found to be sensitive to the spin configuration of the ionized pair. This asymmetry, also found in experiments of photoionization of Li with synchrotron radiation, shows evidence of the influence of the exclusion principle on the underlying rescattering mechanism.

Coherent population trapping in two-electron three-level systems with aligned spins.

The possibility of coherent population trapping in two electron states with aligned spins (orthosystem) is evidenced. From the analysis of a three-level atomic system containing two electrons, and driven by the two laser fields needed for coherent population trapping, a conceptually new kind of dark state appears. The properties of this trapping are physically interpreted in terms of a dark hole, instead of a dark two-electron state. This technique, among many other applications, offers the possibility of measuring, with subnatural resolution, some superposition-state matrix elements of the electron-electron correlation that due to their time dependent nature are inaccessible by standard measuring procedures.