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2.
Sci Rep ; 13(1): 12657, 2023 Aug 04.
Artigo em Inglês | MEDLINE | ID: mdl-37542076

RESUMO

The neutron capture cross section of [Formula: see text]Ta is relevant to s-process of nuclear astrophysics, extraterrestrial samples analysis in planetary geology and new generation nuclear energy system design. The [Formula: see text]Ta([Formula: see text]) cross section had been measured between 1 eV and 800 keV at the back-streaming white neutron facility (Back-n) of China spallation neutron source(CSNS) using the time-of-flight (TOF) technique and [Formula: see text] liquid scintillator detectors. The experimental results are compared with the data of several evaluated libraries and previous experiments in the resolved and unresolved resonance region. Resonance parameters are extracted using the R-Matrix code SAMMY in the 1-700 eV region. The astrophysical Maxwell average cross section(MACS) from kT = 5 to 100 keV is calculated over a sufficiently wide range of neutron energies. For the characteristic thermal energy of an astrophysical site, at kT = 30keV the MACS value of [Formula: see text]Ta is 834 ± 75 mb, which shows an obvious discrepancy with the Karlsruhe Astrophysical Database of Nucleosynthesis in Stars (KADoNiS) recommended value 766 ± 15 mb. The new measurements strongly constrain the MACS of [Formula: see text]Ta([Formula: see text]) reaction in the stellar s-process temperatures.

3.
Appl Radiat Isot ; 200: 110948, 2023 Oct.
Artigo em Inglês | MEDLINE | ID: mdl-37556935

RESUMO

The precise measurement of the (n, 2n) reaction cross-sections of xenon isotopes is of great significance for the diagnosis of the Inertial Confinement Fusion fuel area density ρR. The preparation of xenon samples and how they can be efficiently adsorbed to obtain an optimal reaction cross section are extremely difficult in existing experiments. This work aims to use the 93Nb(n,2n)92mNb reaction cross section as the standard to calculate the cross-sections and isomeric ratio for 134Xe(n,2n)133m,gXe and 136Xe(n,2n)135m,gXe reactions. This work also aims to explore the feasibility of adsorbent selection, the method of adsorption sample and the feasibility of the method used in the laboratory. In this paper, the Geant4 program was used to simulate and calculate the adsorption factors of activated carbon and polymer for standard 152Eu multi-line sources, so as to determine the most suitable adsorption material. Next, the GammaVision analysis software was used to observe whether the characteristic γ-rays released by other isotope reaction products of xenon in the sample and packaging material had an effect on the characteristic γ-rays of the target product. Then, the basic principle of activation method and the relative measurement principle are used to calculate the cross-sections and isomeric ratio for 134Xe(n,2n)133Xe and 136Xe(n,2n)135Xe reactions. Finally, the experimental results are compared and analyzed with the existing data in EXFOR database to verify whether the experimental method is correct.

4.
Appl Radiat Isot ; 200: 110907, 2023 Oct.
Artigo em Inglês | MEDLINE | ID: mdl-37429224

RESUMO

Off-line gamma-ray spectrometry was used to accurately measure the Cumulative fission product yields (CFPYs) of fission products in the 235U (n, f) reaction induced by 2.8 MeV neutrons. The 2.8 MeV quasi-monoenergetic neutron beam was produced by the CPNG-600 Cockcroft Walton accelerator at the China Institute of Atomic Energy (CIAE)and the gamma spectra were measured by the HPGe γ-ray Spectrometer. After fully considering and revising the sources of uncertainty, high-precision CFPYs of 4 fission products were obtained. This study has important applications in reactor design and operation and is conducive to the establishment of an evaluated nuclear database.

5.
Appl Radiat Isot ; 186: 110260, 2022 Aug.
Artigo em Inglês | MEDLINE | ID: mdl-35537299

RESUMO

The measurement of the 59Co(n,2n)58Co reaction cross section with the neutron energy of 14.8 MeV has been performed by the activation method and relative measurement principle. The 300 kV Cockcroft Walton Accelerator of China Institute of Atomic Energy was used to produce quasi monoenergetic neutron beams by the T(D, n)4He reaction. Two thin 27Al and 93Nb foils were attached to the 59Co target and performed as monitors. After the irradiation, the HPGe detector and the GammaVision software were used to measure the activity of the irradiated samples and record the counts of γ-rays, respectively. Finally, some relevant physical quantities were corrected after comparing the results with experimental data in the EXFOR database and evaluated data in the ENDF database.

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