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1.
J Air Waste Manag Assoc ; 67(9): 986-999, 2017 09.
Artigo em Inglês | MEDLINE | ID: mdl-28498778

RESUMO

In recent years, many air quality monitoring programs have favored measurement of particles less than 2.5 µm (PM2.5) over particles less than 10 µm (PM10) in light of evidence that health impacts are mostly from the fine fraction. However, the coarse fraction (PM10-2.5) may have independent health impacts that support continued measurement of PM10 in some areas, such as those affected by road dust. The objective of this study was to evaluate the associations between different measures of daily PM exposure and two daily indicators of population health in seven communities in British Columbia, Canada, where road dust is an ongoing concern. The measures of exposure were PM10, PM2.5, PM10-2.5, PM2.5 adjusted for PM10-2.5, and PM10-2.5 adjusted for PM2.5. The indicators of population health were dispensations of the respiratory reliever medication salbutamol sulfate and nonaccidental mortality. This study followed a time-series design using Poisson regression over a 2003-2015 study period, with analyses stratified by three seasons: residential woodsmoke in winter; road dust in spring; and wildfire smoke in summer. A random-effects meta-analysis was conducted to establish a pooled estimate. Overall, an interquartile range increase in daily PM10-2.5 was associated with a 3.6% [1.6, 5.6] increase in nonaccidental mortality during the road dust season, which was reduced to 3.1% [0.8, 5.4] after adjustment for PM2.5. The adjusted coarse fraction had no effect on salbutamol dispensations in any season. However, an interquartile range increase in PM2.5 was associated with a 2.7% [2.0, 3.4] increase in dispensations during the wildfire season. These analyses suggest different impacts of different PM fractions by season, with a robust association between the coarse fraction and nonaccidental mortality in communities and periods affected by road dust. We recommend that PM10 monitoring networks be maintained in these communities to provide feedback for future dust mitigation programs. IMPLICATIONS: There was a significant association between daily concentrations of the coarse fraction and nonaccidental mortality during the road dust season, even after adjustment for the fine fraction. The acute and chronic health effects associated with exposure to the coarse fraction remain unclear, which supports the maintenance of PM10 monitoring networks to allow for further research in communities affected by sources such as road dust.


Assuntos
Poluentes Atmosféricos/análise , Material Particulado/análise , Saúde da População , Adolescente , Idoso , Albuterol/uso terapêutico , Colúmbia Britânica , Monitoramento Ambiental , Humanos , Mortalidade , Tamanho da Partícula , Prescrições/estatística & dados numéricos , Estações do Ano , Meios de Transporte
2.
Environ Pollut ; 220(Pt B): 797-806, 2017 Jan.
Artigo em Inglês | MEDLINE | ID: mdl-27838060

RESUMO

Residential woodsmoke is an under-regulated source of fine particulate matter (PM2.5), often surpassing mobile and industrial emissions in rural communities in North America and elsewhere. In the province of British Columbia (BC), Canada, many municipalities are hesitant to adopt stricter regulations for residential wood burning without empirical evidence that smoke is affecting local air quality. The objective of this study was to develop a retrospective algorithm that uses 1-h PM2.5 concentrations and daily temperature data to identify smoky days in order to prioritise communities by smoke impacts. Levoglucosan measurements from one of the smokiest communities were used to establish the most informative values for three algorithmic parameters: the daily standard deviation of 1-h PM2.5 measurements; the daily mean temperature; and the daytime-to-nighttime ratio of PM2.5 concentrations. Alternate parameterizations were tested in 45 sensitivity analyses. Using the most informative parameter values on the most recent two years of data for each community, the number of smoky days ranged from 5 to 277. Heat maps visualizing seasonal and diurnal variation in PM2.5 concentrations showed clear differences between the higher- and lower-ranked communities. Some communities were sensitive to one or more of the parameters, but the overall rankings were consistent across the 45 analyses. This information will allow stakeholder agencies to work with local governments on implementing appropriate intervention strategies for the most smoke-impacted communities.


Assuntos
Poluentes Atmosféricos/análise , Monitoramento Ambiental , Material Particulado/análise , Fumaça/análise , Madeira/química , Colúmbia Britânica , Cidades , Habitação , Humanos , América do Norte , Estudos Retrospectivos
3.
Environ Sci Technol ; 50(6): 3174-83, 2016 Mar 15.
Artigo em Inglês | MEDLINE | ID: mdl-26885573

RESUMO

This paper presents a Geographical Information System (GIS) based probabilistic simulation framework to estimate PM2.5 population exposure in New Delhi, India. The framework integrates PM2.5 output from spatiotemporal LUR models and trip distribution data using a Gravity model based on zonal data for population, employment and enrollment in educational institutions. Time-activity patterns were derived from a survey of randomly sampled individuals (n = 1012) and in-vehicle exposure was estimated using microenvironmental monitoring data based on field measurements. We simulated population exposure for three different scenarios to capture stay-at-home populations (Scenario 1), working population exposed to near-road concentrations during commutes (Scenario 2), and the working population exposed to on-road concentrations during commutes (Scenario 3). Simulated annual average levels of PM2.5 exposure across the entire city were very high, and particularly severe in the winter months: ∼200 µg m(-3) in November, roughly four times higher compared to the lower levels in the monsoon season. Mean annual exposures ranged from 109 µg m(-3) (IQR: 97-120 µg m(-3)) for Scenario 1, to 121 µg m(-3) (IQR: 110-131 µg m(-3)), and 125 µg m(-3) (IQR: 114-136 µ gm(-3)) for Scenarios 2 and 3 respectively. Ignoring the effects of mobility causes the average annual PM2.5 population exposure to be underestimated by only 11%.


Assuntos
Poluentes Atmosféricos/análise , Exposição Ambiental/análise , Modelos Estatísticos , Material Particulado/análise , Poluentes Atmosféricos/efeitos adversos , Cidades , Exposição Ambiental/efeitos adversos , Monitoramento Ambiental , Sistemas de Informação Geográfica , Humanos , Índia , Material Particulado/efeitos adversos , Estações do Ano
4.
Environ Sci Technol ; 47(22): 12903-11, 2013 Nov 19.
Artigo em Inglês | MEDLINE | ID: mdl-24087939

RESUMO

Air pollution in New Delhi, India, is a significant environmental and health concern. To assess determinants of variability in air pollutant concentrations, we develop land use regression (LUR) models for fine particulate matter (PM2.5), black carbon (BC), and ultrafine particle number concentrations (UFPN). We used 136 h (39 sites), 112 h (26 sites), 147 h (39 sites) of PM2.5, BC, and UFPN data respectively, to develop separate morning (0800-1200) and afternoon (1200-1800) models. Continuous measurements of PM2.5 and BC were also made at a single fixed rooftop site located in a high-income residential neighborhood. No continuous measurements of UFPN were available. In addition to spatial variables, measurements from the fixed continuous monitoring site were used as independent variables in the PM2.5 and BC models. The median concentrations (and interquartile range) of PM2.5, BC, and UFPN at LUR sites were 133 (96-232) µg m(-3), 11 (6-21) µg m(-3), and 40 (27-72) × 10(3) cm(-3) respectively. In addition (a) for PM2.5 and BC, the temporal variability was higher than the spatial variability; (b) the magnitude and spatial variability in pollutant concentrations was higher during morning than during afternoon hours. Further, model R(2) values were higher for morning (for PM2.5, BC, and UFPN, respectively: 0.85, 0.86, and 0.28) than for afternoon models (0.73, 0.69, and 0.23); (c) the PM2.5 and BC concentrations measured at LUR sites all over the city were strongly correlated with measured concentrations at a fixed rooftop site; (d) spatial patterns were similar for PM2.5 and BC but different for UFPN; (e) population density and road variables were statistically significant predictors of pollutant concentrations; and (f) available geographic predictors explained a much lower proportion of variability in measured PM2.5, BC, and UFPN than observed in other LUR studies, indicating the importance of temporal variability and suggesting the existence of uncharacterized sources.


Assuntos
Cidades , Monitoramento Ambiental , Tamanho da Partícula , Material Particulado/química , Fuligem/química , Análise Espaço-Temporal , Poluentes Atmosféricos/química , Poluição do Ar/análise , Geografia , Índia , Análise de Regressão
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