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1.
Science ; 348(6232): 317-20, 2015 Apr 17.
Artigo em Inglês | MEDLINE | ID: mdl-25814065

RESUMO

In the quest for superconductors with higher transition temperatures (T(c)), one emerging motif is that electronic interactions favorable for superconductivity can be enhanced by fluctuations of a broken-symmetry phase. Recent experiments have suggested the existence of the requisite broken-symmetry phase in the high-T(c) cuprates, but the impact of such a phase on the ground-state electronic interactions has remained unclear. We used magnetic fields exceeding 90 tesla to access the underlying metallic state of the cuprate YBa2Cu3O(6+δ) over a wide range of doping, and observed magnetic quantum oscillations that reveal a strong enhancement of the quasiparticle effective mass toward optimal doping. This mass enhancement results from increasing electronic interactions approaching optimal doping, and suggests a quantum critical point at a hole doping of p(crit) ≈ 0.18.

2.
Phys Rev Lett ; 106(22): 226402, 2011 Jun 03.
Artigo em Inglês | MEDLINE | ID: mdl-21702619

RESUMO

A multiple wave vector (Q) reconstruction of the Fermi surface is shown to yield a profoundly different electronic structure to that characteristic of single wave vector reconstruction, despite their proximity in energy. We consider the specific case in which ordering is generated by Q(x)=[2πa,0] and Q(y)=[0,2πb] (in which a=b=1/4)-similar to those identified in neutron diffraction and scanning tunneling microscopy experiments-and more generally show that an isolated pocket adjacent to the nodal point k(nodal)=[±π/2,±π/2] is a protected feature of such a multiple-Q model, potentially corresponding to the nodal "Fermi arcs" observed in photoemission and the small size of the electronic heat capacity found in high magnetic fields-importantly, containing electron carriers which can yield negative Hall and Seebeck coefficients observed in high magnetic fields.

3.
Phys Rev Lett ; 106(14): 146403, 2011 Apr 08.
Artigo em Inglês | MEDLINE | ID: mdl-21561207

RESUMO

Using Shubnikov-de Haas oscillations measured in URu2Si2 over a broad range in a magnetic field of 11-45 T, we find a cascade of field-induced Fermi surface changes within the hidden order phase I and further signatures of oscillations within field-induced phases III and V [previously discovered by Kim et al., [Phys. Rev. Lett. 91, 256401 (2003)]. A comparison of kinetic and Zeeman energies indicates a pocket-by-pocket polarization of the Fermi surface leading up to the destruction of the hidden order phase I at ≈35 T. The anisotropy of the Zeeman energy driving the transitions in URu2Si2 points to an itinerant hidden order parameter involving quasiparticles whose spin degrees of freedom depart significantly from those of free electrons.

4.
Phys Rev Lett ; 102(21): 216402, 2009 May 29.
Artigo em Inglês | MEDLINE | ID: mdl-19519118

RESUMO

We present a detailed quantum oscillation study of the Fermi surface of the recently discovered Yb-based heavy fermion superconductor beta-YbAlB4. We compare the data, obtained at fields from 10 to 45 T, to band structure calculations performed using the local density approximation. Analysis of the data suggests that f holes participate in the Fermi surface up to the highest magnetic fields studied. We comment on the significance of these findings for the unconventional superconducting properties of this material.

5.
Phys Rev Lett ; 99(5): 056401, 2007 Aug 03.
Artigo em Inglês | MEDLINE | ID: mdl-17930772

RESUMO

We report measurements of the de Haas-van Alphen effect in CeIn(3) in magnetic fields extending to approximately 90 T, well above the Néel critical field of mu(0)H(c) approximately 61 T. The unreconstructed Fermi surface a sheet is observed in the high magnetic field polarized paramagnetic limit, but with its effective mass and Fermi surface volume strongly reduced in size compared to that observed in the low magnetic field paramagnetic regime under pressure. The spheroidal topology of this sheet provides an ideal realization of the transformation from a "large Fermi surface" accommodating f electrons to a "small Fermi surface" when the f-electron moments become polarized.

6.
Phys Rev Lett ; 98(25): 257201, 2007 Jun 22.
Artigo em Inglês | MEDLINE | ID: mdl-17678050

RESUMO

We show that the spatial dimensionality of the quantum critical point associated with Bose-Einstein condensation at T=0 is reduced when the underlying lattice comprises layers coupled by a frustrating interaction. Our theoretical predictions for the critical behavior correspond very well with recent measurements in BaCuSi(2)O(6) [ S. E. Sebastian et al., Nature (London) 441, 617 (2006)].

7.
Phys Rev Lett ; 98(1): 017202, 2007 Jan 05.
Artigo em Inglês | MEDLINE | ID: mdl-17358501

RESUMO

The compound BaCuSi2O6 is a quantum magnet with antiferromagnetic dimers of S=1/2 moments on a quasi-2D square lattice. We have investigated its spin dynamics by inelastic neutron scattering experiments on single crystals with an energy resolution considerably higher than in an earlier study. We observe multiple magnon modes, indicating clearly the presence of magnetically inequivalent dimer sites. The more complex spin Hamiltonian revealed in our study leads to a distinct form of magnon Bose-Einstein condensate phase with a spatially modulated condensate amplitude.

8.
Nature ; 441(7093): 617-20, 2006 Jun 01.
Artigo em Inglês | MEDLINE | ID: mdl-16738655

RESUMO

Competition between electronic ground states near a quantum critical point (QCP)--the location of a zero-temperature phase transition driven solely by quantum-mechanical fluctuations--is expected to lead to unconventional behaviour in low-dimensional systems. New electronic phases of matter have been predicted to occur in the vicinity of a QCP by two-dimensional theories, and explanations based on these ideas have been proposed for significant unsolved problems in condensed-matter physics, such as non-Fermi-liquid behaviour and high-temperature superconductivity. But the real materials to which these ideas have been applied are usually rendered three-dimensional by a finite electronic coupling between their component layers; a two-dimensional QCP has not been experimentally observed in any bulk three-dimensional system, and mechanisms for dimensional reduction have remained the subject of theoretical conjecture. Here we show evidence that the Bose-Einstein condensate of spin triplets in the three-dimensional Mott insulator BaCuSi2O6 (refs 12-16) provides an experimentally verifiable example of dimensional reduction at a QCP. The interplay of correlations on a geometrically frustrated lattice causes the individual two-dimensional layers of spin-(1/2) Cu2+ pairs (spin dimers) to become decoupled at the QCP, giving rise to a two-dimensional QCP characterized by linear power law scaling distinctly different from that of its three-dimensional counterpart. Thus the very notion of dimensionality can be said to acquire an 'emergent' nature: although the individual particles move on a three-dimensional lattice, their collective behaviour occurs in lower-dimensional space.

9.
Phys Rev Lett ; 96(18): 189703; author reply 189704, 2006 May 12.
Artigo em Inglês | MEDLINE | ID: mdl-16712410
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