Estimation with Ultimate Quantum Precision of the Transverse Displacement between Two Photons via Two-Photon Interference Sampling Measurements.

We present a quantum sensing scheme achieving the ultimate quantum sensitivity in the estimation of the transverse displacement between two photons interfering at a balanced beam splitter, based on transverse-momentum sampling measurements at the output. This scheme can possibly lead to enhanced high-precision nanoscopic techniques, such as superresolved single-molecule localization microscopy with quantum dots, by circumventing the requirements in standard direct imaging of camera resolution at the diffraction limit, and of highly magnifying objectives. Interestingly, we show that our interferometric technique achieves the ultimate spatial precision in nature irrespectively of the overlap of the two displaced photonic wave packets, while its precision is only reduced of a constant factor for photons differing in any nonspatial degrees of freedom. This opens a new research paradigm based on the interface between spatially resolved quantum interference and quantum-enhanced spatial sensitivity.

Fluorescence lifetime Hong-Ou-Mandel sensing.

Fluorescence Lifetime Imaging Microscopy in the time domain is typically performed by recording the arrival time of photons either by using electronic time tagging or a gated detector. As such the temporal resolution is limited by the performance of the electronics to 100's of picoseconds. Here, we demonstrate a fluorescence lifetime measurement technique based on photon-bunching statistics with a resolution that is only dependent on the duration of the reference photon or laser pulse, which can readily reach the 1-0.1 picosecond timescale. A range of fluorescent dyes having lifetimes spanning from 1.6 to 7 picoseconds have been here measured with only ~1 s measurement duration. We corroborate the effectiveness of the technique by measuring the Newtonian viscosity of glycerol/water mixtures by means of a molecular rotor having over an order of magnitude variability in lifetime, thus introducing a new method for contact-free nanorheology. Accessing fluorescence lifetime information at such high temporal resolution opens a doorway for a wide range of fluorescent markers to be adopted for studying yet unexplored fast biological processes, as well as fundamental interactions such as lifetime shortening in resonant plasmonic devices.

Coherent Two-Photon LIDAR with Incoherent Light.

Coherent light detection and ranging (LIDAR) offers exceptional sensitivity and precision in measuring the distance of remote objects by employing first-order interference. However, the ranging capability of coherent LIDAR is principally constrained by the coherence time of the light source determined by the spectral bandwidth. Here, we introduce coherent two-photon LIDAR, which eliminates the range limitation of coherent LIDAR due to the coherence time. Our scheme capitalizes on the counterintuitive phenomenon of two-photon interference of thermal light, in which the second-order interference fringe remains impervious to the short coherence time of the light source determined by the spectral bandwidth. By combining this feature with transverse two-photon interference of thermal light, we demonstrate distance ranging beyond the coherence time without relying on time-domain interference fringes. Moreover, we show that our coherent two-photon LIDAR scheme is robust to turbulence and ambient noise. This work opens up novel applications of two-photon correlation in classical light.

Estimation with Heisenberg-Scaling Sensitivity of a Single Parameter Distributed in an Arbitrary Linear Optical Network.

Quantum sensing and quantum metrology propose schemes for the estimation of physical properties, such as lengths, time intervals, and temperatures, achieving enhanced levels of precision beyond the possibilities of classical strategies. However, such an enhanced sensitivity usually comes at a price: the use of probes in highly fragile states, the need to adaptively optimise the estimation schemes to the value of the unknown property we want to estimate, and the limited working range, are some examples of challenges which prevent quantum sensing protocols to be practical for applications. This work reviews two feasible estimation schemes which address these challenges, employing easily realisable resources, i.e., squeezed light, and achieve the desired quantum enhancement of the precision, namely the Heisenberg-scaling sensitivity. In more detail, it is here shown how to overcome, in the estimation of any parameter affecting in a distributed manner multiple components of an arbitrary M-channel linear optical network, the need to iteratively optimise the network. In particular, we show that this is possible with a single-step adaptation of the network based only on a prior knowledge of the parameter achievable through a "classical" shot-noise limited estimation strategy. Furthermore, homodyne measurements with only one detector allow us to achieve Heisenberg-limited estimation of the parameter. We further demonstrate that one can avoid the use of any auxiliary network at the price of simultaneously employing multiple detectors.

Interference of Temporally Distinguishable Photons Using Frequency-Resolved Detection.

We demonstrate quantum interference of three photons that are distinguishable in time by resolving them in the conjugate parameter frequency. We show that the multiphoton interference pattern in our setup can be manipulated by tuning the relative delays between the photons, without the need for reconfiguring the optical network. Furthermore, we observe that the symmetries of our optical network and the spectral amplitude of the input photons are manifested in the interference pattern. We also demonstrate time-reversed Hong-Ou-Mandel-like interference in the spectral correlations using time-bin entangled photon pairs. By adding a time-varying dispersion using a phase modulator, our setup can be used to realize dynamically reconfigurable and scalable boson sampling in the time domain as well as frequency-resolved multiboson correlation sampling.

Hectometer Revivals of Quantum Interference.

Cavity-enhanced single photon sources exhibit mode-locked biphoton states with comblike correlation functions. Our ultrabright source additionally emits single photon pairs as well as two-photon NOON states, dividing the output into an even and an odd comb, respectively. With even-comb photons we demonstrate revivals of the typical nonclassical Hong-Ou-Mandel interference up to the 84th dip, corresponding to a path length difference exceeding 100 m. With odd-comb photons we observe single photon interference fringes modulated over twice the displacement range of the Hong-Ou-Mandel interference.

Experimental Time-Resolved Interference with Multiple Photons of Different Colors.

Interference of multiple photons via a linear-optical network has profound applications for quantum foundation, quantum metrology, and quantum computation. Particularly, a boson sampling experiment with a moderate number of photons becomes intractable even for the most powerful classical computers. Scaling up from small-scale experiments requires highly indistinguishable single photons, which may be prohibited for many physical systems. Here we report a time-resolved multiphoton interference experiment by using photons not overlapping in their frequency spectra from three atomic-ensemble quantum memories. Time-resolved measurement enables us to observe nonclassical multiphoton correlation landscapes, which agree well with theoretical calculations. Symmetries in the landscapes are identified to reflect symmetries of the optical network. Our experiment can be further extended to realize boson sampling with many photons and plenty of modes, which thus may provide a route towards quantum supremacy with nonidentical photons.

Characterization of two distant double-slits by chaotic light second-order interference.

We present the experimental characterization of two distant double-slit masks illuminated by chaotic light, in the absence of first-order imaging and interference. The scheme exploits second-order interference of light propagating through two indistinguishable pairs of disjoint optical paths passing through the masks of interest. The proposed technique leads to a deeper understanding of biphoton interference and coherence, and opens the way to the development of novel schemes for retrieving information on the relative position and the spatial structure of distant objects, which is of interest in remote sensing, biomedical imaging, as well as monitoring of laser ablation, when first-order imaging and interference are not feasible.

Spatial interference between pairs of disjoint optical paths with a single chaotic source.

We demonstrate a novel second-order spatial interference effect between two indistinguishable pairs of disjoint optical paths from a single chaotic source. Beside providing a deeper understanding of the physics of multi-photon interference and coherence, the effect enables retrieving information on both the spatial structure and the relative position of two distant double-pinhole masks, in the absence of first order coherence. We also demonstrate the exploitation of the phenomenon for simulating quantum logic gates, including a controlled-NOT gate operation.

Second-Order Temporal Interference with Thermal Light: Interference beyond the Coherence Time.

We report the observation of a counterintuitive phenomenon in multipath correlation interferometry with thermal light. The intensity correlation between the outputs of two unbalanced Mach-Zehnder interferometers (UMZIs) with two classically correlated beams of thermal light at the input exhibits genuine second-order interference with the visibility of 1/3. Surprisingly, the second-order interference does not degrade at all no matter how much the path length difference in each UMZI is increased beyond the coherence length of the thermal light. Moreover, the second-order interference is dependent on the difference of the UMZI phases. These results differ substantially from those of the entangled-photon Franson interferometer, which exhibits two-photon interference dependent on the sum of the UMZI phases and the interference vanishes as the path length difference in each UMZI exceeds the coherence length of the pump laser. Our work offers deeper insight into the interplay between interference and coherence in multiphoton interferometry.

Experimental controlled-NOT gate simulation with thermal light.

We report a recent experimental simulation of a controlled-NOT gate operation based on polarization correlation measurements of thermal fields in photon-number fluctuations. The interference between pairs of correlated paths at the very heart of these experiments has the potential for the simulation of correlations between a larger number of qubits.

From the Physics to the Computational Complexity of Multiboson Correlation Interference.

We demonstrate how the physics of multiboson correlation interference leads to the computational complexity of linear optical interferometers based on correlation measurements in the degrees of freedom of the input bosons. In particular, we address the task of multiboson correlation sampling (MBCS) from the probability distribution associated with polarization- and time-resolved detections at the output of random linear optical networks. We show that the MBCS problem is fundamentally hard to solve classically even for nonidentical input photons, regardless of the color of the photons, making it also very appealing from an experimental point of view. These results fully manifest the quantum computational supremacy inherent to the fundamental nature of quantum interference.

Multiboson Correlation Interferometry with Arbitrary Single-Photon Pure States.

We provide a compact full description of multiboson correlation measurements of arbitrary order N in passive linear interferometers with arbitrary input single-photon pure states. This allows us to physically analyze the novel problem of multiboson correlation sampling at the output of random linear interferometers. Our results also describe general multiboson correlation landscapes for an arbitrary number of input single photons and arbitrary interferometers. In particular, we use two different schemes to demonstrate, respectively, arbitrary-order quantum beat interference and 100% visibility entanglement correlations even for input photons distinguishable in their frequencies.