An improved surgical procedure to establish a gastroesophageal reflux model with a high incidence of Barrett's esophagus in rats.

Barrett's esophagus (BE) is a complication of gastroesophageal reflux disease and is a precursor lesion of esophageal adenocarcinoma. In existing BE models, the incidence of BE is typically low and induction is usually time consuming. In the present study, a gastroesophageal reflux model with a high incidence of BE in rats. Rats were divided into a model group and a sham operation group, and anesthetized with an inhalation anesthesia machine. Stomach-jejunal anastomosis (SJA) and esophagus-jejunal anastomosis (EJA) were simultaneously performed in the model group. The distance between the Treitz ligament and the gastro-jejunal anastomosis was shortened to 3 cm. The distance between the SJA and the EJA was prolonged to 1-1.5 cm. However, 15/40 rats in the model group succumbed to post-surgical complications (mortality rate was 37.5%). The weight of surviving rats in the model group was significantly lower compared with the sham group rats post-surgery. Erosions and ulcers were common of the surviving rats in the model group, with an incidence of 80% (20/25). Squamous cell dysplasia was identified in 40% (10/25) of rats in model group. The modified model was well established within 16 weeks. Notably, the modified surgical procedure used enhanced the incidence of BE in rats from 47% in the EJGJ model (as establish by Zhang) to 100%. To conclude, this model can be used as a reliable animal model for basic research on BE.

Influence of Plasmonic Effect on the Upconversion Emission Characteristics of NaYF4 Hexagonal Microrods.

The influence of plasmonic effect on the upconversion emission characteristics of Yb3+-Er3+-Tm3+ tridoped ß-NaYF4 hexagonal microrods is studied. Upconversion spontaneous emission can be improved by 10 times if the microrod is deposited on an Ag-coated substrate. The enhancement is also dependent on the emission wavelength and the polarization of the excitation source. Furthermore, upconversion lasing is supported by the geometry of the microrods via the formation of whispering gallery modes. The corresponding excitation threshold can also be reduced by 50% through the influence of plasmonic effect, the coupling between the whispering gallery modes and the surface plasmonic resonance modes.

Spiniform phase-encoded metagratings entangling arbitrary rational-order orbital angular momentum.

Quantum entanglements between integer-order and fractional-order orbital angular momentums (OAMs) have been previously discussed. However, the entangled nature of arbitrary rational-order OAM has long been considered a myth due to the absence of an effective strategy for generating arbitrary rational-order OAM beams. Therefore, we report a single metadevice comprising a bilaterally symmetric grating with an aperture, creating optical beams with dynamically controllable OAM values that are continuously varying over a rational range. Due to its encoded spiniform phase, this novel metagrating enables the production of an average OAM that can be increased without a theoretical limit by embracing distributed singularities, which differs significantly from the classic method of stacking phase singularities using fork gratings. This new method makes it possible to probe the unexplored niche of quantum entanglement between arbitrarily defined OAMs in light, which could lead to the complex manipulation of microparticles, high-dimensional quantum entanglement and optical communication. We show that quantum coincidence based on rational-order OAM-superposition states could give rise to low cross-talks between two different states that have no significant overlap in their spiral spectra. Additionally, future applications in quantum communication and optical micromanipulation may be found.

All-Optical Chirality-Sensitive Sorting via Reversible Lateral Forces in Interference Fields.

Separating substances by their chirality faces great challenges as well as opportunities in chemistry and biology. In this study, we propose an all-optical solution for passive sorting of chiral objects using chirality-dependent lateral optical forces induced by judiciously interfered fields. First, we investigate the optical forces when the chiral objects are situated in the interference field formed by two plane waves with arbitrary polarization states. When the plane waves are either linearly or circularly polarized, nonzero lateral forces are found at the particle's trapping positions, making such sideways motions observable. Although the lateral forces have different magnitudes on particles with different chirality, their directions are the same for opposite handedness particles, rendering it difficult to separate the chiral particles. We further solve the sorting problem by investigating more complicated polarization states. Finally, we achieve the chiral-selective separation by illuminating only one beam toward the chiral substance situated at an interface between two media, taking advantage of the native interference between the incident and reflective beams at the interface. Our study provides a robust and insightful approach to sort chiral substances and biomolecules with plausible optical setups.

Polarization-Independent Multiple Fano Resonances in Plasmonic Nonamers for Multimode-Matching Enhanced Multiband Second-Harmonic Generation.

Plasmonic oligomers composed of metallic nanoparticles are one class of the most promising platforms for generating Fano resonances with unprecedented optical properties for enhancing various linear and nonlinear optical processes. For efficient generation of second-harmonic emissions at multiple wavelength bands, it is critical to design a plasmonic oligomer concurrently having multiple Fano resonances spectrally matching the fundamental excitation wavelengths and multiple plasmon resonance modes coinciding with the harmonic wavelengths. Thus far, the realization of such a plasmonic oligomer remains a challenge. This study demonstrates both theoretically and experimentally that a plasmonic nonamer consisting of a gold nanocross surrounded by eight nanorods simultaneously sustains multiple polarization-independent Fano resonances in the near-infrared region and several higher-order plasmon resonances in the visible spectrum. Due to coherent amplification of the nonlinear excitation sources by the Fano resonances and efficient scattering-enhanced outcoupling by the higher-order modes, the second-harmonic emission of the nonamer is significantly increased at multiple spectral bands, and their spectral positions and radiation patterns can be flexibly manipulated by easily tuning the length of the surrounding nanorods in the nonamer. These results provide us with important implications for realizing ultrafast multichannel nonlinear optoelectronic devices.

Fluid-enabled significant enhancement and active tuning of magnetic resonances in free-standing plasmonic metamaterials.

We report significantly enhanced magnetic resonance by fluid infiltration in a free-standing metamaterial that consists of metal-dielectric-metal films on an ultrathin Si3N4 membrane patterned with etched through nanohole arrays. When different fluids are drop-casted on the structure, the magnetic resonance has high sensitivities of 282 nm per RIU in peak shift and 12% per RIU in peak intensity change, whereas the electric resonance has nearly no changes. This work shows a promising way of using fluids to actively tune the magnetic resonance of metamaterial structures by combining with micro/nano-fluidic technologies.

Atomic layer deposition of a MoS2 film.

A mono- to multilayer thick MoS2 film has been grown by using the atomic layer deposition (ALD) technique at 300 °C on a sapphire wafer. ALD provides precise control of the MoS2 film thickness due to pulsed introduction of the reactants and self-limiting reactions of MoCl5 and H2S. A post-deposition annealing of the ALD-deposited monolayer film improves the crystallinity of the film, which is evident from the presence of triangle-shaped crystals that exhibit strong photoluminescence in the visible range.

Sub-30 nm thick plasmonic films and structures with ultralow loss.

We report an alternative method of producing sub-30 nm thick silver films and structures with ultralow loss using gas cluster ion beam irradiation (GCIB). We have direct evidence showing that scattering from grain boundaries and voids rather than surface roughness are the main mechanisms for the increase in loss with reducing thickness. Using GCIB irradiation, we demonstrate the ability to reduce these scattering effects simultaneously through nanoscale surface smoothing, increase in grain width and lower percolation threshold. Significant improvement in electrical and optical properties by up to 4 times is obtained, before deviation from bulk silver properties starts to occur at 12 nm. We show that this is an enabling technology that can be applied post fabrication to metallic films or lithographically patterned nanostructures for enhanced plasmonic performance, especially in the ultrathin regime.

Correction: Atomic layer deposition of a MoS2 film.

Correction for 'Atomic layer deposition of a MoS2 film' by Lee Kheng Tan et al., Nanoscale, 2014, 6, 10584-10588.

Holographically formed, acoustically switchable gratings based on polymer-dispersed liquid crystals.

We report holographic polymer-dispersed liquid crystal (H-PDLC) gratings driven by surface acoustic waves (SAWs). Our experiments show that upon applying SAWs, the H-PDLC grating exhibited switchable properties: The diffraction of the H-PDLC grating decreased, whereas the transmission increased. This acoustically switchable behavior is due to the acoustic streaming-induced realignment of liquid crystals as well as absorption-resulted thermal diffusion. Such SAW-driven H-PDLC gratings are potentially useful in many photonic applications, such as optical switches, spatial light modulators, and switchable add/drop filters.

Ultrathin multi-band planar metamaterial absorber based on standing wave resonances.

We present a planar waveguide model and a mechanism based on standing wave resonances to interpret the unity absorptions of ultrathin planar metamaterial absorbers. The analytical model predicts that the available absorption peaks of the absorber are corresponding to the fundamental mode and only its odd harmonic modes of the standing wave. The model is in good agreement with numerical simulation and can explain the main features observed in typical ultrathin planar metamaterial absorbers. Based on this model, ultrathin planar metamaterial absorbers with multi-band absorptions at desired frequencies can be easily designed.

Metal-assisted photonic mode for ultrasmall bending with long propagation length at visible wavelengths.

In this work, we investigate the use of metal-assisted photonic guiding in a polymer-metal waveguide as an alternative approach for high density photonic integration at visible wavelengths. We demonstrate high confinement and long propagation length in sub-wavelength dimensions down to 300nm × 200nm using leakage radiation microscopy at a wavelength of 632.8 nm. Simulations using the finite element method (FEM) show that the optimum dimension that gives good confinement and propagation length is similar to that of the predicted plasmonic mode supported in the same waveguide. Under such optimum conditions, the metal-assisted photonic mode shows a five times longer propagation length and higher transmission efficiency for all 90° bending radius down to 1 µm compared to the plasmonic mode.

Nanoimprinted ultrafine line and space nanogratings for liquid crystal alignment.

Ultrafine 50 nm line and space nanogratings were fabricated using nanoimprint lithography, and were further used as an alignment layer for liquid crystals. The surface morphologies of the nanogratings were characterized and their surface energies were estimated through the measurement of the contact angles for two different liquids. Experimental results show that the surface energies of the nanogratings are anisotropic: the surface free energy towards the direction parallel to the grating lines is higher than that in the direction perpendicular to the grating lines. Electro-optical characteristics were tested from a twisted nematic liquid crystal cell, which was assembled using two identical nanogratings. Experimental results show that such a kind of nanograting is promising as an alternative to the conventional rubbing process for liquid crystal alignment.

Enhanced photoelectrochemical performance of bridged ZnO nanorod arrays grown on V-grooved structure.

Bridged ZnO nanorod arrays on a V-grooved Si(100) substrate were used as the photoanode of a photoelectrochemical (PEC) cell for water splitting. Photolithography followed by reactive ion etching was employed to create a V-grooved structure on a Si substrate. ZnO nanorod arrays were grown via a hydrothermal method. The light trapping and PEC properties are greatly enhanced using the bridged ZnO nanorod arrays on a V-grooved Si substrate compared with those on a flat one. Increased short circuit photocurrent density (J(SC), 0.73 mA cm(-2)) and half-life time (1500 s) are achieved. This improved J(SC) and half-life time are 4 times and 10 times, respectively, higher than those of the ZnO nanorod arrays grown on a flat substrate. The overall PEC cell performance improvement for the V-groove grown ZnO array is attributed to the reduced light reflection and enhanced light trapping effect. Moreover, V-groove ZnO showed stronger adhesion between ZnO nanorod arrays and the substrate.

Distortion of terahertz signals due to imperfect synchronization with chirped probe pulses.

Terahertz (THz) signals measured by means of the spectral-encoding technique with different temporal discrepancies between probe pulses and THz signals are investigated. It is found that imperfect synchronization between the chirped probe and THz pulses induce a distortion and this distortion affects significantly the retrieved THz spectrum if the temporal discrepancy is large. The distortion becomes more prominent if the probe pulse length is less than the optimal chirped probe pulse duration. A simple approach is proposed to realize the synchronization and minimize the distortion. THz signals from a high-voltage-biased air plasma filament are measured with this approach and distortion similar to the simulation results is observed.

Colloidal woodpile structure: three-dimensional photonic crystal with a dual periodicity.

With planar photolithography and self-assembly techniques, multilayer colloidal crystals with a woodpile structure were fabricated. They represent a new kind of photonic crystals, that is, three-dimensional (3D) photonic crystals with a dual periodicity; one comes from the face-centered cubic (fcc) structure within the colloidal crystal strips and the other one results from the periodic arrangement of the colloidal crystal strips.