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1.
Phys Rev Lett ; 130(23): 233602, 2023 Jun 09.
Artigo em Inglês | MEDLINE | ID: mdl-37354413

RESUMO

We experimentally and theoretically study a driven hybrid circuit quantum electrodynamics (cQED) system beyond the dispersive coupling regime. Treating the cavity as part of the driven system, we develop a theory applicable to such strongly coupled and to multiqubit systems. The fringes measured for a single driven double quantum dot (DQD)-cavity setting and the enlarged splittings of the hybrid Floquet states in the presence of a second DQD are well reproduced with our model. This opens a path to study Floquet states of multiqubit systems with arbitrarily strong coupling and reveals a new perspective for understanding strongly driven hybrid systems.

2.
Nano Lett ; 23(10): 4176-4182, 2023 May 24.
Artigo em Inglês | MEDLINE | ID: mdl-37133858

RESUMO

We fabricate and characterize a hybrid quantum device that consists of five gate-defined double quantum dots (DQDs) and a high-impedance NbTiN transmission resonator. The controllable interactions between DQDs and the resonator are spectroscopically explored by measuring the microwave transmission through the resonator in the detuning parameter space. Utilizing the high tunability of the system parameters and the high cooperativity (Ctotal > 17.6) interaction between the qubit ensemble and the resonator, we tune the charge-photon coupling and observe the collective microwave response changing from linear to nonlinear. Our results present the maximum number of DQDs coupled to a resonator and manifest a potential platform for scaling up qubits and studying collective quantum effects in semiconductor-superconductor hybrid cavity quantum electrodynamics systems.

3.
Chem Commun (Camb) ; 58(53): 7408-7411, 2022 Jun 30.
Artigo em Inglês | MEDLINE | ID: mdl-35695118

RESUMO

An azido pyridoxal derivative (PLAA) was developed as a protein azidolation reagent, with selectivity towards N-terminal glycine. Successful PLAA modification was achieved with small peptides, natural proteins and lab-expressed proteins under mild conditions, offering a unique method for post-synthesis site-specific azidolation of a peptide or protein.


Assuntos
Proteínas , Piridoxal
4.
Sci Bull (Beijing) ; 66(4): 332-338, 2021 Feb 26.
Artigo em Inglês | MEDLINE | ID: mdl-36654412

RESUMO

We develop a new spectroscopic method to quickly and intuitively characterize the coupling of two microwave-photon-coupled semiconductor qubits via a high-impedance resonator. Highly distinctive and unique geometric patterns are revealed as we tune the qubit tunnel couplings relative to the frequency of the mediating photons. These patterns are in excellent agreement with a simulation using the Tavis-Cummings model, and allow us to readily identify different parameter regimes for both qubits in the detuning space. This method could potentially be an important component in the overall spectroscopic toolbox for quickly characterizing certain collective properties of multiple cavity quantum electrodynamics (QED) coupled qubits.

5.
Sci Bull (Beijing) ; 62(10): 712-716, 2017 May 30.
Artigo em Inglês | MEDLINE | ID: mdl-36659443

RESUMO

We investigate a spin-to-charge conversion mechanism which maps the spin singlet and triplet states to two charge states differing by one electron mediated by an intermediate metastable charge state. This mechanism allows us to observe fringes in the spin-unblocked region beyond the triplet transition line in the measurement of the exchange oscillations between singlet and triplet states in a four-electron double quantum dot. Moreover, these fringes are amplified and π-phase shifted, compared with those in the spin blockade region. Unlike the signal enhancement mechanism reported before which produces similar effects, this mechanism only requires one dot coupling to the lead, which is a commonly encountered case especially in imperfect devices. Besides, the crucial tunnel rate asymmetry is provided by the dependence on spin state, not by the asymmetric couplings to the leads. We also design a scheme to control the amplification process, which enables us to extract the relevant time parameters. This mechanism will have potential applications in future investigations of spin qubits.

6.
Phys Rev Lett ; 116(8): 086801, 2016 Feb 26.
Artigo em Inglês | MEDLINE | ID: mdl-26967435

RESUMO

We experimentally demonstrate a tunable hybrid qubit in a five-electron GaAs double quantum dot. The qubit is encoded in the (1,4) charge regime of the double dot and can be manipulated completely electrically. More importantly, dot anharmonicity leads to quasiparallel energy levels and a new anticrossing, which help preserve quantum coherence of the qubit and yield a useful working point. We have performed Larmor precession and Ramsey fringe experiments near the new working point and find that the qubit decoherence time is significantly improved over a charge qubit. This work shows a new way to encode a semiconductor qubit that is controllable and coherent.

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