General design formalism for highly efficient flat optics for broadband applications.

The use of flat diffractive optical elements (DOEs) for broadband applications, e.g. conventional optical systems, requires DOEs that maintain high efficiencies across the required range of wavelengths, angles of incidence, and grating periods. Here we introduce a general framework for how dispersion engineering can be used to design DOEs that fulfill these requirements and use our approach to determine design rules for broadband DOEs. Our analysis shows that the key to making échelette-type gratings (EGs) suitable for broadband optical systems is the development of new optical materials with specific uncommon dispersion properties. Subsequently, we use our framework to design a representative range of prototype EGs, which allows us to link the specifications of an optical system to the requirements on the EGs' materials. Finally, we show that our design rules apply to all DOEs based on propagation delays including GRIN DOEs and metagratings. Our design rules therefore guide the way towards unlocking the full potential of DOEs for different kinds of broadband applications.

Photo-excited dynamics in the excitonic insulator Ta2NiSe5.

The excitonic insulator is an intriguing correlated electron phase formed of condensed excitons. A promising candidate is the small band gap semiconductor Ta2NiSe5. Here we investigate the quasiparticle and coherent phonon dynamics in Ta2NiSe5 in a time resolved pump probe experiment. Using the models originally developed by Kabanov et al for superconductors (Kabanov et al 1999 Phys. Rev. B 59 1497), we show that the material's intrinsic gap can be described as almost temperature independent for temperatures up to about 250 K to 275 K. This behavior supports the existence of the excitonic insulator state in Ta2NiSe5. The onset of an additional temperature dependent component to the gap above these temperatures suggests that the material is located in the BEC-BCS crossover regime. Furthermore, we show that this state is very stable against strong photoexcitation, which reveals that the free charge carriers are unable to effectively screen the attractive Coulomb interaction between electrons and holes, likely due to the quasi 1D structure of Ta2NiSe5.

Coherent order parameter oscillations in the ground state of the excitonic insulator Ta2NiSe5.

The excitonic insulator is an intriguing electronic phase of condensed excitons. A prominent candidate is the small bandgap semiconductor Ta2NiSe5, in which excitons are believed to undergo a Bose-Einstein condensation-like transition. However, direct experimental evidence for the existence of a coherent condensate in this material is still missing. A direct fingerprint of such a state would be the observation of its collective modes, which are equivalent to the Higgs and Goldstone modes in superconductors. We report evidence for the existence of a coherent amplitude response in the excitonic insulator phase of Ta2NiSe5. Using nonlinear excitations with short laser pulses, we identify a phonon-coupled state of the condensate that can be understood as a novel amplitude mode. The condensate density contribution substantiates the picture of an electronically driven phase transition and characterizes the transient order parameter of the excitonic insulator as a function of temperature and excitation density.

1.9 octave supercontinuum generation in a As2S3 step-index fiber driven by mid-IR OPCPA.

Using a 3.1-µm optical parametric chirped-pulse amplifier (OPCPA), we generate a supercontinuum in a step-index chalcogenide fiber that spans from 1.6 to 5.9 µm at the -20 dB points. The rugged step-index geometry allows for long-term operation, while the spectral bandwidth is limited by the transmission of the As2S3 fiber.