Ferromagnetic Resonance with Magnetic Phase Selectivity by Means of Resonant Elastic X-Ray Scattering on a Chiral Magnet.

Cubic chiral magnets, such as Cu_{2}OSeO_{3}, exhibit a variety of noncollinear spin textures, including a trigonal lattice of spin whirls, the so-called skyrmions. Using magnetic resonant elastic x-ray scattering (REXS) on a crystalline Bragg peak and its magnetic satellites while exciting the sample with magnetic fields at gigahertz frequencies, we probe the ferromagnetic resonance (FMR) modes of these spin textures by means of the scattered intensity. Most notably, the three eigenmodes of the skyrmion lattice are detected with large sensitivity. As this novel technique, which we label REXS FMR, is carried out at distinct positions in reciprocal space, it allows us to distinguish contributions originating from different magnetic states, providing information on the precise character, weight, and mode mixing as a prerequisite of tailored excitations for applications.

Magneto-optical properties of Au upon the injection of hot spin-polarized electrons across Fe/Au(0 0 1) interfaces.

We demonstrate a novel method for the excitation of sizable magneto-optical effects in Au by means of the laser-induced injection of hot spin-polarized electrons in Au/Fe/MgO(0 0 1) heterostructures. It is based on the energy- and spin-dependent electron transmittance of Fe/Au interface which acts as a spin filter for non-thermalized electrons optically excited in Fe. We show that after crossing the interface, majority electrons propagate through the Au layer with the velocity on the order of 1 nm fs-1 (close to the Fermi velocity) and the decay length on the order of 100 nm. Featuring ultrafast functionality and requiring no strong external magnetic fields, spin injection results in a distinct magneto-optical response of Au. We develop a formalism based on the phase of the transient complex MOKE response and demonstrate its robustness in a plethora of experimental and theoretical MOKE studies on Au, including our ab initio calculations. Our work introduces a flexible tool to manipulate magneto-optical properties of metals on the femtosecond timescale that holds high potential for active magneto-photonics, plasmonics, and spintronics.

Terahertz-Driven Nonlinear Spin Response of Antiferromagnetic Nickel Oxide.

Terahertz magnetic fields with amplitudes of up to 0.4 Tesla drive magnon resonances in nickel oxide while the induced dynamics is recorded by femtosecond magneto-optical probing. We observe distinct spin-mediated optical nonlinearities, including oscillations at the second harmonic of the 1 THz magnon mode. The latter originate from coherent dynamics of the longitudinal component of the antiferromagnetic order parameter, which are probed by magneto-optical effects of second order in the spin deflection. These observations allow us to dynamically disentangle electronic from lattice-related contributions to magnetic linear birefringence and dichroism-information so far only accessible by ultrafast THz spin control. The nonlinearities discussed here foreshadow physics that will become essential in future subcycle spin switching.

Extremely Nonperturbative Nonlinearities in GaAs Driven by Atomically Strong Terahertz Fields in Gold Metamaterials.

Terahertz near fields of gold metamaterials resonant at a frequency of 0.88 THz allow us to enter an extreme limit of nonperturbative ultrafast terahertz electronics: Fields reaching a ponderomotive energy in the keV range are exploited to drive nondestructive, quasistatic interband tunneling and impact ionization in undoped bulk GaAs, injecting electron-hole plasmas with densities in excess of 10^{19} cm^{-3}. This process causes bright luminescence at energies up to 0.5 eV above the band gap and induces a complete switch-off of the metamaterial resonance accompanied by self-amplitude-modulation of transmitted few-cycle terahertz transients. Our results pave the way towards highly nonlinear terahertz optics and optoelectronic nanocircuitry with subpicosecond switching times.

Proximity induced enhancement of the Curie temperature in hybrid spin injection devices.

We investigate the increase of the Curie temperature T(C) in a lateral spin injection geometry where the ferromagnetic (Ga,Mn)As injector and detector contacts are capped by a thin iron film. Because of interlayer coupling between Fe and (Ga,Mn)As T(C) gets enhanced by nearly 100% for the thinnest (Ga,Mn)As films. The use of the proximity effect might pave the way for practical implementation of spintronic devices.

Anisotropic propagation and damping of spin waves in a nanopatterned antidot lattice.

All-electrical spin-wave spectroscopy, Brillouin light scattering, as well as the magneto-optical Kerr effect are combined to study spin-wave propagation through a magnetic antidot lattice nanopatterned into a Ni(80)Fe(20) thin film. The propagation velocities and, in particular, the relaxation are found to depend characteristically on the applied in-plane magnetic field. We explain the observed anisotropies by magnetic field-controlled spin-wave guiding in a network of interconnected nanowires which takes place over distances of up to 20 µm.

Damping by slow relaxing rare earth impurities in Ni80Fe20.

Doping Ni80Fe20 by heavy rare earth atoms alters the magnetic relaxation properties of this material drastically. We show that this effect can be well explained by the slow relaxing impurity mechanism. This process is a consequence of the anisotropy of the on site exchange interaction between the 4f magnetic moments and the conduction band. As expected from this model the magnitude of the damping effect scales with the anisotropy of the exchange interaction and increases by an order of magnitude at low temperatures. In addition, our measurements allow us to determine the relaxation time of the 4f electrons as a function of temperature.

Laser-induced magnetization dynamics of lanthanide-doped permalloy thin films.

We investigate the effect of Ho, Dy, Tb, and Gd impurities on the femtosecond laser-induced magnetization dynamics of thin Permalloy films using the time-resolved magneto-optical Kerr effect. Varying the amount of Ho, Dy, Tb content from 0% to 8%, we observe a gradual change of the characteristic demagnetization time constant from approximately 60 to approximately 150 fs. In contrast, Gd concentrations up to 15% do not influence the time scale of the initial photoinduced magnetization loss. We propose a demagnetization mechanism that relies on strong magnetic inertia of the rare-earth dopant which stabilizes the ferrimagnetic ordering and thereby delays the demagnetization.

Evidence for a magnetic proximity effect up to room temperature at Fe/(Ga, Mn)As interfaces.

We report x-ray magnetic circular dichroism and superconducting quantum interference device magnetometry experiments to study magnetic order and coupling in thin Fe/(Ga, Mn)As(100) films. We observe induced magnetic order in the (Ga, Mn)As layer that extends over more than 2 nm, even at room temperature. We find spectroscopic evidences of a hybridized d configuration of Mn atoms in Fe/(Ga, Mn)As, with negligible Mn diffusion and/or MnFe intermixing. We show by experiment as well as by theory that the magnetic moment of the Mn ions couples antiparallel to the moment of the Fe overlayer.

Magnetization dynamics due to pure spin currents in magnetic double layers.

The magnetization dynamics in magnetic double layers is affected by spin-pump and spin-sink effects. So far, only the spin pumping and its effect on the magnetic damping has been studied. However, due to conservation of angular momentum this spin current also leads to magnetic excitation of the layer dissipating this angular momentum. In this Letter we use time resolved magneto-optic Kerr effect to directly show the excitation due to the pure spin current. In particular, we observe magnetization dynamics due to transfer of angular momentum in magnetic double layers. In contrast to other experiments where a spin polarized charge current is passed through a nanomagnet, the effects discussed in this Letter are based on pure spin currents without net transfer of electric charge.

Dissipation of spin angular momentum in magnetic switching.

Applying one ultrashort magnetic field pulse, we observe up to 10 precessional switches of the magnetization direction in single crystalline Fe films of 10 and 15 atomic layers. We find that the rate at which angular momentum is dissipated in uniform large angle spin precession increases with time and film thickness, surpassing the intrinsic ferromagnetic resonance spin lattice relaxation of Fe by nearly an order of magnitude.

Time resolved magnetization dynamics of ultrathin Fe(001) films: spin-pumping and two-magnon scattering.

The time-resolved magnetic response of ultrathin epitaxial Fe(001) films grown on GaAs(001) and covered by Au, Pd, and Cr capping layers was investigated by time and spatially resolved Kerr effect measurements. The magnetization was excited by an in-plane magnetic field pulse using the transient internal field generated at a Schottky barrier while the wavelength of the excitation (resonant mode) was roughly 4 microm. Each of the three cap layers affected the spin relaxation in a unique way. Au cap layers resulted in the bulk Gilbert damping of the Fe film. Pd cap layers caused an additional Gilbert damping due to spin-pump or spin-sink effects. Cr cap layers lead to a strong extrinsic damping which can be described by two-magnon scattering. In this case the strength of the extrinsic damping can be controlled by a field induced shift of the spin wave manifold with respect to the excited k vector.

Gilbert damping in single and multilayer ultrathin films: role of interfaces in nonlocal spin dynamics.

Unique features of the Gilbert damping in magnetic multilayers were investigated by ferromagnetic resonance (FMR) using magnetic single and double layer structures prepared by molecular beam epitaxy. The FMR linewidth for the Fe films in the double layer structures was larger than the FMR linewidth in the single Fe films having the same thickness. The additional FMR linewidth scaled inversely with the film thickness, and increased linearly with increasing microwave frequency. These results demonstrate that a transfer of electron angular momentum between the magnetic layers leads to additional relaxation torques.