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1.
Phys Med Biol ; 69(3)2024 Feb 02.
Artigo em Inglês | MEDLINE | ID: mdl-38198704

RESUMO

Objective.The aim of this work is to investigate the dose rate dependence of thermoluminescence and optically stimulated luminescence detectors (TLDs and OSLDs) in a wide uniform ultra-high dose rate electron beam and demonstrate the potential use of TLDs and OSLDs to correct the ion recombination in air-filled ionization chambers. This study avoids previously reported complications related to the field size and homogeneity.Approach.Two types of OSLDs (BeO and Al2O3:C) and three types of TLDs (LiF:Mg,Ti, LiF:Mg,Cu,P, CaF2:Tm) were irradiated simultaneously in a uniform 16 MeV electron beam generated by a clinically decommissioned C-Arm LINAC, modified to deliver doses per pulse between 8.3 × 10-4Gy and 1.255 Gy, corresponding to instantaneous dose rates between 2 × 102Gy s-1and 3 × 105Gy s-1. A prototype ultra-thin parallel plate ionization chamber was employed as reference detector.Main results.Reproducible results were achieved both at conventional (standard deviation of the data <2%) and at the highest dose per pulse (standard deviation of the data <4%). No trend in the dose rate response of the TLDs and OSLDs was observed in the investigated dose per pulse range. The Al2O3:C OSLD was found to be the most precise detector, with a standard deviation of the data <2% at all investigated dose rates and dose levels.Significance.The dose rate independence of the investigated TLDs and OSLDs make them good candidates for dosimetry at ultra-high dose rates, at least up to 3 × 105Gy s-1. A dose rate independent method to measure the dose per pulse is proposed, which can be applied to characterize ultra-high dose rate electron beams and correct for ion recombination in ionization chambers.


Assuntos
Dosimetria por Luminescência Estimulada Opticamente , Elétrons , Radiometria/métodos , Luminescência
2.
Radiat Res ; 200(4): 357-365, 2023 10 01.
Artigo em Inglês | MEDLINE | ID: mdl-37702413

RESUMO

Significant past work has identified unexpected risks of central nervous system (CNS) exposure to the space radiation environment, where long-lasting functional decrements have been associated with multiple ion species delivered at low doses and dose rates. As shielding is the only established intervention capable of limiting exposure to the dangerous radiation fields in space, the recent discovery that pions, emanating from regions of enhanced shielding, can contribute significantly to the total absorbed dose on a deep space mission poses additional concerns. As a prerequisite to biological studies evaluating pion dose equivalents for various CNS exposure scenarios of mice, a careful dosimetric validation study is required. Within our ultimate goal of evaluating the functional consequences of defined pion exposures to CNS functionality, we report in this article the detailed dosimetry of the PiMI pion beam line at the Paul Scherrer Institute, which was developed in support of radiobiological experiments. Beam profiles and contamination of the beam by protons, electrons, positrons and muons were characterized prior to the mice irradiations. The dose to the back and top of the mice was measured using thermoluminescent dosimeters (TLD) and optically simulated luminescence (OSL) to cross-validate the dosimetry results. Geant4 Monte Carlo simulations of radiation exposure of a mouse phantom in water by charged pions were also performed to quantify the difference between the absorbed dose from the OSL and TLD and the absorbed dose to water, using a simple model of the mouse brain. The absorbed dose measured by the OSL dosimeters and TLDs agreed within 5-10%. A 30% difference between the measured absorbed dose and the dose calculated by Geant4 in the dosimeters was obtained, probably due to the approximated Monte Carlo configuration compared to the experiment. A difference of 15-20% between the calculated absorbed dose to water at a 5 mm depth and in the passive dosimeters was obtained, suggesting the need for a correction factor of the measured dose to obtain the absorbed dose in the mouse brain. Finally, based on the comparison of the experimental data and the Monte Carlo calculations, we consider the dose measurement to be accurate to within 15-20%.


Assuntos
Mésons , Animais , Camundongos , Radiometria/métodos , Prótons , Sistema Nervoso Central , Método de Monte Carlo , Dosimetria Termoluminescente/métodos , Água , Imagens de Fantasmas
3.
Phys Med Biol ; 68(14)2023 07 11.
Artigo em Inglês | MEDLINE | ID: mdl-37336230

RESUMO

Objective.This work aims at investigating the response of various thermally stimulated luminescence detectors (TLDs) and optically stimulated luminescence detectors (OSLDs) for dosimetry of ultra-high dose rate electron beams. The study was driven by the challenges of dosimetry at ultra-high dose rates and the importance of dosimetry for FLASH radiotherapy and radiobiology experiments.Approach.Three types of TLDs (LiF:Mg,Ti; LiF:Mg,Cu,P; CaF2:Tm) and one type of OSLD (Al2O3:C) were irradiated in a 15 MeV electron beam with instantaneous dose rates in the (1-324) kGy s-1range. Reference dosimetry was carried out with an integrating current transformer, which was calibrated in absorbed dose to water against a reference ionization chamber. Additionally, dose rate independent BeO OSLDs were employed as a reference. Beam non-uniformity was addressed using a matrix of TLDs/OSLDs.Main results.The investigated TLDs were shown to be dose rate independent within the experimental uncertainties, which take into account the uncertainty of the dosimetry protocol and the irradiation uncertainty. The relative deviation between the TLDs and the reference dose was lower than 4 % for all dose rates. A decreasing response with the dose rate was observed for Al2O3:C OSLDs, but still within 10 % from the reference dose.Significance.The precision of the investigated luminescence detectors make them suitable for dosimetry of ultra-high dose rate electron beams. Specifically, the dose rate independence of the TLDs can support the investigation of the beam uniformity as a function of the dose rate, which is one of the challenges of the employed beam. Al2O3:C OSLDs provided high precision measurements, but the decreasing response with the dose rate needs to be confirmed by additional experiments.


Assuntos
Elétrons , Radiometria , Radiometria/métodos , Luminescência , Água
4.
Phys Med Biol ; 68(4)2023 02 17.
Artigo em Inglês | MEDLINE | ID: mdl-36696696

RESUMO

Objective.This work aims at characterizing LiF:Mg,Ti thermoluminescence detectors (TLDs) for dosimetry of a 250 MeV proton beam delivered at ultra-high dose rates (UHDR). Possible dose rate effects in LiF:Mg,Ti, as well as its usability for dosimetry of narrow proton beams are investigated.Approach.LiF:Mg,Ti (TLD-100TMMicrocubes, 1 mm × 1 mm × 1 mm) was packaged in matrices of 5 × 5 detectors. The center of each matrix was irradiated with single-spot low-LET (energy >244 MeV) proton beam in the (1-4500) Gy s-1average dose rates range. A beam reconstruction procedure was applied to the detectors irradiated at the highest dose rate (Gaussian beam sigma <2 mm) to correct for volumetric averaging effects. Reference dosimetry was carried out with a diamond detector and radiochromic films. The delivered number of protons was measured by a Faraday cup, which was employed to normalize the detector responses.Main results.The lateral beam spread obtained from the beam reconstruction agreed with the one derived from the radiochromic film measurements. No dose rates effects were observed in LiF:Mg,Ti for the investigated dose rates within 3% (k= 1). On average, the dose response of the TLDs agreed with the reference detectors within their uncertainties. The largest deviation (-5%) was measured at 4500 Gy s-1.Significance.The dose rate independence of LiF:Mg,Ti TLDs makes them suitable for dosimetry of UHDR proton beams. Additionally, the combination of a matrix of TLDs and the beam reconstruction can be applied to determine the beam profile of narrow proton beams.


Assuntos
Prótons , Radioatividade , Titânio , Dosimetria Termoluminescente/métodos , Radiometria/métodos
5.
Phys Med ; 104: 101-111, 2022 Dec.
Artigo em Inglês | MEDLINE | ID: mdl-36395638

RESUMO

PURPOSE: To characterize an experimental setup for ultra-high dose rate (UHDR) proton irradiations, and to address the challenges of dosimetry in millimetre-small pencil proton beams. METHODS: At the PSI Gantry 1, high-energy transmission pencil beams can be delivered to biological samples and detectors up to a maximum local dose rate of âˆ¼9000 Gy/s. In the presented setup, a Faraday cup is used to measure the delivered number of protons up to ultra-high dose rates. The response of transmission ion-chambers, as well as of different field detectors, was characterized over a wide range of dose rates using the Faraday cup as reference. RESULTS: The reproducibility of the delivered proton charge was better than 1 % in the proposed experimental setup. EBT3 films, Al2O3:C optically stimulated luminescence detectors and a PTW microDiamond were used to validate the predicted dose. Transmission ionization chambers showed significant volume ion-recombination (>30 % in the tested conditions) which can be parametrized as a function of the maximum proton current density. Over the considered range, EBT3 films, inorganic scintillator-based screens and the PTW microDiamond were demonstrated to be dose rate independent within ±3 %, ±1.8 % and ±1 %, respectively. CONCLUSIONS: Faraday cups are versatile dosimetry instruments that can be used for dose estimation, field detector characterization and on-line dose verification for pre-clinical experiments in UHDR proton pencil beams. Among the tested detectors, the commercial PTW microDiamond was found to be a suitable option to measure real time the dosimetric properties of narrow pencil proton beams for dose rates up to 2.2 kGy/s.


Assuntos
Prótons , Reprodutibilidade dos Testes
6.
Radiat Prot Dosimetry ; 180(1-4): 196-200, 2018 Aug 01.
Artigo em Inglês | MEDLINE | ID: mdl-29036486

RESUMO

The objective of this study was to compare poly-allyl diglycol carbonate (PADC) track detectors from different suppliers for linear energy transfer (LET) spectrometry and neutron dosimetry. PADCs are commonly used for passive personal neutron dosimetry, where a common approach is to couple the PADC with a plastic radiator to generate secondary charged particles. The neutron dose can be estimated using the track density or the average LET of the secondary particles. The characterisation of PADC in terms of LET spectrometric capability and neutron sensitivity was previously performed using PADC from Intercast S.r.l., Parma, Italy, but this company stopped the production. Since it is common experience that material from different suppliers can have different properties, it became necessary to perform a comparison of PADCs from different suppliers with the Intercast material. The study permits to compare the reading procedures used at Politecnico di Milano and at the Paul Scherrer Institute.


Assuntos
Doses de Radiação , Monitoramento de Radiação/instrumentação , Proteção Radiológica/instrumentação , Radiometria/instrumentação , Nêutrons Rápidos , Glicóis/química , Nêutrons , Reprodutibilidade dos Testes , Sensibilidade e Especificidade
7.
Radiat Prot Dosimetry ; 180(1-4): 225-229, 2018 Aug 01.
Artigo em Inglês | MEDLINE | ID: mdl-29036622

RESUMO

The objective of this study was to compare a neutron dosimetry system based on polyallyl diglycol carbonate (PADC) detectors with a new system based on Al2O3:C,Mg fluorescence nuclear track detectors (FNTD). The irradiations, performed as part of an intercomparison organized by the Physikalisch-Technische Bundesanstalt (PTB), Germany, were on a PMMA phantom with 252Cf or 241Am-Be source, usually with the phantom surface perpendicular to the radiation beam (0° angle), and with Hp(10) values between 0.3 and 7 mSv. One 252Cf irradiation was performed at 30° angle, and one with an additional 1 mSv gamma irradiation. The results showed an agreement between the two techniques with an average and maximum difference between PADCs and FNTDs of 1.5 and 22%, respectively, if one compares only cases of doses >1 mSv. For one of the irradiation conditions with dose of 0.9 mSv, use of the incorrect calibration factor for the FNTD (252Cf instead of 241Am-Be) led to reported values ~×2 larger than the given doses, due to low statistics in the determination of the ratio between 6Li-doped glass and polyethylene neutron converters. Although the FNTD track analysis algorithm may need further development, the results presented here demonstrate the feasibility of the FNTD technology and indicate areas requiring improvements.


Assuntos
Glicóis/química , Nêutrons , Monitoramento de Radiação/instrumentação , Proteção Radiológica/instrumentação , Radiometria/instrumentação , Algoritmos , Calibragem , Nêutrons Rápidos , Fluorescência , Nylons/química , Imagens de Fantasmas , Polietileno/química , Doses de Radiação , Reprodutibilidade dos Testes
8.
Radiat Prot Dosimetry ; 180(1-4): 220-224, 2018 Aug 01.
Artigo em Inglês | MEDLINE | ID: mdl-29036689

RESUMO

The objective of this work is to demonstrate the possibility of performing fast neutron dosimetry up to 5 Sv using optical absorbance of polyallyl diglycol carbonate (PADC) detectors, obtained through grey level analysis of PADC images acquired with a commercial track-counting dosimetry system, and estimate the uncertainties involved. PADCs were irradiated with doses from 100 mSv to 5 Sv (252Cf source) and etched. PADC images were acquired using the TASLIMAGE™ Neutron Dosimetry System (Track Analysis Systems Ltd.) and analysed to obtain the grey levels and the optical absorbance. The absorbance from different detectors and batches was analysed to determine the uncertainties involved, from which the final uncertainty in the method, ~30% and dominated by the uncertainty in the calibration curve, was estimated. A dose estimation <2 Sv can also be performed using a 'universal curve' by normalising the absorbance to that of a detector irradiated with 1 Sv. The data presented here allows the extension of the dose range of track counting systems using no additional equipment, only the images already acquired by the systems.


Assuntos
Nêutrons Rápidos , Processamento de Imagem Assistida por Computador/métodos , Plásticos , Monitoramento de Radiação/instrumentação , Proteção Radiológica/instrumentação , Radiometria/instrumentação , Calibragem , Desenho de Equipamento , Doses de Radiação , Incerteza
9.
Phys Med Biol ; 61(21): 7551-7570, 2016 11 07.
Artigo em Inglês | MEDLINE | ID: mdl-27716632

RESUMO

This work evaluates the dosimetric properties of newly developed optically stimulated luminescence (OSL) films, fabricated with either Al2O3:C or Al2O3:C,Mg, using a prototype laser scanning reader, a developed image reconstruction algorithm, and a 6 MV therapeutic photon beam. Packages containing OSL films (Al2O3:C and Al2O3:C,Mg) and a radiochromic film (Gafchromic EBT3) were irradiated using a 6 MV photon beam using different doses, field sizes, with and without wedge filter. Dependence on film orientation of the OSL system was also tested. Diode-array (MapCHECK) and ionization chamber measurements were performed for comparison. The OSLD film doses agreed with the MapCHECK and ionization chamber data within the experimental uncertainties (<2% at 1.5 Gy). The system background and minimum detectable dose (MDD) were <0.5 mGy, and the dose response was approximately linear from the MDD up to a few grays (the linearity correction was <10% up to ~2-4 Gy), with no saturation up to 30 Gy. The dose profiles agreed with those obtained using EBT3 films (analyzed using the triple channel method) in the high dose regions of the images. In the low dose regions, the dose profiles from the OSLD films were more reproducible than those from the EBT3 films. We also demonstrated that the OSL film data are independent on scan orientation and field size over the investigated range. The results demonstrate the potential of OSLD films for 2D dosimetry, particularly for the characterization of small fields, due to their wide dynamic range, linear response, resolution and dosimetric properties. The negligible background and potential simple calibration make these OSLD films suitable for remote audits. The characterization presented here may motivate further commercial development of a 2D dosimetry system based on the OSL from Al2O3:C or Al2O3:C,Mg.


Assuntos
Algoritmos , Óxido de Alumínio/química , Dosimetria Fotográfica/instrumentação , Medições Luminescentes/instrumentação , Óptica e Fotônica , Calibragem , Relação Dose-Resposta à Radiação , Dosimetria Fotográfica/métodos
10.
Phys Med Biol ; 61(20): 7484-7506, 2016 10 21.
Artigo em Inglês | MEDLINE | ID: mdl-27694704

RESUMO

The objective of this work was to develop an image reconstruction algorithm for 2D dosimetry using Al2O3:C and Al2O3:C,Mg optically stimulated luminescence (OSL) films imaged using a laser scanning system. The algorithm takes into account parameters associated with detector properties and the readout system. Pieces of Al2O3:C films (~8 mm × 8 mm × 125 µm) were irradiated and used to simulate dose distributions with extreme dose gradients (zero and non-zero dose regions). The OSLD film pieces were scanned using a custom-built laser-scanning OSL reader and the data obtained were used to develop and demonstrate a dose reconstruction algorithm. The algorithm includes corrections for: (a) galvo hysteresis, (b) photomultiplier tube (PMT) linearity, (c) phosphorescence, (d) 'pixel bleeding' caused by the 35 ms luminescence lifetime of F-centers in Al2O3, (e) geometrical distortion inherent to Galvo scanning system, and (f) position dependence of the light collection efficiency. The algorithm was also applied to 6.0 cm × 6.0 cm × 125 µm or 10.0 cm × 10.0 cm × 125 µm Al2O3:C and Al2O3:C,Mg films exposed to megavoltage x-rays (6 MV) and 12C beams (430 MeV u-1). The results obtained using pieces of irradiated films show the ability of the image reconstruction algorithm to correct for pixel bleeding even in the presence of extremely sharp dose gradients. Corrections for geometric distortion and position dependence of light collection efficiency were shown to minimize characteristic limitations of this system design. We also exemplify the application of the algorithm to more clinically relevant 6 MV x-ray beam and a 12C pencil beam, demonstrating the potential for small field dosimetry. The image reconstruction algorithm described here provides the foundation for laser-scanned OSL applied to 2D dosimetry.


Assuntos
Processamento de Imagem Assistida por Computador/métodos , Magnésio/química , Dosimetria por Luminescência Estimulada Opticamente/métodos , Algoritmos , Óxido de Alumínio/química , Carbono/química , Lasers , Dosimetria por Luminescência Estimulada Opticamente/instrumentação
11.
Health Phys ; 98(2): 432-9, 2010 Feb.
Artigo em Inglês | MEDLINE | ID: mdl-20065717

RESUMO

Optically stimulated luminescence (OSL) properties of dental enamel are discussed with a view to the development of an in vivo dose assessment technique for medical triage following a radiological/nuclear accident or terrorist event. In the OSL technique, past radiation exposure is assessed by stimulating the sample with light of one wavelength and monitoring the luminescence at another wavelength, under the assumption that the luminescence originates from the recombination of radiation-induced charges trapped at metastable defects in the enamel and that the intensity of the luminescence signal is in proportion to the absorbed radiation dose. Several primary findings emerged from this research: (a) sensitivities varied considerably between different teeth and also between fragments of the same tooth, (b) OSL signals were found to decay rapidly during the first 12 h after irradiation and more slowly afterward, (c) the fading rate of the luminescence signal varied between fragments, and (d) blue light stimulation yields greater sensitivity than infra-red stimulation, while the OSL signal obtained with a high-intensity pulsed green-light laser was found not to be correlated with the radiation dose. Significant challenges remain to developing a practical in vivo technique, including the development of calibration procedures and lowering minimum detectable doses.


Assuntos
Bioensaio/métodos , Esmalte Dentário/química , Esmalte Dentário/efeitos da radiação , Exposição Ambiental/análise , Iluminação/métodos , Medições Luminescentes/métodos , Radiometria/métodos , Relação Dose-Resposta à Radiação , Humanos , Luz , Doses de Radiação , Reprodutibilidade dos Testes , Sensibilidade e Especificidade , Triagem/métodos
12.
Phys Med Biol ; 54(20): 6337-52, 2009 Oct 21.
Artigo em Inglês | MEDLINE | ID: mdl-19809126

RESUMO

This paper describes an LED-based optically stimulated luminescence (OSL) system for dose profile measurements using OSL detector strips and investigates its performance in x-ray computed tomography (CT) dosimetry. To compensate for the energy response of the Al(2)O(3):C OSL detectors, which have an effective atomic number of 11.28, field-specific energy correction factors were determined using two methods: (a) comparing the OSL profiles with ionization chamber point measurements (0.3 cm(3) ionization chamber) and (b) comparing the OSL profiles integrated over a 100 mm length with 100 mm long pencil ionization chamber measurements. These correction factors were obtained for the CT body and head phantoms, central and peripheral positions and three x-ray tube potential differences (100 kVp, 120 kVp and 140 kVp). The OSL dose profiles corrected by the energy dependence agreed with the ionization chamber point measurements over the entire length of the phantom (300 mm). For 120 kVp x-ray tube potential difference, the CTDI(100) values calculated using the OSL dose profiles corrected for the energy dependence and those obtained from an independent measurement with a 100 mm long pencil ionization chamber also agreed within +/-5%.


Assuntos
Luminescência , Imagens de Fantasmas , Tomografia Computadorizada por Raios X/métodos , Calibragem , Relação Dose-Resposta à Radiação , Cabeça/efeitos da radiação , Corpo Humano , Humanos , Óptica e Fotônica , Fótons , Pós , Doses de Radiação , Radiometria/métodos , Reprodutibilidade dos Testes
13.
Phys Med Biol ; 53(20): R351-79, 2008 Oct 21.
Artigo em Inglês | MEDLINE | ID: mdl-18799833

RESUMO

This paper reviews fundamental and practical aspects of optically stimulated luminescence (OSL) dosimetry pertaining to applications in medicine, having particularly in mind new researchers and medical physicists interested in gaining familiarity with the field. A basic phenomenological model for OSL is presented and the key processes affecting the outcome of an OSL measurement are discussed. Practical aspects discussed include stimulation modalities (continuous-wave OSL, pulsed OSL and linear modulation OSL), basic experimental setup, available OSL readers, optical fiber systems and basic properties of available OSL dosimeters. Finally, results from the recent literature on applications of OSL in radiotherapy, radiodiagnostics and heavy charged particle dosimetry are discussed in light of the theoretical and practical framework presented in this review. Open questions and future challenges in OSL dosimetry are highlighted as a guide to the research needed to further advance the field.


Assuntos
Medições Luminescentes/instrumentação , Medições Luminescentes/tendências , Dispositivos Ópticos/tendências , Radiometria/instrumentação , Radiometria/tendências , Desenho de Equipamento , Previsões , Medições Luminescentes/métodos , Radiometria/métodos , Avaliação da Tecnologia Biomédica
14.
Med Phys ; 35(1): 260-9, 2008 Jan.
Artigo em Inglês | MEDLINE | ID: mdl-18293581

RESUMO

This article investigates the performance of Al2O3: C optically stimulated luminescence dosimeters (OSLDs) for application in radiotherapy. Central-axis depth dose curves and optically stimulated luminescence (OSL) responses were obtained in a water phantom for 6 and 18 MV photons, and for 6, 9, 12, 16, and 20 MeV electron beams from a Varian 21EX linear accelerator. Single OSL measurements could be repeated with a precision of 0.7% (one standard deviation) and the differences between absorbed doses measured with OSLDs and an ionization chamber were within +/- 1% for photon beams. Similar results were obtained for electron beams in the low-gradient region after correction for a 1.9% photon-to-electron bias. The distance-to-agreement values were of the order of 0.5-1.0 mm for electrons in high dose gradient regions. Additional investigations also demonstrated that the OSL response dependence on dose rate, field size, and irradiation temperature is less than 1% in the conditions of the present study. Regarding the beam energy/quality dependence, the relative response of the OSLD for 18 MV was (0.51 +/- 0.48)% of the response for the 6 MV photon beam. The OSLD response for the electron beams relative to the 6 MV photon beam. The OSLD response for the electron beams relative to the 6 MV photon beam was in average 1.9% higher, but this result requires further confirmation. The relative response did not seem to vary with electron energy at dmax within the experimental uncertainties (0.5% in average) and, therefore, a fixed correction factor of 1.9% eliminated the energy dependence in our experimental conditions.


Assuntos
Óxido de Alumínio/química , Carbono/química , Elétrons , Luminescência , Óptica e Fotônica , Fótons , Doses de Radiação , Calibragem , Relação Dose-Resposta à Radiação , Humanos , Imagens de Fantasmas , Radioterapia de Alta Energia/métodos , Temperatura
15.
Radiat Meas ; 42(6): 1256-1260, 2007 Jul 01.
Artigo em Inglês | MEDLINE | ID: mdl-19623269

RESUMO

This paper briefly reviews the optically stimulated luminescence (OSL) properties of dental enamel and discusses the potential and challenges of OSL for filling the technology gap in biodosimetry required for medical triage following a radiological/nuclear accident or terrorist event. The OSL technique uses light to stimulate a radiation-induced luminescence signal from materials previously exposed to ionizing radiation. This luminescence originates from radiation-induced defects in insulating crystals and is proportional to the absorbed dose of ionizing radiation. In our research conducted to date, we focused on fundamental investigations of the OSL properties of dental enamel using extracted teeth and tabletop OSL readers. The objective was to obtain information to support the development of the necessary instrumentation for retrospective dosimetry using dental enamel in laboratory, or for in situ and non-invasive accident dosimetry using dental enamel in emergency triage. An OSL signal from human dental enamel was detected using blue, green, or IR stimulation. Blue/green stimulation associated with UV emission detection seems to be the most appropriate combination in the sense that there is no signal from un-irradiated samples and the shape of the OSL decay is clear. Improvements in the minimum detection level were achieved by incorporating an ellipsoidal mirror in the OSL system to maximize light collection. Other possibilities to improve the sensitivity and research steps necessary to establish the feasibility of the technique for retrospective assessment of radiation exposure are also discussed.

16.
Radiat Prot Dosimetry ; 119(1-4): 454-7, 2006.
Artigo em Inglês | MEDLINE | ID: mdl-16735565

RESUMO

We have developed a system to irradiate samples and record radioluminescence (RL), optically stimulated luminescence (OSL), and thermoluminescence (TL) at temperatures ranging from -150 degrees C to 200 degrees C. The system consists of a cryostat, an irradiation/stimulation unit fitted with an X-ray tube (40 kV Moxtek) and a quartz window for optical stimulation, and a detection unit that utilises a photomultiplier tube and an interchangeable filter pack. Experiments have been conducted with quartz and albite (a feldspar). TL and OSL experiments show that several optically sensitive trapping states are stable below -50 degrees C. In addition, an increase in OSL is seen as the OSL stimulation temperature is lowered below -50 degrees C, and an increase in RL is apparent as the temperature is lowered during irradiation. This indicates that not only are optically sensitive low temperature traps present but that luminescence becomes more efficient at low temperatures.


Assuntos
Algoritmos , Silicatos de Alumínio/análise , Silicatos de Alumínio/efeitos da radiação , Teste de Materiais/métodos , Compostos de Potássio/análise , Compostos de Potássio/efeitos da radiação , Quartzo/análise , Quartzo/efeitos da radiação , Dosimetria Termoluminescente/métodos , Temperatura
17.
Radiat Prot Dosimetry ; 119(1-4): 421-4, 2006.
Artigo em Inglês | MEDLINE | ID: mdl-16606659

RESUMO

A long-term in situ subsurface instrument for monitoring radioactive contaminant plumes, as an alternative to soil analysis, is described. A portable, laser-based reader optically stimulates luminescence from sensors, each containing an Al2O3:C dosemeter. The sensors, designed for placement at various subsurface locations around a waste site, are allowed to accumulate dose for a predetermined time that is based on the instrument's minimum detectable dose (MDD). The reader is then attached to the sensor by fibre optic cable to read the accumulated dose; an increase above natural background levels indicating the presence of leaked radioactivity. Based on an MDD of 5 microGy, it is shown that the sensor can measure soil concentrations of 1.85 Bq cm(-3) after an exposure time of 50 h for 137Cs and 67 h for 90Sr/90Y. Discrimination between beta and gamma radiation is possible using an end cap placed over one of the two paired sensors, allowing simultaneous measurement of 137Cs and 90Sr/90Y in a mixed field. The monitor system represents a substantial improvement over quarterly soil sampling because of a greatly increased measurement frequency and the ability to perform measurements reproducibly.


Assuntos
Tecnologia de Fibra Óptica/instrumentação , Proteção Radiológica/instrumentação , Resíduos Radioativos/análise , Dosimetria Termoluminescente/instrumentação , Relação Dose-Resposta à Radiação , Monitoramento Ambiental/métodos , Desenho de Equipamento , Análise de Falha de Equipamento , Tecnologia de Fibra Óptica/métodos , Teste de Materiais , Doses de Radiação , Proteção Radiológica/métodos , Reprodutibilidade dos Testes , Sensibilidade e Especificidade , Dosimetria Termoluminescente/métodos
18.
Radiat Prot Dosimetry ; 120(1-4): 354-7, 2006.
Artigo em Inglês | MEDLINE | ID: mdl-16644985

RESUMO

This paper presents two different approaches of quantifying the optically stimulated luminescence (OSL) response of Al(2)O(3):C to high-energy heavy charged particles (HCPs). The OSL efficiency of Al(2)O(3):C exposed to different HCPs is defined as the sensitivity of the material to HCPs normalised by the sensitivity to gamma. In this paper, we investigate the possibility of introducing a 'mean efficiency' eta(mean), which when used in conjunction with the total gamma dose D(gamma) measured for a mixed radiation exposure allows for the determination of the absorbed dose without the need to determine the individual contributions of different types of radiation to the OSL signal. We tested the hypothesis that information regarding the 'mean efficiency' eta(mean) is contained in the shape of the OSL decay curve, using several approaches in the analysis of the OSL data. This analysis was applied to various mixed field irradiations performed at the HIMAC facility, Chiba, Japan. The results of this analysis are discussed.


Assuntos
Óxido de Alumínio/química , Óxido de Alumínio/efeitos da radiação , Íons Pesados , Modelos Químicos , Nêutrons , Dosimetria Termoluminescente/instrumentação , Dosimetria Termoluminescente/métodos , Simulação por Computador , Relação Dose-Resposta à Radiação , Desenho de Equipamento , Análise de Falha de Equipamento , Luz , Teste de Materiais , Doses de Radiação , Reprodutibilidade dos Testes , Sensibilidade e Especificidade
19.
Radiat Prot Dosimetry ; 120(1-4): 433-7, 2006.
Artigo em Inglês | MEDLINE | ID: mdl-16644947

RESUMO

The laboratory of Microbiology at SCK.CEN, in collaboration with different universities, participates in several ESA programmes with bacterial experiments that are carried out in the International Space Station (ISS). The main objective of these programmes is to study the effects of space flight conditions such as microgravity and cosmic radiation on the general behaviour of model bacteria. To measure the radiation doses received by the bacteria, different detectors accompanied the microbiological experiments. The results obtained during two space flight missions are discussed. This dosimetry experiment was a collaboration between different institutes so that the doses could be estimated by different techniques. For measurement of the high linear energy transfer (LET) doses (>10 keV microm(-1)), two types of etched track detectors were used. The low LET part of the spectrum was measured by three types of thermoluminescent detectors ((7)LiF:Mg,Ti; (7)LiF:Mg,Cu,P; Al(2)O(3):C) and by the optically stimulated luminescence technique using Al(2)O(3):C detectors.


Assuntos
Radiação Cósmica , Microbiologia/instrumentação , Exposição Ocupacional/análise , Proteção Radiológica/instrumentação , Voo Espacial/instrumentação , Dosimetria Termoluminescente/instrumentação , Relação Dose-Resposta à Radiação , Desenho de Equipamento , Análise de Falha de Equipamento , Doses de Radiação , Reprodutibilidade dos Testes , Sensibilidade e Especificidade , Voo Espacial/métodos , Propriedades de Superfície , Dosimetria Termoluminescente/métodos
20.
Radiat Prot Dosimetry ; 119(1-4): 450-3, 2006.
Artigo em Inglês | MEDLINE | ID: mdl-16565207

RESUMO

Published single-aliquot regenerative-dose (SAR) procedures for quartz use a 'cutheat' different from the pre-heat. In contrast, previous work has shown that the SAR procedure can be used to correct for sensitivity changes exhibited by feldspars if the cutheat is equal to the pre-heat. In this paper, a procedure that corrects for sensitivity changes in both quartz and feldspar is tested. The results indicate that for sedimentary quartz the cutheat can be equal to the pre-heat. Thus, it may be possible to develop one procedure to measure equivalent doses in a polymineral sample. We also tested several different optical stimulation methods. Using the infrared (IR)-stimulated signal from a post-IR blue-stimulated optically stimulated luminescence sequence extends the potential age range when using feldpathic materials. In addition, since the post-IR blue-stimulated signal from feldspar is much smaller than the blue-stimulated signal from quartz, the possibility exists of extracting a 'quartz signal' from a mixed mineral sample.


Assuntos
Algoritmos , Silicatos de Alumínio/análise , Silicatos de Alumínio/efeitos da radiação , Geologia/métodos , Teste de Materiais/métodos , Minerais/análise , Minerais/efeitos da radiação , Compostos de Potássio/análise , Compostos de Potássio/efeitos da radiação , Dosimetria Termoluminescente/métodos , Meia-Vida , Temperatura Alta , Luz
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