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1.
ACS Omega ; 7(40): 35840-35850, 2022 Oct 11.
Artigo em Inglês | MEDLINE | ID: mdl-36249369

RESUMO

The sandstone aquifer is an important underground water storage space, and the study of its water abundance is of great significance to ensure the safety of underground engineering and to explore the occurrence mechanism of groundwater sources. Based on the correlation between geological characteristics and aquifer water abundance, this paper proposed an aquifer water abundance prediction model based on a cloud model that improved combination weighting. The model took the roof sandstone aquifer of the Qingshuiying Coalfield as an example and selected five basic geological indicators that are closely related to the water-rich influence degree of the aquifer as evaluation indicators. The model was based on the idea of game theory, combined the analytic hierarchy process (AHP) and the entropy weight method, and introduced the cloud model evaluation method. The establishment of the model was based on the idea of game theory, combining the AHP and the entropy weight method and introducing the cloud model evaluation method. The results show that most of the study areas are located in weak or relatively weak water abundance areas; relatively strong water abundance areas are mainly distributed in the central, western, and southeastern parts of the study; strong water abundance areas are scattered in parts of the northeast, southwest, and southeast. The unit water inflow data of the actual pumping test is consistent with the water-rich prediction partition, which proves the accuracy and scientificity of the method. The model provides a new idea for the study of groundwater geology and a new method for predicting the water abundance of the roof aquifer in coal mines.

2.
RSC Adv ; 12(10): 5768, 2022 Feb 16.
Artigo em Inglês | MEDLINE | ID: mdl-35427080

RESUMO

[This corrects the article DOI: 10.1039/D1RA07500D.].

3.
Polymers (Basel) ; 14(3)2022 Feb 08.
Artigo em Inglês | MEDLINE | ID: mdl-35160627

RESUMO

The requirements regarding the weight and capacity reduction of neutron shielding materials have become an urgent issue for advanced nuclear facilities and plants. An epoxy-based neutron shielding material with high-temperature stability and good neutron irradiation resistance was designed in this paper to solve the above issue. Aminophenol trifunctional epoxy resin (AFG-90H) was compounded with samarium oxide (Sm2O3) by means of an ultrasonic-assisted method and the compatibility of Sm2O3 with the AFG-90H matrix was improved by 3-aminopropyltriethoxysilane (APTES) surface modification. Fabricated Sm2O3-APTES/AFG-90H composites exhibited improved thermal stability, glass transition temperature and Young's modulus with increased Sm2O3-APTES content. Neutronics calculation results show that the neutron permeability of 2 mm-thick 30 wt% Sm2O3-APTES/AFG-90H was 98.9% higher than that of the AFG-90H matrix under the irradiation of the thermal neutron source. The results show that the proper addition range of Sm2O3-APTES is between 20% and 25%. The Sm2O3-APTES/AFG-90H composite is a promising neutron shielding material for advanced nuclear system.

4.
RSC Adv ; 11(63): 40148-40158, 2021 12 13.
Artigo em Inglês | MEDLINE | ID: mdl-35424325

RESUMO

None of the currently commercialized shielding materials in Generation IV nuclear energy systems are satisfactory in their performance. Developing a candidate neutron shielding material with good heat resistance and high strength is a challenging task. In this work, various gadolinium metal-organic frameworks (Gd-MOFs) with obvious advantages, such as porous structures, organic surfaces and strong neutron-absorbing nuclei, were synthesized to constrain polyimide (PI) chains. A series of Gd-MOF/PI conjugates were subsequently assessed for their thermal stability, mechanical properties and neutron shielding performance. The increase of the Gd-MOF content improved the thermal neutron shielding ability but slightly reduced the fast neutron shielding ability. Compared with those of pure PI, the Gd-MOF/PI films demonstrate a higher glass transition temperature (T g), which is considered the gold standard of engineering plastics. It was also observed that the tensile strength directly correlates with the Gd-MOF content, which continuously increases until a maximum is reached, and then subsequently decreases. Furthermore, the high-temperature tensile test showed that these tunable Gd-MOF/PI films are intact and robust, indicating their potential application for neutron shielding materials in Generation IV nuclear energy systems.

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