Experimental Demonstration of Effective Medium Approximation Breakdown in Deeply Subwavelength All-Dielectric Multilayers.

We report the first experimental demonstration of anomalous breakdown of the effective medium approximation in all-dielectric deeply subwavelength thickness (d∼λ/160-λ/30) multilayers, as recently predicted theoretically [H. H. Sheinfux et al., Phys. Rev. Lett. 113, 243901 (2014)]. Multilayer stacks are composed of alternating alumina and titania layers fabricated using atomic layer deposition. For light incident on such multilayers at angles near the total internal reflection, we observe pronounced differences in the reflectance spectra for structures with 10- vs 20-nm thick layers, as well as for structures with different layers ordering, contrary to the predictions of the effective medium approximation. The reflectance difference can reach values up to 0.5, owing to the chosen geometrical configuration with an additional resonator layer employed for the enhancement of the effect. Our results are important for the development of new high-precision multilayer ellipsometry methods and schemes, as well as in a broad range of sensing applications.

Dark-field hyperlens: Super-resolution imaging of weakly scattering objects.

We propose a device for subwavelength optical imaging based on a metal-dielectric multilayer hyperlens designed in such a way that only large-wavevector (evanescent) waves are transmitted while all propagating (small-wavevector) waves from the object area are blocked by the hyper-lens. We numerically demonstrate that as the result of such filtering, the image plane only contains scattered light from subwavelength features of the objects and is completely free from background illumination. Similar in spirit to conventional dark-field microscopy, the proposed dark-field hyperlens is shown to enhance the subwavelength image contrast by more than two orders of magnitude. These findings are essential for optical imaging of weakly scattering subwavelength objects, such as real-time dynamic nanoscopy of label-free biological objects.

Water: Promising Opportunities For Tunable All-dielectric Electromagnetic Metamaterials.

We reveal an outstanding potential of water as an inexpensive, abundant and bio-friendly high-refractive-index material for creating tunable all-dielectric photonic structures and metamaterials. Specifically, we demonstrate thermal, mechanical and gravitational tunability of magnetic and electric resonances in a metamaterial consisting of periodically positioned water-filled reservoirs. The proposed water-based metamaterials can find applications not only as cheap and ecological microwave devices, but also in optical and terahertz metamaterials prototyping and educational lab equipment.

Anomalous effective medium approximation breakdown in deeply subwavelength all-dielectric photonic multilayers.

We present a comprehensive analysis of the applicability of the effective medium approximation to deeply subwavelength (period ≤λ/50 all-dielectric multilayer structures. We demonstrate that even though the dispersion relations for such multilayers differ from the effective medium prediction only slightly, there can be regimes when an actual multilayer stack exhibits significantly different properties compared to its homogenized model. In particular, reflection near the critical angle is shown to strongly depend on even very small period variations, as well as on the choice of the multilayer termination. We identify the geometries for which the influence of the subwavelength features is maximized and demonstrate that the difference between the reflectance from the actual multilayer and the effective medium prediction can be as great as 0.98. The results of this analysis can be useful for high-precision multilayer ellipsometry and in sensing applications.

Bismuth ferrite as low-loss switchable material for plasmonic waveguide modulator.

We propose new designs of plasmonic modulators, which can be used for dynamic signal switching in photonic integrated circuits. We study performance of a plasmonic waveguide modulator with bismuth ferrite as a tunable material. The bismuth ferrite core is sandwiched between metal plates (metal-insulator-metal configuration), which also serve as electrodes. The core changes its refractive index by means of partial in-plane to out-of-plane reorientation of ferroelectric domains in bismuth ferrite under applied voltage. As a result, guided modes change their propagation constant and absorption coefficient, allowing light modulation in both phase and amplitude control schemes. Due to high field confinement between the metal layers, existence of mode cut-offs for certain values of the core thickness, and near-zero material losses in bismuth ferrite, efficient modulation performance is achieved. For the phase control scheme, the π phase shift is provided by a 0.8-µm long device with propagation losses 0.29 dB/µm. For the amplitude control scheme, up to 38 dB/µm extinction ratio with 1.2 dB/µm propagation loss is predicted.

Rough metal and dielectric layers make an even better hyperbolic metamaterial absorber.

We numerically investigate the influence of roughness in layer thicknesses on the properties of hyperbolic metamaterials (HMMs). We show that random spatial variation of dielectric and metal layer thicknesses, similar to what occurs during actual structure fabrication, leads to dramatic absorption increase compared to an ideal, smooth-layer HMM; the absorption increases more strongly when roughness is induced throughout the HMM rather than in its surface layer only. Hence, we have found that moderate surface roughness does not deteriorate the HMM functionality, at least in absorption-related applications, thus eliminating the challenge of ultrasmooth metal layer fabrication. More severe roughness can also prove useful in the design of inexpensive HMM-based broadband absorbers.

Internal photoemission from plasmonic nanoparticles: comparison between surface and volume photoelectric effects.

We study the emission of photoelectrons from plasmonic nanoparticles into a surrounding matrix. We consider two mechanisms of electron emission from the nanoparticles--surface and volume ones--and use models for these two mechanisms which allow us to obtain analytical results for the photoelectron emission rate from a nanoparticle. Calculations have been carried out for a step potential at the surface of a spherical nanoparticle, and a simple model for the hot electron cooling has been used. We highlight the effect of the discontinuity of the dielectric permittivity at the nanoparticle boundary in the surface mechanism, which leads to a substantial (by ∼5 times) increase of the internal photoelectron emission rate from a nanoparticle compared to the case when such a discontinuity is absent. For a plasmonic nanoparticle, a comparison of the two photoeffect mechanisms was undertaken for the first time which showed that the surface photoeffect can in the general case be larger than the volume one, which agrees with the results obtained for a flat metal surface first formulated by Tamm and Schubin in their pioneering development of a quantum-mechanical theory of photoeffect in 1931. In accordance with our calculations, this possible predominance of the surface effect is based on two factors: (i) effective cooling of hot carriers during their propagation from the volume of the nanoparticle to its surface in the scenario of the volume mechanism and (ii) strengthening of the surface mechanism through the effect of the discontinuity of the dielectric permittivity at the nanoparticle boundary. The latter is stronger at relatively lower photon energies and correspondingly is more substantial for internal photoemission than for an external one. We show that in the general case, it is essential to take both mechanisms into account in the development of devices based on the photoelectric effect and when considering hot electron emission from a plasmonic nanoantenna.

Inherent polarization entanglement generated from a monolithic semiconductor chip.

Creating miniature chip scale implementations of optical quantum information protocols is a dream for many in the quantum optics community. This is largely because of the promise of stability and scalability. Here we present a monolithically integratable chip architecture upon which is built a photonic device primitive called a Bragg reflection waveguide (BRW). Implemented in gallium arsenide, we show that, via the process of spontaneous parametric down conversion, the BRW is capable of directly producing polarization entangled photons without additional path difference compensation, spectral filtering or post-selection. After splitting the twin-photons immediately after they emerge from the chip, we perform a variety of correlation tests on the photon pairs and show non-classical behaviour in their polarization. Combined with the BRW's versatile architecture our results signify the BRW design as a serious contender on which to build large scale implementations of optical quantum processing devices.

Physical nature of volume plasmon polaritons in hyperbolic metamaterials.

We investigate electromagnetic wave propagation in multilayered metal-dielectric hyperbolic metamaterials (HMMs). We demonstrate that high-k propagating waves in HMMs are volume plasmon polaritons. The volume plasmon polariton band is formed by coupling of short-range surface plasmon polariton excitations in the individual metal layers.

Dipole radiation near hyperbolic metamaterials: applicability of effective-medium approximation.

We investigate the radiation rate of a dipole in close proximity to a hyperbolic metamaterial and confirm that both the radiation rate and its fraction directed into the metamaterial are greatly increased compared to bulk dielectric or metal. However, we find that the homogenized effective-medium approach greatly overestimates the Purcell factor compared to metal-dielectric subwavelength multilayers with previously reported layer thicknesses.

Plasmonic rod dimers as elementary planar chiral meta-atoms.

We theoretically calculate the electromagnetic response of metallic rod dimers for the arbitrary planar arrangement of rods in the dimer. It is shown that dimers without an in-plane symmetry axis exhibit elliptical dichroism and act as "atoms" in planar chiral metamaterials. Because of a very simple geometry of the rod dimer, such planar metamaterials are much easier to fabricate than conventional split-ring or gammadion-type structures and lend themselves to a simple analytical treatment based on a coupled dipole model. Dependencies of the metamaterial's directional asymmetry on the dimer's geometry are established analytically and confirmed in numerical simulations.

Optical memory based on ultrafast wavelength switching in a bistable microlaser.

We propose an optical memory cell based on ultrafast wavelength switching in coupled-cavity microlasers, featuring bistability between modes separated by several nanometers. A numerical implementation is demonstrated by simulating a two-dimensional photonic crystal microlaser. Switching times of less than 10 ps, switching energy around 15-30 fJ, and on-off contrast of more than 40 dB are achieved. Theoretical guidelines for optimizing the performance of the memory cell in terms of switching time and energy are drawn.

Elliptical dichroism: operating principle of planar chiral metamaterials.

We employ a homogenization technique based on the Lorentz electronic theory to show that planar chiral structures (PCSs) can be described by an effective dielectric tensor similar to that of biaxial elliptically dichroic crystals. Such a crystal is shown to behave like a PCS insofar as it exhibits its characteristic optical properties, namely, corotating elliptical polarization eigenstates and asymmetric, direction-dependent transmission for left- or right-handed incident wave polarization.

Switchable lasing in multimode microcavities.

We propose the new concept of a switchable multimode microlaser. As a generic, realistic model of a multimode microresonator a system of two coupled defects in a two-dimensional photonic crystal is considered. We demonstrate theoretically that lasing of the cavity into one selected resonator mode can be caused by injecting an appropriate optical pulse at the onset of laser action (injection seeding). Temporal mode-to-mode switching by reseeding the cavity after a short cooldown period is demonstrated by direct numerical solution. A qualitative analytical explanation of the mode switching in terms of the laser bistability is presented.