Spin-orbit mediated interference in the radiative and nonradiative channels of the La 4d core resonances.
Phys Rev Lett
; 103(13): 137401, 2009 Sep 25.
Article
em En
| MEDLINE
| ID: mdl-19905539
ABSTRACT
Symmetrical fluorescence yield profiles and asymmetrical electron yield profiles of the preresonances at the La N_{IV,V} x-ray absorption edge are experimentally observed in LaPO_{4} nanoparticles. Theoretical studies show that they are caused by interference effects. The spin-orbit interaction and the giant resonance produce symmetry entangled intermediate states that activate coherent scattering and alter the spectral distribution of the oscillator strength. The scattering amplitudes of the electron and fluorescence decays are further modified by the spin-orbit coupling in the final 5p;{5}epsilonl and 5p;{5}4f;{1} states.
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Coleções:
01-internacional
Base de dados:
MEDLINE
Idioma:
En
Revista:
Phys Rev Lett
Ano de publicação:
2009
Tipo de documento:
Article
País de afiliação:
Alemanha