Behavior of Per- and polyfluoroalkyl substances (PFAS) in Pilot-Scale vertical flow constructed wetlands treating landfill leachate.
Waste Manag
; 161: 187-192, 2023 Apr 15.
Article
em En
| MEDLINE
| ID: mdl-36893712
ABSTRACT
This study investigated the behavior of per- and polyfluoroalkyl substances (PFAS) in multiple pilot-scale vertical flow constructed wetlands (VFCW) treating landfill leachate. Eight pilot-scale VFCW columns planted with Typha latifolia or Scirpus Californicus were fed untreated municipal solid waste (MSW) landfill leachate that was diluted with potable water at a 110 ratio (1 part leachate to 10 parts total) at a fixed daily hydraulic loading rate of 0.525 m d-1. Ninety-two PFAS were examined and 18 PFAS were detected at quantifiable concentrations (7 precursor species and 11 terminal species). The average concentration of Σ92 PFAS in the influent was 3,100 ng L-1, which corresponded with minimal reduction in the effluents from the four VFCW (decreases ranged from 1% to 12% on average for Σ18 PFAS); however, precursors 63 FTCA, 73 FTCA, N-MeFOSAA, and N-EtFOSAA concentrations decreased significantly in the VFCW effluents, and significant decreases in the concentrations of these PFAA-precursors were concurrent with a significant increase in concentrations of five PFAAs (PFBA, PFNA, PFBS, PFOS, and PFOSI). This trend indicates that from a regulatory perspective, standalone VFCWs are likely to produce an apparent PFAS increase, which may also be true for many other leachate treatment processes incorporating aerobic biological treatment. Additional treatment to address PFAS should be integrated prior to the use of any system, including VFCWs, for the treatment of constituents of concern in MSW landfill leachate.
Palavras-chave
Texto completo:
1
Coleções:
01-internacional
Base de dados:
MEDLINE
Assunto principal:
Poluentes Químicos da Água
/
Fluorocarbonos
Idioma:
En
Revista:
Waste Manag
Assunto da revista:
SAUDE AMBIENTAL
/
TOXICOLOGIA
Ano de publicação:
2023
Tipo de documento:
Article
País de afiliação:
Estados Unidos
País de publicação:
EEUU
/
ESTADOS UNIDOS
/
ESTADOS UNIDOS DA AMERICA
/
EUA
/
UNITED STATES
/
UNITED STATES OF AMERICA
/
US
/
USA