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Enantioselective Synthesis of Axially Chiral Sulfone-Containing Styrenes Based on Ion-Exchange Strategy.
Lian, Peng-Fei; Wang, Ying; Li, Zi-Hao; Zhang, Shu-Yu; Duan, Abing; Bai, He-Yuan.
Afiliação
  • Lian PF; Shanghai Key Laboratory for Molecular Engineering of Chiral Drugs, and School of Chemistry and Chemical Engineering, Shanghai Jiao Tong University, Shanghai 200240, P. R. China.
  • Wang Y; College of Environmental Science and Engineering, Hunan University, Changsha 410082, P. R. China.
  • Li ZH; Shanghai Key Laboratory for Molecular Engineering of Chiral Drugs, and School of Chemistry and Chemical Engineering, Shanghai Jiao Tong University, Shanghai 200240, P. R. China.
  • Zhang SY; Shanghai Key Laboratory for Molecular Engineering of Chiral Drugs, and School of Chemistry and Chemical Engineering, Shanghai Jiao Tong University, Shanghai 200240, P. R. China.
  • Duan A; College of Environmental Science and Engineering, Hunan University, Changsha 410082, P. R. China.
  • Bai HY; Shanghai Key Laboratory for Molecular Engineering of Chiral Drugs, and School of Chemistry and Chemical Engineering, Shanghai Jiao Tong University, Shanghai 200240, P. R. China.
Org Lett ; 26(17): 3498-3502, 2024 May 03.
Article em En | MEDLINE | ID: mdl-38661476
ABSTRACT
A novel ion exchange strategy has been developed to enable the asymmetric construction of axially chiral sulfone-containing styrenes. This approach provides a practical synthesis pathway for various axially chiral sulfone-containing styrenes with good yields, exceptional enantioselectivities, and nearly complete E/Z selectivities. Additionally, the reaction mechanism is elucidated in detail through density functional theory (DFT) calculations.
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Texto completo: 1 Coleções: 01-internacional Base de dados: MEDLINE Idioma: En Revista: Org Lett Assunto da revista: BIOQUIMICA Ano de publicação: 2024 Tipo de documento: Article País de publicação: Estados Unidos
Texto completo
Adicionar na Minha BVS
Imprimir
XML
PubMed Links
Buscar no Google

Texto completo: 1 Coleções: 01-internacional Base de dados: MEDLINE Idioma: En Revista: Org Lett Assunto da revista: BIOQUIMICA Ano de publicação: 2024 Tipo de documento: Article País de publicação: Estados Unidos