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1.
Nano Lett ; 24(2): 601-606, 2024 Jan 17.
Artigo em Inglês | MEDLINE | ID: mdl-38180909

RESUMO

Electronic spectra of solids subjected to a magnetic field are often discussed in terms of Landau levels and Hofstadter-butterfly-style Brown-Zak minibands manifested by magneto-oscillations in two-dimensional electron systems. Here, we present the semiclassical precursors of these quantum magneto-oscillations which appear in graphene superlattices at low magnetic field near the Lifshitz transitions and persist at elevated temperatures. These oscillations originate from Aharonov-Bohm interference of electron waves following open trajectories that belong to a kagome-shaped network of paths characteristic for Lifshitz transitions in the moire superlattice minibands of twistronic graphenes.

2.
Proc Natl Acad Sci U S A ; 110(9): 3282-6, 2013 Feb 26.
Artigo em Inglês | MEDLINE | ID: mdl-23401538

RESUMO

Capacitance measurements provide a powerful means of probing the density of states. The technique has proved particularly successful in studying 2D electron systems, revealing a number of interesting many-body effects. Here, we use large-area high-quality graphene capacitors to study behavior of the density of states in this material in zero and high magnetic fields. Clear renormalization of the linear spectrum due to electron-electron interactions is observed in zero field. Quantizing fields lead to splitting of the spin- and valley-degenerate Landau levels into quartets separated by interaction-enhanced energy gaps. These many-body states exhibit negative compressibility but the compressibility returns to positive in ultrahigh B. The reentrant behavior is attributed to a competition between field-enhanced interactions and nascent fractional states.

3.
Nat Nanotechnol ; 8(2): 100-3, 2013 Feb.
Artigo em Inglês | MEDLINE | ID: mdl-23263726

RESUMO

The celebrated electronic properties of graphene have opened the way for materials just one atom thick to be used in the post-silicon electronic era. An important milestone was the creation of heterostructures based on graphene and other two-dimensional crystals, which can be assembled into three-dimensional stacks with atomic layer precision. Such layered structures have already demonstrated a range of fascinating physical phenomena, and have also been used in demonstrating a prototype field-effect tunnelling transistor, which is regarded to be a candidate for post-CMOS (complementary metal-oxide semiconductor) technology. The range of possible materials that could be incorporated into such stacks is very large. Indeed, there are many other materials with layers linked by weak van der Waals forces that can be exfoliated and combined together to create novel highly tailored heterostructures. Here, we describe a new generation of field-effect vertical tunnelling transistors where two-dimensional tungsten disulphide serves as an atomically thin barrier between two layers of either mechanically exfoliated or chemical vapour deposition-grown graphene. The combination of tunnelling (under the barrier) and thermionic (over the barrier) transport allows for unprecedented current modulation exceeding 1 × 10(6) at room temperature and very high ON current. These devices can also operate on transparent and flexible substrates.

4.
Nano Lett ; 12(9): 4629-34, 2012 Sep 12.
Artigo em Inglês | MEDLINE | ID: mdl-22935053

RESUMO

The above question is frequently asked by theorists who are interested in graphene as a model system, especially in context of relativistic quantum physics. We offer an experimental answer by describing electron transport in suspended devices with carrier mobilities of several 10(6) cm(2) V(-1) s(-1) and with the onset of Landau quantization occurring in fields below 5 mT. The observed charge inhomogeneity is as low as ≈10(8) cm(-2), allowing a neutral state with a few charge carriers per entire micrometer-scale device. Above liquid helium temperatures, the electronic properties of such devices are intrinsic, being governed by thermal excitations only. This yields that the Dirac point can be approached within 1 meV, a limit currently set by the remaining charge inhomogeneity. No sign of an insulating state is observed down to 1 K, which establishes the upper limit on a possible bandgap.


Assuntos
Grafite/química , Modelos Químicos , Simulação por Computador , Transporte de Elétrons , Eletricidade Estática
5.
Nano Lett ; 12(3): 1707-10, 2012 Mar 14.
Artigo em Inglês | MEDLINE | ID: mdl-22380756

RESUMO

We investigate the electronic properties of ultrathin hexagonal boron nitride (h-BN) crystalline layers with different conducting materials (graphite, graphene, and gold) on either side of the barrier layer. The tunnel current depends exponentially on the number of h-BN atomic layers, down to a monolayer thickness. Conductive atomic force microscopy scans across h-BN terraces of different thickness reveal a high level of uniformity in the tunnel current. Our results demonstrate that atomically thin h-BN acts as a defect-free dielectric with a high breakdown field. It offers great potential for applications in tunnel devices and in field-effect transistors with a high carrier density in the conducting channel.


Assuntos
Compostos de Boro/química , Nanoestruturas/química , Nanoestruturas/ultraestrutura , Semicondutores , Condutividade Elétrica , Transporte de Elétrons , Teste de Materiais , Tamanho da Partícula
6.
Nano Lett ; 11(6): 2396-9, 2011 Jun 08.
Artigo em Inglês | MEDLINE | ID: mdl-21574627

RESUMO

Devices made from graphene encapsulated in hexagonal boron-nitride exhibit pronounced negative bend resistance and an anomalous Hall effect, which are a direct consequence of room-temperature ballistic transport at a micrometer scale for a wide range of carrier concentrations. The encapsulation makes graphene practically insusceptible to the ambient atmosphere and, simultaneously, allows the use of boron nitride as an ultrathin top gate dielectric.


Assuntos
Compostos de Boro/química , Grafite/química , Temperatura , Eletrônica , Propriedades de Superfície
8.
Nano Lett ; 8(6): 1704-8, 2008 Jun.
Artigo em Inglês | MEDLINE | ID: mdl-18444691

RESUMO

Graphene is only one atom thick, optically transparent, chemically inert, and an excellent conductor. These properties seem to make this material an excellent candidate for applications in various photonic devices that require conducting but transparent thin films. In this letter, we demonstrate liquid crystal devices with electrodes made of graphene that show excellent performance with a high contrast ratio. We also discuss the advantages of graphene compared to conventionally used metal oxides in terms of low resistivity, high transparency and chemical stability.


Assuntos
Cristalização/métodos , Grafite/química , Cristais Líquidos/química , Nanoestruturas/química , Nanoestruturas/ultraestrutura , Nanotecnologia/métodos , Impedância Elétrica , Luz , Substâncias Macromoleculares/química , Teste de Materiais , Conformação Molecular , Tamanho da Partícula , Propriedades de Superfície
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